Sources of PM2.5 exposure and health benefits of clean air actions in Shanghai

Estimating PM2.5 exposure and its health impacts in cities involves large uncertainty due to the limitations of model resolutions. Consequently, attributing the sources of PM2.5-related health impacts at the city level remains challenging. We characterize the health impacts associated with chronic P...

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Main Authors: Yixuan Gu, Daven K. Henze, Hong Liao
Format: Article
Language:English
Published: Elsevier 2025-01-01
Series:Environment International
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Online Access:http://www.sciencedirect.com/science/article/pii/S0160412025000108
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author Yixuan Gu
Daven K. Henze
Hong Liao
author_facet Yixuan Gu
Daven K. Henze
Hong Liao
author_sort Yixuan Gu
collection DOAJ
description Estimating PM2.5 exposure and its health impacts in cities involves large uncertainty due to the limitations of model resolutions. Consequently, attributing the sources of PM2.5-related health impacts at the city level remains challenging. We characterize the health impacts associated with chronic PM2.5 exposure and anthropogenic emissions in Shanghai using a chemical transport model (GEOS-Chem) and its adjoint. By incorporating high-resolution satellited-derived PM2.5 estimates into the calculation, we investigate the response of PM2.5 exposure and its related health impacts in Shanghai to changes in anthropogenic emissions from each individual region, species, sector, and month. We estimate that a 10% decrease in anthropogenic emissions throughout China avoids over 752 (506–1,044) PM2.5-related premature deaths in Shanghai, with changes in local emissions potentially saving 241 (161–334) lives. Ammonia (NH3) emissions are identified as the marginal dominant contributor to the health impacts due to the NH3-limited PM2.5 formation within the city, thus controlling NH3 emissions at both the local and regional scales are effective at reducing the population’s exposure to PM2.5. A negative response of the PM2.5 exposure to local nitrogen oxides (NOx) emission changes is detected in winter. Even so, controlling NOx emissions is still justified since the negative impacts decrease as anthropogenic emissions decline and NOx emission reductions benefit the public health on average. The anthropogenic emission changes due to Clean Air Actions helped avoid 3,132 (2,108–4,346) PM2.5-related premature deaths in 2019 relative to 2013, most of which are associated with emission reductions in the agricultural and industrial sectors.
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spelling doaj-art-f3abfa32c47642f4bef5898f70b216032025-01-24T04:44:16ZengElsevierEnvironment International0160-41202025-01-01195109259Sources of PM2.5 exposure and health benefits of clean air actions in ShanghaiYixuan Gu0Daven K. Henze1Hong Liao2Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Joint International Research Laboratory of Climate and Environment Change, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing 210044, China; Department of Mechanical Engineering, University of Colorado, Boulder, CO 80309, USA; Shanghai Typhoon Institute, China Meteorological Administration, Shanghai 200030, China; Corresponding author at: Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, School of Environmental Science and Engineering, Nanjing University of Information Science & Technology, Nanjing 210044, China.Department of Mechanical Engineering, University of Colorado, Boulder, CO 80309, USAJiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Joint International Research Laboratory of Climate and Environment Change, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing 210044, ChinaEstimating PM2.5 exposure and its health impacts in cities involves large uncertainty due to the limitations of model resolutions. Consequently, attributing the sources of PM2.5-related health impacts at the city level remains challenging. We characterize the health impacts associated with chronic PM2.5 exposure and anthropogenic emissions in Shanghai using a chemical transport model (GEOS-Chem) and its adjoint. By incorporating high-resolution satellited-derived PM2.5 estimates into the calculation, we investigate the response of PM2.5 exposure and its related health impacts in Shanghai to changes in anthropogenic emissions from each individual region, species, sector, and month. We estimate that a 10% decrease in anthropogenic emissions throughout China avoids over 752 (506–1,044) PM2.5-related premature deaths in Shanghai, with changes in local emissions potentially saving 241 (161–334) lives. Ammonia (NH3) emissions are identified as the marginal dominant contributor to the health impacts due to the NH3-limited PM2.5 formation within the city, thus controlling NH3 emissions at both the local and regional scales are effective at reducing the population’s exposure to PM2.5. A negative response of the PM2.5 exposure to local nitrogen oxides (NOx) emission changes is detected in winter. Even so, controlling NOx emissions is still justified since the negative impacts decrease as anthropogenic emissions decline and NOx emission reductions benefit the public health on average. The anthropogenic emission changes due to Clean Air Actions helped avoid 3,132 (2,108–4,346) PM2.5-related premature deaths in 2019 relative to 2013, most of which are associated with emission reductions in the agricultural and industrial sectors.http://www.sciencedirect.com/science/article/pii/S0160412025000108Urban PM2.5 pollutionHealth impactsSource apportionmentAdjoint modelingEmission controlUrban health
spellingShingle Yixuan Gu
Daven K. Henze
Hong Liao
Sources of PM2.5 exposure and health benefits of clean air actions in Shanghai
Environment International
Urban PM2.5 pollution
Health impacts
Source apportionment
Adjoint modeling
Emission control
Urban health
title Sources of PM2.5 exposure and health benefits of clean air actions in Shanghai
title_full Sources of PM2.5 exposure and health benefits of clean air actions in Shanghai
title_fullStr Sources of PM2.5 exposure and health benefits of clean air actions in Shanghai
title_full_unstemmed Sources of PM2.5 exposure and health benefits of clean air actions in Shanghai
title_short Sources of PM2.5 exposure and health benefits of clean air actions in Shanghai
title_sort sources of pm2 5 exposure and health benefits of clean air actions in shanghai
topic Urban PM2.5 pollution
Health impacts
Source apportionment
Adjoint modeling
Emission control
Urban health
url http://www.sciencedirect.com/science/article/pii/S0160412025000108
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