Preparation of Manganese Dioxide Nanoparticles on Laterite for Methylene Blue Degradation

The laterite-coating manganese dioxide nanoparticle material (M2) prepared by the immersion method was used for the efficient removal of methylene blue (MB) from aqueous solution. The adsorption and heterogeneous Fenton catalytic oxidation experiments of M2 were investigated by changing the effectiv...

Full description

Saved in:
Bibliographic Details
Main Authors: Thu-Huong Le, Thu Hong Anh Ngo, Van Thuan Doan, Le Minh Tri Nguyen, Manh Cuong Le
Format: Article
Language:English
Published: Wiley 2019-01-01
Series:Journal of Chemistry
Online Access:http://dx.doi.org/10.1155/2019/1602752
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850163703796727808
author Thu-Huong Le
Thu Hong Anh Ngo
Van Thuan Doan
Le Minh Tri Nguyen
Manh Cuong Le
author_facet Thu-Huong Le
Thu Hong Anh Ngo
Van Thuan Doan
Le Minh Tri Nguyen
Manh Cuong Le
author_sort Thu-Huong Le
collection DOAJ
description The laterite-coating manganese dioxide nanoparticle material (M2) prepared by the immersion method was used for the efficient removal of methylene blue (MB) from aqueous solution. The adsorption and heterogeneous Fenton catalytic oxidation experiments of M2 were investigated by changing the effective factors such as time, pH, amount of M2, and concentration of MB. The adsorption data of M2 showed good fitting with the Langmuir isotherm, suggesting that the adsorption of MB on the surface of M2 is a heterogeneous and physical adsorption process. Degradation of MB was also carried out to evaluate the heterogeneous Fenton catalytic oxidation characterization of a new catalytic oxidation material (M2). The results show that the M2 material has both adsorption and heterogeneous Fenton catalytic oxidation. However, the heterogeneous Fenton catalytic oxidation of the M2 material is the main performance. Hence, our groups have investigated the ability of the catalytic column treatment with high efficiency of 98–100% and the degradation efficiency after the sample running through the column almost does not change much. This proves that heterogeneous Fenton catalytic activity of the catalytic column is completely unaffected and reused many times after oxidizing MB. Specifically, even if the M2 material is reused for five times, the degradation efficiency still reaches 98.86%.
format Article
id doaj-art-f47d8a4ee4b248bb9a23b25e4d8a1294
institution OA Journals
issn 2090-9063
2090-9071
language English
publishDate 2019-01-01
publisher Wiley
record_format Article
series Journal of Chemistry
spelling doaj-art-f47d8a4ee4b248bb9a23b25e4d8a12942025-08-20T02:22:10ZengWileyJournal of Chemistry2090-90632090-90712019-01-01201910.1155/2019/16027521602752Preparation of Manganese Dioxide Nanoparticles on Laterite for Methylene Blue DegradationThu-Huong Le0Thu Hong Anh Ngo1Van Thuan Doan2Le Minh Tri Nguyen3Manh Cuong Le4Departerment of Chemistry and Environment, Thuyloi University, Hanoi 100000, VietnamFaculty of Chemistry, University of Science, Vietnam National University, 334 Nguyen Trai, Thanh Xuan, Hanoi, VietnamNTT Hi-Tech Institute, Nguyen Tat Thanh University, Ho Chi Minh City 700000, VietnamLaboratory of Advanced Materials Chemistry, Advanced Institute of Materials Science, Ton Duc Thang University, Ho Chi Minh City, VietnamFaculty of Building Material, National University of Civil Engineering, Hanoi 100000, VietnamThe laterite-coating manganese dioxide nanoparticle material (M2) prepared by the immersion method was used for the efficient removal of methylene blue (MB) from aqueous solution. The adsorption and heterogeneous Fenton catalytic oxidation experiments of M2 were investigated by changing the effective factors such as time, pH, amount of M2, and concentration of MB. The adsorption data of M2 showed good fitting with the Langmuir isotherm, suggesting that the adsorption of MB on the surface of M2 is a heterogeneous and physical adsorption process. Degradation of MB was also carried out to evaluate the heterogeneous Fenton catalytic oxidation characterization of a new catalytic oxidation material (M2). The results show that the M2 material has both adsorption and heterogeneous Fenton catalytic oxidation. However, the heterogeneous Fenton catalytic oxidation of the M2 material is the main performance. Hence, our groups have investigated the ability of the catalytic column treatment with high efficiency of 98–100% and the degradation efficiency after the sample running through the column almost does not change much. This proves that heterogeneous Fenton catalytic activity of the catalytic column is completely unaffected and reused many times after oxidizing MB. Specifically, even if the M2 material is reused for five times, the degradation efficiency still reaches 98.86%.http://dx.doi.org/10.1155/2019/1602752
spellingShingle Thu-Huong Le
Thu Hong Anh Ngo
Van Thuan Doan
Le Minh Tri Nguyen
Manh Cuong Le
Preparation of Manganese Dioxide Nanoparticles on Laterite for Methylene Blue Degradation
Journal of Chemistry
title Preparation of Manganese Dioxide Nanoparticles on Laterite for Methylene Blue Degradation
title_full Preparation of Manganese Dioxide Nanoparticles on Laterite for Methylene Blue Degradation
title_fullStr Preparation of Manganese Dioxide Nanoparticles on Laterite for Methylene Blue Degradation
title_full_unstemmed Preparation of Manganese Dioxide Nanoparticles on Laterite for Methylene Blue Degradation
title_short Preparation of Manganese Dioxide Nanoparticles on Laterite for Methylene Blue Degradation
title_sort preparation of manganese dioxide nanoparticles on laterite for methylene blue degradation
url http://dx.doi.org/10.1155/2019/1602752
work_keys_str_mv AT thuhuongle preparationofmanganesedioxidenanoparticlesonlateriteformethylenebluedegradation
AT thuhonganhngo preparationofmanganesedioxidenanoparticlesonlateriteformethylenebluedegradation
AT vanthuandoan preparationofmanganesedioxidenanoparticlesonlateriteformethylenebluedegradation
AT leminhtringuyen preparationofmanganesedioxidenanoparticlesonlateriteformethylenebluedegradation
AT manhcuongle preparationofmanganesedioxidenanoparticlesonlateriteformethylenebluedegradation