A European aerosol phenomenology – 9: Light absorption properties of carbonaceous aerosol particles across surface Europe
Carbonaceous aerosols (CA), composed of black carbon (BC) and organic matter (OM), significantly impact the climate. Light absorption properties of CA, particularly of BC and brown carbon (BrC), are crucial due to their contribution to global and regional warming. We present the absorption propertie...
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2025-01-01
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| author | Jordi Rovira Marjan Savadkoohi Gang I. Chen Griša Močnik Wenche Aas Lucas Alados-Arboledas Begoña Artiñano Minna Aurela John Backman Sujai Banerji David Beddows Benjamin Brem Benjamin Chazeau Martine Collaud Coen Cristina Colombi Sebastien Conil Francesca Costabile Esther Coz Joel F. de Brito Kostas Eleftheriadis Olivier Favez Harald Flentje Evelyn Freney Asta Gregorič Martin Gysel-Beer Roy Harrison Christoph Hueglin Antti Hyvärinen Matic Ivančič Athina-Cerise Kalogridis Hannes Keernik Granakis Konstantinos Paolo Laj Eleni Liakakou Chunshui Lin Stefano Listrani Krista Luoma Marek Maasikmets Hanna E. Manninen Nicolas Marchand Sebastiao Martins dos Santos Saliou Mbengue Nikos Mihalopoulos Doina Nicolae Jarkko V. Niemi Michael Norman Jurgita Ovadnevaite Jean-Eudes Petit Stephen Platt André S.H. Prévôt Manuel Pujadas Jean-Philippe Putaud Véronique Riffault Martin Rigler Matteo Rinaldi Jaroslav Schwarz Sanna Silvergren Erik Teinemaa Kimmo Teinilä Hilkka Timonen Gloria Titos Anna Tobler Jeni Vasilescu Stergios Vratolis Karl Espen Yttri Eduardo Yubero Naděžda Zíková Andrés Alastuey Tuukka Petäjä Xavier Querol Jesús Yus-Díez Marco Pandolfi |
| author_facet | Jordi Rovira Marjan Savadkoohi Gang I. Chen Griša Močnik Wenche Aas Lucas Alados-Arboledas Begoña Artiñano Minna Aurela John Backman Sujai Banerji David Beddows Benjamin Brem Benjamin Chazeau Martine Collaud Coen Cristina Colombi Sebastien Conil Francesca Costabile Esther Coz Joel F. de Brito Kostas Eleftheriadis Olivier Favez Harald Flentje Evelyn Freney Asta Gregorič Martin Gysel-Beer Roy Harrison Christoph Hueglin Antti Hyvärinen Matic Ivančič Athina-Cerise Kalogridis Hannes Keernik Granakis Konstantinos Paolo Laj Eleni Liakakou Chunshui Lin Stefano Listrani Krista Luoma Marek Maasikmets Hanna E. Manninen Nicolas Marchand Sebastiao Martins dos Santos Saliou Mbengue Nikos Mihalopoulos Doina Nicolae Jarkko V. Niemi Michael Norman Jurgita Ovadnevaite Jean-Eudes Petit Stephen Platt André S.H. Prévôt Manuel Pujadas Jean-Philippe Putaud Véronique Riffault Martin Rigler Matteo Rinaldi Jaroslav Schwarz Sanna Silvergren Erik Teinemaa Kimmo Teinilä Hilkka Timonen Gloria Titos Anna Tobler Jeni Vasilescu Stergios Vratolis Karl Espen Yttri Eduardo Yubero Naděžda Zíková Andrés Alastuey Tuukka Petäjä Xavier Querol Jesús Yus-Díez Marco Pandolfi |
| author_sort | Jordi Rovira |
| collection | DOAJ |
| description | Carbonaceous aerosols (CA), composed of black carbon (BC) and organic matter (OM), significantly impact the climate. Light absorption properties of CA, particularly of BC and brown carbon (BrC), are crucial due to their contribution to global and regional warming. We present the absorption properties of BC (bAbs,BC) and BrC (bAbs,BrC) inferred using Aethalometer data from 44 European sites covering different environments (traffic (TR), urban (UB), suburban (SUB), regional background (RB) and mountain (M)). Absorption coefficients showed a clear relationship with station setting decreasing as follows: TR > UB > SUB > RB > M, with exceptions. The contribution of bAbs,BrC to total absorption (bAbs), i.e. %AbsBrC, was lower at traffic sites (11–20 %), exceeding 30 % at some SUB and RB sites. Low AAE values were observed at TR sites, due to the dominance of internal combustion emissions, and at some remote RB/M sites, likely