Enhancing the Separation Performance of Cellulose Membranes Fabricated from 1-Ethyl-3-methylimidazolium Acetate by Introducing Acetone as a Co-Solvent

Cellulose, a sustainable raw material, holds great promise as an ideal candidate for membrane materials. In this work, we focused on establishing a low-cost route for producing cellulose microfiltration membranes by adopting a co-solvent system comprising the ionic liquid 1-ethyl-3-methylimidazolium...

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Main Authors: Luying Chen, Dooli Kim, Wiebe M. de Vos
Format: Article
Language:English
Published: MDPI AG 2024-09-01
Series:Membranes
Subjects:
Online Access:https://www.mdpi.com/2077-0375/14/9/202
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author Luying Chen
Dooli Kim
Wiebe M. de Vos
author_facet Luying Chen
Dooli Kim
Wiebe M. de Vos
author_sort Luying Chen
collection DOAJ
description Cellulose, a sustainable raw material, holds great promise as an ideal candidate for membrane materials. In this work, we focused on establishing a low-cost route for producing cellulose microfiltration membranes by adopting a co-solvent system comprising the ionic liquid 1-ethyl-3-methylimidazolium acetate ([EMIM]OAc) and acetone. The introduction of acetone as a co-solvent into the casting solution allowed control over the viscosity, thereby significantly enhancing the morphologies and filtration performances of the resulting cellulose membranes. Indeed, applying this co-solvent allowed the water permeability to be significantly increased, while maintaining high rejections. Furthermore, the prepared cellulose membrane demonstrated excellent fouling resistance behavior and flux recovery behavior during a challenging oil-in-water emulsion filtration. These results highlight a promising approach to fabricate high-performance cellulose membranes.
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spelling doaj-art-89fe84c9e4e647eaa8ecb2bb3f7ca00a2025-08-20T01:55:41ZengMDPI AGMembranes2077-03752024-09-0114920210.3390/membranes14090202Enhancing the Separation Performance of Cellulose Membranes Fabricated from 1-Ethyl-3-methylimidazolium Acetate by Introducing Acetone as a Co-SolventLuying Chen0Dooli Kim1Wiebe M. de Vos2Membrane Science and Technology, MESA+ Institute for Nanotechnology, University of Twente, P.O. Box 217, 7500 AE Enschede, The NetherlandsSustainable Process Technology, Faculty of Science and Technology, University of Twente, P.O. Box 217, 7500 AE Enschede, The NetherlandsMembrane Science and Technology, MESA+ Institute for Nanotechnology, University of Twente, P.O. Box 217, 7500 AE Enschede, The NetherlandsCellulose, a sustainable raw material, holds great promise as an ideal candidate for membrane materials. In this work, we focused on establishing a low-cost route for producing cellulose microfiltration membranes by adopting a co-solvent system comprising the ionic liquid 1-ethyl-3-methylimidazolium acetate ([EMIM]OAc) and acetone. The introduction of acetone as a co-solvent into the casting solution allowed control over the viscosity, thereby significantly enhancing the morphologies and filtration performances of the resulting cellulose membranes. Indeed, applying this co-solvent allowed the water permeability to be significantly increased, while maintaining high rejections. Furthermore, the prepared cellulose membrane demonstrated excellent fouling resistance behavior and flux recovery behavior during a challenging oil-in-water emulsion filtration. These results highlight a promising approach to fabricate high-performance cellulose membranes.https://www.mdpi.com/2077-0375/14/9/202cellulosemembranesco-solvent introductionwater filtrationfouling behavior
spellingShingle Luying Chen
Dooli Kim
Wiebe M. de Vos
Enhancing the Separation Performance of Cellulose Membranes Fabricated from 1-Ethyl-3-methylimidazolium Acetate by Introducing Acetone as a Co-Solvent
Membranes
cellulose
membranes
co-solvent introduction
water filtration
fouling behavior
title Enhancing the Separation Performance of Cellulose Membranes Fabricated from 1-Ethyl-3-methylimidazolium Acetate by Introducing Acetone as a Co-Solvent
title_full Enhancing the Separation Performance of Cellulose Membranes Fabricated from 1-Ethyl-3-methylimidazolium Acetate by Introducing Acetone as a Co-Solvent
title_fullStr Enhancing the Separation Performance of Cellulose Membranes Fabricated from 1-Ethyl-3-methylimidazolium Acetate by Introducing Acetone as a Co-Solvent
title_full_unstemmed Enhancing the Separation Performance of Cellulose Membranes Fabricated from 1-Ethyl-3-methylimidazolium Acetate by Introducing Acetone as a Co-Solvent
title_short Enhancing the Separation Performance of Cellulose Membranes Fabricated from 1-Ethyl-3-methylimidazolium Acetate by Introducing Acetone as a Co-Solvent
title_sort enhancing the separation performance of cellulose membranes fabricated from 1 ethyl 3 methylimidazolium acetate by introducing acetone as a co solvent
topic cellulose
membranes
co-solvent introduction
water filtration
fouling behavior
url https://www.mdpi.com/2077-0375/14/9/202
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