Zn(TFSI)2-Mediated Ring-Opening Polymerization for Electrolyte Engineering Toward Stable Aqueous Zinc Metal Batteries

Highlights A novel electrolyte enabled by Zn(TFSI)2-mediated ring-opening polymerization strategy for highly reversible aqueous zinc metal batteries was proposed. The novel electrolyte has good antioxidant stability and non-inflammability. The novel electrolyte widens the electrochemical window, imp...

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Bibliographic Details
Main Authors: Zhenjie Liu, Murong Xi, Rui Sheng, Yudai Huang, Juan Ding, Zhouliang Tan, Jiapei Li, Wenjun Zhang, Yonggang Wang
Format: Article
Language:English
Published: SpringerOpen 2025-01-01
Series:Nano-Micro Letters
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Online Access:https://doi.org/10.1007/s40820-025-01649-9
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Summary:Highlights A novel electrolyte enabled by Zn(TFSI)2-mediated ring-opening polymerization strategy for highly reversible aqueous zinc metal batteries was proposed. The novel electrolyte has good antioxidant stability and non-inflammability. The novel electrolyte widens the electrochemical window, improves the low-temperature performance, and inhibits Zn dendrite. The Zn metal anode shows an 8200 h lifespan at 1 mAh cm−2 and a 2500 h lifespan at 60% depth of discharge.
ISSN:2311-6706
2150-5551