due to the lack of proximity to BrC sources, insufficient secondary processes generating BrC or the effect of photobleaching during transport. Higher bAbs and AAE were observed in Central/Eastern Europe compared to Western/Northern Europe, due to higher coal and biomass burning emissions in the east. Seasonal analysis showed increased bAbs, bAbs,BC, bAbs,BrC in winter, with stronger %AbsBrC, leading to higher AAE. Diel cycles of bAbs,BC peaked during morning and evening rush hours, whereas bAbs,BrC, %AbsBrC, AAE, and AAEBrC peaked at night when emissions from household activities accumulated. Decade-long trends analyses demonstrated a decrease in bAbs, due to reduction of BC emissions, while bAbs,BrC and AAE increased, suggesting a shift in CA composition, with a relative increase in BrC over BC. This study provides a unique dataset to assess the BrC effects on climate and confirms that BrC can contribute significantly to UV–VIS radiation presenting highly variable absorption properties in Europe. |
| format | Article |
| id | doaj-art-7eff434f68ad46c28e4a659a2235bd0f |
| institution | Kabale University |
| issn | 0160-4120 |
| language | English |
| publishDate | 2025-01-01 |
| publisher | Elsevier |
| record_format | Article |
| series | Environment International |
| spelling | doaj-art-7eff434f68ad46c28e4a659a2235bd0f2025-01-24T04:43:59ZengElsevierEnvironment International0160-41202025-01-01195109185A European aerosol phenomenology – 9: Light absorption properties of carbonaceous aerosol particles across surface EuropeJordi Rovira0Marjan Savadkoohi1Gang I. Chen2Griša Močnik3Wenche Aas4Lucas Alados-Arboledas5Begoña Artiñano6Minna Aurela7John Backman8Sujai Banerji9David Beddows10Benjamin Brem11Benjamin Chazeau12Martine Collaud Coen13Cristina Colombi14Sebastien Conil15Francesca Costabile16Esther Coz17Joel F. de Brito18Kostas Eleftheriadis19Olivier Favez20Harald Flentje21Evelyn Freney22Asta Gregorič23Martin Gysel-Beer24Roy Harrison25Christoph Hueglin26Antti Hyvärinen27Matic Ivančič28Athina-Cerise Kalogridis29Hannes Keernik30Granakis Konstantinos31Paolo Laj32Eleni Liakakou33Chunshui Lin34Stefano Listrani35Krista Luoma36Marek Maasikmets37Hanna E. Manninen38Nicolas Marchand39Sebastiao Martins dos Santos40Saliou Mbengue41Nikos Mihalopoulos42Doina Nicolae43Jarkko V. Niemi44Michael Norman45Jurgita Ovadnevaite46Jean-Eudes Petit47Stephen Platt48André S.H. Prévôt49Manuel Pujadas50Jean-Philippe Putaud51Véronique Riffault52Martin Rigler53Matteo Rinaldi54Jaroslav Schwarz55Sanna Silvergren56Erik Teinemaa57Kimmo Teinilä58Hilkka Timonen59Gloria Titos60Anna Tobler61Jeni Vasilescu62Stergios Vratolis63Karl Espen Yttri64Eduardo Yubero65Naděžda Zíková66Andrés Alastuey67Tuukka Petäjä68Xavier Querol69Jesús Yus-Díez70Marco Pandolfi71Institute of Environmental Assessment and Water Research (IDAEA-CSIC), 08034 Barcelona, Spain; Department of Applied Physics-Meteorology, Universitat de Barcelona, Barcelona, 08028, Spain; Corresponding authors at: Institute of Environmental Assessment and Water Research (IDAEA-CSIC), 08034 Barcelona, Spain (Jordi Rovira).Institute of Environmental Assessment and Water Research (IDAEA-CSIC), 08034 Barcelona, Spain; Department of Mining, Industrial and ICT Engineering (EMIT), Manresa School of Engineering (EPSEM), Universitat Politècnica de Catalunya (UPC), Manresa 08242, SpainEnvironmental Research Group, MRC Centre for Environment and Health, Imperial College London, London W12 0BZ, UKCenter for Atmospheric Research, University of Nova Gorica, Ajdovščina 5270, Slovenia; Haze Instruments d.o.o., Ljubljana 1000, Slovenia; Department of Condensed Matter Physics, Jozef Stefan Institute, Ljubljana, 1000, SloveniaNILU, 2027 Kjeller, NorwayAndalusian Institute for Earth System Research (IISTA-CEAMA), University of Granada, Granada, SpainEnvironment Department, CIEMAT, Madrid, SpainAtmospheric Composition