Efficient Sunlight-Induced Methylene Blue Removal over One-Dimensional Mesoporous Monoclinic BiVO4 Nanorods

Sunlight-driven mesoporous BiVO4 nanorods with monoclinic structure have been successfully synthesized via a simple hydrothermal method. The as-prepared one-dimensional BiVO4 nanorods exhibited high specific surface area due to their unique mesoporous structure. The mesoporous BiVO4 nanorods possess...

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Main Authors: Linrui Hou, Long Yang, Jiaoyang Li, Jie Tan, Changzhou Yuan
Format: Article
Language:English
Published: Wiley 2012-01-01
Series:Journal of Analytical Methods in Chemistry
Online Access:http://dx.doi.org/10.1155/2012/345247
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author Linrui Hou
Long Yang
Jiaoyang Li
Jie Tan
Changzhou Yuan
author_facet Linrui Hou
Long Yang
Jiaoyang Li
Jie Tan
Changzhou Yuan
author_sort Linrui Hou
collection DOAJ
description Sunlight-driven mesoporous BiVO4 nanorods with monoclinic structure have been successfully synthesized via a simple hydrothermal method. The as-prepared one-dimensional BiVO4 nanorods exhibited high specific surface area due to their unique mesoporous structure. The mesoporous BiVO4 nanorods possessed strong photoabsorption properties in the visible light region as well as the ultravisible region, and the band gap was estimated to be ca. 2.18 eV. The photocatalytic activities were evaluated by decolorization of methylene blue under sunlight irradiation. Photocatalytic tests demonstrated that the decolorization rate of as-prepared mesoporous BiVO4 nanorods was even up to 98.8% in 180 min, much better than that prepared by solid-state reaction (23.1%) and the commercial TiO2 (Degussa P25) (14.2%) under the same conditions, due to their higher specific surface area and appropriate band gap. Moreover, the unique BiVO4 nanorods exhibit high stability after five photocatalytic degradation recycles.
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issn 2090-8865
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language English
publishDate 2012-01-01
publisher Wiley
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spelling doaj-art-f41eb5bbfcad4cc6adc3b258bc01c2102025-08-20T02:21:43ZengWileyJournal of Analytical Methods in Chemistry2090-88652090-88732012-01-01201210.1155/2012/345247345247Efficient Sunlight-Induced Methylene Blue Removal over One-Dimensional Mesoporous Monoclinic BiVO4 NanorodsLinrui Hou0Long Yang1Jiaoyang Li2Jie Tan3Changzhou Yuan4Anhui Key Laboratory of Metal Materials and Processing, School of Materials Science and Engineering, Anhui University of Technology, Ma'anshan 243002, ChinaAnhui Key Laboratory of Metal Materials and Processing, School of Materials Science and Engineering, Anhui University of Technology, Ma'anshan 243002, ChinaAnhui Key Laboratory of Metal Materials and Processing, School of Materials Science and Engineering, Anhui University of Technology, Ma'anshan 243002, ChinaAnhui Key Laboratory of Metal Materials and Processing, School of Materials Science and Engineering, Anhui University of Technology, Ma'anshan 243002, ChinaAnhui Key Laboratory of Metal Materials and Processing, School of Materials Science and Engineering, Anhui University of Technology, Ma'anshan 243002, ChinaSunlight-driven mesoporous BiVO4 nanorods with monoclinic structure have been successfully synthesized via a simple hydrothermal method. The as-prepared one-dimensional BiVO4 nanorods exhibited high specific surface area due to their unique mesoporous structure. The mesoporous BiVO4 nanorods possessed strong photoabsorption properties in the visible light region as well as the ultravisible region, and the band gap was estimated to be ca. 2.18 eV. The photocatalytic activities were evaluated by decolorization of methylene blue under sunlight irradiation. Photocatalytic tests demonstrated that the decolorization rate of as-prepared mesoporous BiVO4 nanorods was even up to 98.8% in 180 min, much better than that prepared by solid-state reaction (23.1%) and the commercial TiO2 (Degussa P25) (14.2%) under the same conditions, due to their higher specific surface area and appropriate band gap. Moreover, the unique BiVO4 nanorods exhibit high stability after five photocatalytic degradation recycles.http://dx.doi.org/10.1155/2012/345247
spellingShingle Linrui Hou
Long Yang
Jiaoyang Li
Jie Tan
Changzhou Yuan
Efficient Sunlight-Induced Methylene Blue Removal over One-Dimensional Mesoporous Monoclinic BiVO4 Nanorods
Journal of Analytical Methods in Chemistry
title Efficient Sunlight-Induced Methylene Blue Removal over One-Dimensional Mesoporous Monoclinic BiVO4 Nanorods
title_full Efficient Sunlight-Induced Methylene Blue Removal over One-Dimensional Mesoporous Monoclinic BiVO4 Nanorods
title_fullStr Efficient Sunlight-Induced Methylene Blue Removal over One-Dimensional Mesoporous Monoclinic BiVO4 Nanorods
title_full_unstemmed Efficient Sunlight-Induced Methylene Blue Removal over One-Dimensional Mesoporous Monoclinic BiVO4 Nanorods
title_short Efficient Sunlight-Induced Methylene Blue Removal over One-Dimensional Mesoporous Monoclinic BiVO4 Nanorods
title_sort efficient sunlight induced methylene blue removal over one dimensional mesoporous monoclinic bivo4 nanorods
url http://dx.doi.org/10.1155/2012/345247
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AT longyang efficientsunlightinducedmethyleneblueremovaloveronedimensionalmesoporousmonoclinicbivo4nanorods
AT jiaoyangli efficientsunlightinducedmethyleneblueremovaloveronedimensionalmesoporousmonoclinicbivo4nanorods
AT jietan efficientsunlightinducedmethyleneblueremovaloveronedimensionalmesoporousmonoclinicbivo4nanorods
AT changzhouyuan efficientsunlightinducedmethyleneblueremovaloveronedimensionalmesoporousmonoclinicbivo4nanorods