Performances of halide scintillators for the dosimetry based on gamma-ray spectrometry for environmental monitoring systems

High pressure ion chambers (HPIC) and NaI(Tl) scintillation detectors are widely used to monitor the ambient dose equivalent rate H∗(10) within and around the Korean nuclear facilities. However, HPIC cannot provide spectrometric information and NaI(Tl) detector is limited in identifying nuclides, su...

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Main Authors: Wanook Ji, Eunjoong Lee, Young-Yong Ji
Format: Article
Language:English
Published: Elsevier 2025-02-01
Series:Nuclear Engineering and Technology
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S1738573324004212
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author Wanook Ji
Eunjoong Lee
Young-Yong Ji
author_facet Wanook Ji
Eunjoong Lee
Young-Yong Ji
author_sort Wanook Ji
collection DOAJ
description High pressure ion chambers (HPIC) and NaI(Tl) scintillation detectors are widely used to monitor the ambient dose equivalent rate H∗(10) within and around the Korean nuclear facilities. However, HPIC cannot provide spectrometric information and NaI(Tl) detector is limited in identifying nuclides, such as 131I, 134Cs, and 137Cs, released from nuclear facilities owing to its insufficient energy resolution. This study employed four halide scintillators – LaBr3(Ce), CeBr3, and SrI2(Eu) – to measure the ambient dose equivalent rate and detect gamma nuclides from measured energy spectrum. First, the pulse–shaping time in the signal processing unit was optimized for each scintillator. Second, energy resolution and counting efficiency were estimated for 137Cs and 60Co. Finally, an irradiation test was performed to estimate the dose rate. Based on these results, LaBr3(Ce) and NaI(Tl) were selected as in situ gamma spectrometry system for measuring environmental radiation, and field experiments were conducted near the Fukushima Daiichi nuclear power plant to measure the dose rate.
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spelling doaj-art-ff352156cb0f40d3a27d0110924c16692025-01-31T05:10:59ZengElsevierNuclear Engineering and Technology1738-57332025-02-01572103173Performances of halide scintillators for the dosimetry based on gamma-ray spectrometry for environmental monitoring systemsWanook Ji0Eunjoong Lee1Young-Yong Ji2Korea Atomic Energy Research Institute, Daejeon, 34057, Republic of KoreaKorea Atomic Energy Research Institute, Daejeon, 34057, Republic of KoreaCorresponding author.; Korea Atomic Energy Research Institute, Daejeon, 34057, Republic of KoreaHigh pressure ion chambers (HPIC) and NaI(Tl) scintillation detectors are widely used to monitor the ambient dose equivalent rate H∗(10) within and around the Korean nuclear facilities. However, HPIC cannot provide spectrometric information and NaI(Tl) detector is limited in identifying nuclides, such as 131I, 134Cs, and 137Cs, released from nuclear facilities owing to its insufficient energy resolution. This study employed four halide scintillators – LaBr3(Ce), CeBr3, and SrI2(Eu) – to measure the ambient dose equivalent rate and detect gamma nuclides from measured energy spectrum. First, the pulse–shaping time in the signal processing unit was optimized for each scintillator. Second, energy resolution and counting efficiency were estimated for 137Cs and 60Co. Finally, an irradiation test was performed to estimate the dose rate. Based on these results, LaBr3(Ce) and NaI(Tl) were selected as in situ gamma spectrometry system for measuring environmental radiation, and field experiments were conducted near the Fukushima Daiichi nuclear power plant to measure the dose rate.http://www.sciencedirect.com/science/article/pii/S1738573324004212Halide scintillatorsDosimetryGamma–ray spectrometryNaI(Tl)LaBr3(Ce)CeBr3
spellingShingle Wanook Ji
Eunjoong Lee
Young-Yong Ji
Performances of halide scintillators for the dosimetry based on gamma-ray spectrometry for environmental monitoring systems
Nuclear Engineering and Technology
Halide scintillators
Dosimetry
Gamma–ray spectrometry
NaI(Tl)
LaBr3(Ce)
CeBr3
title Performances of halide scintillators for the dosimetry based on gamma-ray spectrometry for environmental monitoring systems
title_full Performances of halide scintillators for the dosimetry based on gamma-ray spectrometry for environmental monitoring systems
title_fullStr Performances of halide scintillators for the dosimetry based on gamma-ray spectrometry for environmental monitoring systems
title_full_unstemmed Performances of halide scintillators for the dosimetry based on gamma-ray spectrometry for environmental monitoring systems
title_short Performances of halide scintillators for the dosimetry based on gamma-ray spectrometry for environmental monitoring systems
title_sort performances of halide scintillators for the dosimetry based on gamma ray spectrometry for environmental monitoring systems
topic Halide scintillators
Dosimetry
Gamma–ray spectrometry
NaI(Tl)
LaBr3(Ce)
CeBr3
url http://www.sciencedirect.com/science/article/pii/S1738573324004212
work_keys_str_mv AT wanookji performancesofhalidescintillatorsforthedosimetrybasedongammarayspectrometryforenvironmentalmonitoringsystems
AT eunjoonglee performancesofhalidescintillatorsforthedosimetrybasedongammarayspectrometryforenvironmentalmonitoringsystems
AT youngyongji performancesofhalidescintillatorsforthedosimetrybasedongammarayspectrometryforenvironmentalmonitoringsystems