Research, Finnish Meteorological Institute, 00560 Helsinki, Finland; Aerosol Physics Laboratory, Faculty of Engineering and Natural Sciences, Tampere University, Tampere University, P.O. Box 692, FI-33014, FinlandAtmospheric Composition Research, Finnish Meteorological Institute, 00560 Helsinki, FinlandInstitute for Atmospheric and Earth System Research/Physics (INAR), Faculty of Science, University of Helsinki, Helsinki, FinlandDivision of Environmental Health & Risk Management, School of Geography, Earth & Environmental Sciences, University of Birmingham, Edgbaston, Birmingham, UKPSI Center for Energy and Environmental Sciences, Paul Scherrer Institute, 5232 Villigen PSI, SwitzerlandPSI Center for Energy and Environmental Sciences, Paul Scherrer Institute, 5232 Villigen PSI, Switzerland; Aix Marseille Univ., CNRS, LCE, Marseille, FranceFederal Office of Meteorology and Climatology, MeteoSwiss, Payerne, SwitzerlandArpa Lombardia, Settore Monitoraggi Ambientali, Unità Operativa Qualità dell’Aria, Milano, ItalyANDRA DRD/GES Observatoire Pérenne de l’Environnement, 55290 Bure, FranceInstitute of Atmospheric Sciences and Climate (ISAC), National Research Council (CNR), 00133, Rome, ItalyAndalusian Institute for Earth System Research (IISTA-CEAMA), University of Granada, Granada, SpainIMT Nord Europe, Institut Mines-Télécom, Univ. Lille, Centre for Energy and Environment, Lille, FranceENRACT, Institute of Nuclear and Radiological Science & Technology, Energy & Safety, NCSR Demokritos, 15310 Ag. Paraskevi, Athens, GreeceInstitut National de l’Environnement Industriel et des Risques (INERIS), Verneuil-en-Halatte, FranceGerman Meteorological Service (DWD), Observatory Hohenpeissenberg, GermanyLaboratoire de Météorologie Physique, UMR6016, Université Clermont Auvergne-CNRS, Aubière, FranceCenter for Atmospheric Research, University of Nova Gorica, Ajdovščina 5270, Slovenia; Aerosol d.o.o., Kamniška 39A, 1000 Ljubljana, SloveniaPSI Center for Energy and Environmental Sciences, Paul Scherrer Institute, 5232 Villigen PSI, SwitzerlandDivision of Environmental Health & Risk Management, School of Geography, Earth & Environmental Sciences, University of Birmingham, Edgbaston, Birmingham, UK; Department of Environmental Sciences, Faculty of Meteorology, Environment and Arid Land Agriculture, King Abdulaziz University, Jeddah, Saudi ArabiaLaboratory for Air Pollution and Environmental Technology, Swiss Federal Laboratories for Materials Science and Technology (Empa), Duebendorf, SwitzerlandAtmospheric Composition Research, Finnish Meteorological Institute, 00560 Helsinki, FinlandAerosol d.o.o., Kamniška 39A, 1000 Ljubljana, SloveniaENRACT, Institute of Nuclear and Radiological Science & Technology, Energy & Safety, NCSR Demokritos, 15310 Ag. Paraskevi, Athens, GreeceEstonian Environmental Research Centre, Air Quality Management Department, Tallinn, EstoniaENRACT, Institute of Nuclear and Radiological Science & Technology, Energy & Safety, NCSR Demokritos, 15310 Ag. Paraskevi, Athens, GreeceAerosol Physics Laboratory, Faculty of Engineering and Natural Sciences, Tampere University, Tampere University, P.O. Box 692, FI-33014, Finland; Univ. Grenoble, CNRS, IRD, IGE, 38000 Grenoble, FranceInstitute for Environmental Research & Sustainable Development, National Observatory of Athens, Athens, GreeceSchool of Natural Sciences, Physics, Centre for Climate and Air Pollution Studies, Ryan Institute, University of Galway, University Road, Galway H91 CF50, IrelandARPA Lazio, Regional Environmental Protection Agency, Rome, ItalyAtmospheric Composition Research, Finnish Meteorological Institute, 00560 Helsinki, Finland; Institute for Atmospheric and Earth System Research/Physics (INAR), Faculty of Science, University of Helsinki, Helsinki, FinlandEstonian Environmental Research Centre, Air Quality Management Department, Tallinn, EstoniaHelsinki