Single‐Particle Measurement: A Valuable Method for Studying Structural Evolution of Battery and Performance Degradation
Abstract Active particle materials with high capacity, safety, and abundance, such as Sn and Si‐based materials, and nickel‐rich layered materials like LiNixCoyMn1−x−yO2 (with x≥0.8) are viewed as promising candidates for the evolution of next‐generation batteries. However, structural degradation du...
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| Main Authors: | , , , , , |
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| Format: | Article |
| Language: | English |
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Wiley-VCH
2025-02-01
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| Series: | ChemElectroChem |
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| Online Access: | https://doi.org/10.1002/celc.202400529 |
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| author | Xin Zhang Na Li Xu Li Le Yang Wei‐Li Song Ya‐Na Wang |
| author_facet | Xin Zhang Na Li Xu Li Le Yang Wei‐Li Song Ya‐Na Wang |
| author_sort | Xin Zhang |
| collection | DOAJ |
| description | Abstract Active particle materials with high capacity, safety, and abundance, such as Sn and Si‐based materials, and nickel‐rich layered materials like LiNixCoyMn1−x−yO2 (with x≥0.8) are viewed as promising candidates for the evolution of next‐generation batteries. However, structural degradation during cycling often limits the application of these active particle materials. Currently, research efforts are focused on developing new characterization techniques to understand the structural degradation mechanisms of active particle materials during the cycle, to improve their performance. This paper reviews advanced single‐particle electrochemical and structural characterization techniques and their main findings. These findings included lattice displacement and rotation, microstructure evolution, and reaction kinetics of single‐particle during cycling. In addition, we also discuss the potential future applications and developments of single‐particle measurement technologies. |
| format | Article |
| id | doaj-art-e8189264a8514914bda1be9493db92d5 |
| institution | Kabale University |
| issn | 2196-0216 |
| language | English |
| publishDate | 2025-02-01 |
| publisher | Wiley-VCH |
| record_format | Article |
| series | ChemElectroChem |
| spelling | doaj-art-e8189264a8514914bda1be9493db92d52025-02-03T10:00:37ZengWiley-VCHChemElectroChem2196-02162025-02-01123n/an/a10.1002/celc.202400529Single‐Particle Measurement: A Valuable Method for Studying Structural Evolution of Battery and Performance DegradationXin Zhang0Na Li1Xu Li2Le Yang3Wei‐Li Song4Ya‐Na Wang5Institute of Advanced Structure Technology Beijing Institute of Technology Beijing 100081 P. R. ChinaState Key Laboratory of Advanced Metallurgy University of Science and Technology Beijing Beijing 100083 P. R. ChinaInstitute of Advanced Structure Technology Beijing Institute of Technology Beijing 100081 P. R. ChinaInstitute of Advanced Structure Technology Beijing Institute of Technology Beijing 100081 P. R. ChinaInstitute of Advanced Structure Technology Beijing Institute of Technology Beijing 100081 P. R. ChinaSchool of Mechanical and Vehicular Engineering Beijing Institute of Technology Beijing 100081 P. R. ChinaAbstract Active particle materials with high capacity, safety, and abundance, such as Sn and Si‐based materials, and nickel‐rich layered materials like LiNixCoyMn1−x−yO2 (with x≥0.8) are viewed as promising candidates for the evolution of next‐generation batteries. However, structural degradation during cycling often limits the application of these active particle materials. Currently, research efforts are focused on developing new characterization techniques to understand the structural degradation mechanisms of active particle materials during the cycle, to improve their performance. This paper reviews advanced single‐particle electrochemical and structural characterization techniques and their main findings. These findings included lattice displacement and rotation, microstructure evolution, and reaction kinetics of single‐particle during cycling. In addition, we also discuss the potential future applications and developments of single‐particle measurement technologies.https://doi.org/10.1002/celc.202400529Lithium-ion batterySingle-particle measurementsStructural evolutionReaction kinetics |
| spellingShingle | Xin Zhang Na Li Xu Li Le Yang Wei‐Li Song Ya‐Na Wang Single‐Particle Measurement: A Valuable Method for Studying Structural Evolution of Battery and Performance Degradation ChemElectroChem Lithium-ion battery Single-particle measurements Structural evolution Reaction kinetics |
| title | Single‐Particle Measurement: A Valuable Method for Studying Structural Evolution of Battery and Performance Degradation |
| title_full | Single‐Particle Measurement: A Valuable Method for Studying Structural Evolution of Battery and Performance Degradation |
| title_fullStr | Single‐Particle Measurement: A Valuable Method for Studying Structural Evolution of Battery and Performance Degradation |
| title_full_unstemmed | Single‐Particle Measurement: A Valuable Method for Studying Structural Evolution of Battery and Performance Degradation |
| title_short | Single‐Particle Measurement: A Valuable Method for Studying Structural Evolution of Battery and Performance Degradation |
| title_sort | single particle measurement a valuable method for studying structural evolution of battery and performance degradation |
| topic | Lithium-ion battery Single-particle measurements Structural evolution Reaction kinetics |
| url | https://doi.org/10.1002/celc.202400529 |
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