Z 2 flux binding to higher-spin impurities in the Kitaev spin liquid

Abstract Stabilizing Z 2 fluxes in Kitaev spin liquids (KSLs) is crucial for both characterizing candidate materials and identifying Ising anyons. In this study, we investigate the effects of spin-S magnetic impurities embedded in the spin-1/2 KSL. Utilizing exact diagonalization and density matrix...

Full description

Saved in:
Bibliographic Details
Main Authors: Masahiro O. Takahashi, Wen-Han Kao, Satoshi Fujimoto, Natalia B. Perkins
Format: Article
Language:English
Published: Nature Portfolio 2025-01-01
Series:npj Quantum Materials
Online Access:https://doi.org/10.1038/s41535-025-00729-8
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1832572008390459392
author Masahiro O. Takahashi
Wen-Han Kao
Satoshi Fujimoto
Natalia B. Perkins
author_facet Masahiro O. Takahashi
Wen-Han Kao
Satoshi Fujimoto
Natalia B. Perkins
author_sort Masahiro O. Takahashi
collection DOAJ
description Abstract Stabilizing Z 2 fluxes in Kitaev spin liquids (KSLs) is crucial for both characterizing candidate materials and identifying Ising anyons. In this study, we investigate the effects of spin-S magnetic impurities embedded in the spin-1/2 KSL. Utilizing exact diagonalization and density matrix renormalization group methods, we examine the impurity magnetization and ground-state flux sector with varying impurity coupling and spin size. Our findings reveal that impurity magnetization exhibits an integer/half-integer spin dependence, which aligns with analytical predictions, and a flux-sector transition from bound-flux to zero-flux occurs at low coupling strengths, independent of the impurity spin. Notably, for spin-3/2 impurities, we observe a reentrant bound-flux sector, which remains stable under magnetic fields. By considering fermionic representations of our spin Hamiltonian, we provide phenomenological explanations for the transitions. Our results suggest a novel way of binding a flux in KSLs, beyond the proposals of vacancies or Kondo impurities.
format Article
id doaj-art-71b8d680967b4d71aa74c8f6e607bf04
institution Kabale University
issn 2397-4648
language English
publishDate 2025-01-01
publisher Nature Portfolio
record_format Article
series npj Quantum Materials
spelling doaj-art-71b8d680967b4d71aa74c8f6e607bf042025-02-02T12:07:16ZengNature Portfolionpj Quantum Materials2397-46482025-01-011011910.1038/s41535-025-00729-8Z 2 flux binding to higher-spin impurities in the Kitaev spin liquidMasahiro O. Takahashi0Wen-Han Kao1Satoshi Fujimoto2Natalia B. Perkins3Department of Materials Engineering Science, Osaka UniversitySchool of Physics and Astronomy, University of MinnesotaDepartment of Materials Engineering Science, Osaka UniversitySchool of Physics and Astronomy, University of MinnesotaAbstract Stabilizing Z 2 fluxes in Kitaev spin liquids (KSLs) is crucial for both characterizing candidate materials and identifying Ising anyons. In this study, we investigate the effects of spin-S magnetic impurities embedded in the spin-1/2 KSL. Utilizing exact diagonalization and density matrix renormalization group methods, we examine the impurity magnetization and ground-state flux sector with varying impurity coupling and spin size. Our findings reveal that impurity magnetization exhibits an integer/half-integer spin dependence, which aligns with analytical predictions, and a flux-sector transition from bound-flux to zero-flux occurs at low coupling strengths, independent of the impurity spin. Notably, for spin-3/2 impurities, we observe a reentrant bound-flux sector, which remains stable under magnetic fields. By considering fermionic representations of our spin Hamiltonian, we provide phenomenological explanations for the transitions. Our results suggest a novel way of binding a flux in KSLs, beyond the proposals of vacancies or Kondo impurities.https://doi.org/10.1038/s41535-025-00729-8
spellingShingle Masahiro O. Takahashi
Wen-Han Kao
Satoshi Fujimoto
Natalia B. Perkins
Z 2 flux binding to higher-spin impurities in the Kitaev spin liquid
npj Quantum Materials
title Z 2 flux binding to higher-spin impurities in the Kitaev spin liquid
title_full Z 2 flux binding to higher-spin impurities in the Kitaev spin liquid
title_fullStr Z 2 flux binding to higher-spin impurities in the Kitaev spin liquid
title_full_unstemmed Z 2 flux binding to higher-spin impurities in the Kitaev spin liquid
title_short Z 2 flux binding to higher-spin impurities in the Kitaev spin liquid
title_sort z 2 flux binding to higher spin impurities in the kitaev spin liquid
url https://doi.org/10.1038/s41535-025-00729-8
work_keys_str_mv AT masahirootakahashi z2fluxbindingtohigherspinimpuritiesinthekitaevspinliquid
AT wenhankao z2fluxbindingtohigherspinimpuritiesinthekitaevspinliquid
AT satoshifujimoto z2fluxbindingtohigherspinimpuritiesinthekitaevspinliquid
AT nataliabperkins z2fluxbindingtohigherspinimpuritiesinthekitaevspinliquid