Region Environmental Services Authority (HSY), Helsinki, FinlandAix Marseille Univ., CNRS, LCE, Marseille, FranceEuropean Commission, Joint Research Centre (JRC), Ispra, ItalyGlobal Change Research Institute, Czech Academy of Sciences, 603 00 Brno, Czech RepublicInstitute for Environmental Research & Sustainable Development, National Observatory of Athens, Athens, GreeceNational Institute of Research and Development for Optoelectronics INOE 2000, Magurele, RomaniaHelsinki Region Environmental Services Authority (HSY), Helsinki, FinlandEnvironment and Health Administration, SLB-analysis, Stockholm, SwedenSchool of Natural Sciences, Physics, Centre for Climate and Air Pollution Studies, Ryan Institute, University of Galway, University Road, Galway H91 CF50, IrelandLaboratoire des Sciences du Climat et de l’Environnement, CEA/Orme des Merisiers, Gif-sur-Yvette, FranceNILU, 2027 Kjeller, NorwayPSI Center for Energy and Environmental Sciences, Paul Scherrer Institute, 5232 Villigen PSI, SwitzerlandEnvironment Department, CIEMAT, Madrid, SpainEuropean Commission, Joint Research Centre (JRC), Ispra, ItalyIMT Nord Europe, Institut Mines-Télécom, Univ. Lille, Centre for Energy and Environment, Lille, FranceAerosol d.o.o., Kamniška 39A, 1000 Ljubljana, SloveniaInstitute of Atmospheric Sciences and Climate (ISAC), National Research Council (CNR), 40129 Bologna, ItalyInstitute of Chemical Process Fundamentals of the CAS, Rozvojová 135/1, 16502 Prague, Czech RepublicEnvironment and Health Administration, SLB-analysis, Stockholm, SwedenEstonian Environmental Research Centre, Air Quality Management Department, Tallinn, EstoniaAtmospheric Composition Research, Finnish Meteorological Institute, 00560 Helsinki, FinlandAtmospheric Composition Research, Finnish Meteorological Institute, 00560 Helsinki, FinlandAndalusian Institute for Earth System Research (IISTA-CEAMA), University of Granada, Granada, SpainPSI Center for Energy and Environmental Sciences, Paul Scherrer Institute, 5232 Villigen PSI, Switzerland; Datalystica Ltd., Parkstrasse 1, 5234 Villigen, SwitzerlandNational Institute of Research and Development for Optoelectronics INOE 2000, Magurele, RomaniaENRACT, Institute of Nuclear and Radiological Science & Technology, Energy & Safety, NCSR Demokritos, 15310 Ag. Paraskevi, Athens, GreeceNILU, 2027 Kjeller, NorwayAtmospheric Pollution Laboratory (LCA), Department of Applied Physics, Miguel Hernández University, Elche 03202, SpainInstitute of Chemical Process Fundamentals of the CAS, Rozvojová 135/1, 16502 Prague, Czech RepublicInstitute of Environmental Assessment and Water Research (IDAEA-CSIC), 08034 Barcelona, SpainInstitute for Atmospheric and Earth System Research/Physics (INAR), Faculty of Science, University of Helsinki, Helsinki, FinlandInstitute of Environmental Assessment and Water Research (IDAEA-CSIC), 08034 Barcelona, SpainCenter for Atmospheric Research, University of Nova Gorica, Ajdovščina 5270, SloveniaInstitute of Environmental Assessment and Water Research (IDAEA-CSIC), 08034 Barcelona, Spain; Corresponding authors at: Institute of Environmental Assessment and Water Research (IDAEA-CSIC), 08034 Barcelona, Spain (Jordi Rovira).Carbonaceous aerosols (CA), composed of black carbon (BC) and organic matter (OM), significantly impact the climate. Light absorption properties of CA, particularly of BC and brown carbon (BrC), are crucial due to their contribution to global and regional warming. We present the absorption properties of BC (bAbs,BC) and BrC (bAbs,BrC) inferred using Aethalometer data from 44 European sites covering different environments (traffic (TR), urban (UB), suburban (SUB), regional background (RB) and mountain (M)). Absorption coefficients showed a clear relationship with station setting decreasing as follows: TR > UB > SUB > RB > M, with exceptions. The contribution of bAbs,BrC to