Crystalline plasticity in isotactic polypropylene below and above the glass transition temperature

In-situ X-ray diffraction was applied to isotactic polypropylene with a high volume fraction of α-phase (α-iPP) while it has been compressed at temperatures below and above its glass transition temperature Tg. The diffraction patterns were evaluated by the Multi-reflection X-ray Profile Analysis (MX...

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Bibliographic Details
Main Authors: G. Polt, F. Spieckermann, H. Wilhelm, Ch. Fischer, E. Schafler, S. Bernstorff, M. Zehetbauer
Format: Article
Language:English
Published: Budapest University of Technology and Economics 2015-10-01
Series:eXPRESS Polymer Letters
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Online Access:http://www.expresspolymlett.com/letolt.php?file=EPL-0006191&mi=cd
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Summary:In-situ X-ray diffraction was applied to isotactic polypropylene with a high volume fraction of α-phase (α-iPP) while it has been compressed at temperatures below and above its glass transition temperature Tg. The diffraction patterns were evaluated by the Multi-reflection X-ray Profile Analysis (MXPA) method, revealing microstructural parameters such as the density of dislocations and the size of coherently scattering domains (CSD-size). A significant difference in the development of the dislocation density was found compared to compression at temperatures above Tg, pointing at a different plastic deformation mechanism at these temperatures. Based on the individual evolutions of the dislocation density and CSD-size observed as a function of compressive strain, suggestions for the deformation mechanisms occurring below and above Tg are made.
ISSN:1788-618X