total absorption (bAbs), i.e. %AbsBrC, was lower at traffic sites (11–20 %), exceeding 30 % at some SUB and RB sites. Low AAE values were observed at TR sites, due to the dominance of internal combustion emissions, and at some remote RB/M sites, likely due to the lack of proximity to BrC sources, insufficient secondary processes generating BrC or the effect of photobleaching during transport. Higher bAbs and AAE were observed in Central/Eastern Europe compared to Western/Northern Europe, due to higher coal and biomass burning emissions in the east. Seasonal analysis showed increased bAbs, bAbs,BC, bAbs,BrC in winter, with stronger %AbsBrC, leading to higher AAE. Diel cycles of bAbs,BC peaked during morning and evening rush hours, whereas bAbs,BrC, %AbsBrC, AAE, and AAEBrC peaked at night when emissions from household activities accumulated. Decade-long trends analyses demonstrated a decrease in bAbs, due to reduction of BC emissions, while bAbs,BrC and AAE increased, suggesting a shift in CA composition, with a relative increase in BrC over BC. This study provides a unique dataset to assess the BrC effects on climate and confirms that BrC can contribute significantly to UV–VIS radiation presenting highly variable absorption properties in Europe.http://www.sciencedirect.com/science/article/pii/S0160412024007712European overviewOrganic aerosolsLong-term datasetsLight absorptionAir quality |
| spellingShingle | Jordi Rovira Marjan Savadkoohi Gang I. Chen Griša Močnik Wenche Aas Lucas Alados-Arboledas Begoña Artiñano Minna Aurela John Backman Sujai Banerji David Beddows Benjamin Brem Benjamin Chazeau Martine Collaud Coen Cristina Colombi Sebastien Conil Francesca Costabile Esther Coz Joel F. de Brito Kostas Eleftheriadis Olivier Favez Harald Flentje Evelyn Freney Asta Gregorič Martin Gysel-Beer Roy Harrison Christoph Hueglin Antti Hyvärinen Matic Ivančič Athina-Cerise Kalogridis Hannes Keernik Granakis Konstantinos Paolo Laj Eleni Liakakou Chunshui Lin Stefano Listrani Krista Luoma Marek Maasikmets Hanna E. Manninen Nicolas Marchand Sebastiao Martins dos Santos Saliou Mbengue Nikos Mihalopoulos Doina Nicolae Jarkko V. Niemi Michael Norman Jurgita Ovadnevaite Jean-Eudes Petit Stephen Platt André S.H. Prévôt Manuel Pujadas Jean-Philippe Putaud Véronique Riffault Martin Rigler Matteo Rinaldi Jaroslav Schwarz Sanna Silvergren Erik Teinemaa Kimmo Teinilä Hilkka Timonen Gloria Titos Anna Tobler Jeni Vasilescu Stergios Vratolis Karl Espen Yttri Eduardo Yubero Naděžda Zíková Andrés Alastuey Tuukka Petäjä Xavier Querol Jesús Yus-Díez Marco Pandolfi A European aerosol phenomenology – 9: Light absorption properties of carbonaceous aerosol particles across surface Europe Environment International European overview Organic aerosols Long-term datasets Light absorption Air quality |
| title | A European aerosol phenomenology – 9: Light absorption properties of carbonaceous aerosol particles across surface Europe |
| title_full | A European aerosol phenomenology – 9: Light absorption properties of carbonaceous aerosol particles across surface Europe |
| title_fullStr | A European aerosol phenomenology – 9: Light absorption properties of carbonaceous aerosol particles across surface Europe |
| title_full_unstemmed | A European aerosol phenomenology – 9: Light absorption properties of carbonaceous aerosol particles across surface Europe |
| title_short | A European aerosol phenomenology – 9: Light absorption properties of carbonaceous aerosol particles across surface Europe |
| title_sort | european aerosol phenomenology 9 light absorption properties of carbonaceous aerosol particles across surface europe |
| topic | European overview Organic aerosols Long-term datasets Light absorption Air quality |
| url | http://www.sciencedirect.com/science/article/pii/S0160412024007712 |
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