EURAD State-of-the-Art Report: ACED assessment of the chemical evolution at the disposal cell scale—part I—processes at interfaces and evolution at disposal cell scale

Within the framework of the European Joint Programme on Radioactive Waste Management, the work package ACED–Assessment of chemical evolution of intermediate level (ILW) and high level (HLW) waste at disposal cell scale–used combined experimental and modelling methods in a multi-scale approach with p...

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Main Authors: Erika Neeft, Guido Deissmann, Diederik Jacques
Format: Article
Language:English
Published: Frontiers Media S.A. 2025-01-01
Series:Frontiers in Nuclear Engineering
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Online Access:https://www.frontiersin.org/articles/10.3389/fnuen.2024.1433247/full
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author Erika Neeft
Guido Deissmann
Diederik Jacques
author_facet Erika Neeft
Guido Deissmann
Diederik Jacques
author_sort Erika Neeft
collection DOAJ
description Within the framework of the European Joint Programme on Radioactive Waste Management, the work package ACED–Assessment of chemical evolution of intermediate level (ILW) and high level (HLW) waste at disposal cell scale–used combined experimental and modelling methods in a multi-scale approach with process integration to improve the long-term modelling and assessment of the chemical evolution at the disposal cell scale. Part I provides the relevance of the assessment of the chemical evolution for safety, performance, and optimization. It further describes the main characteristics of disposal cells for ILW and vitrified HLW waste in European disposal programmes. From that, a number of interfaces between different types of material are identified that are highly relevant for many national disposal programs: glass-steel, steel-concrete, steel-clay, steel-crystalline, concrete-clay, and concrete-crystalline. Based on literature review, the main processes and consequences occurring at these interfaces are described. The key element is the narrative of the evolution at the disposal cell scale based on process understanding. In part II, tools to obtain process understanding–experiments, analogues, modelling–are discussed in detail.
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spelling doaj-art-e58c367ad11d4ecca95225ce2b22ce892025-01-20T04:11:06ZengFrontiers Media S.A.Frontiers in Nuclear Engineering2813-34122025-01-01310.3389/fnuen.2024.14332471433247EURAD State-of-the-Art Report: ACED assessment of the chemical evolution at the disposal cell scale—part I—processes at interfaces and evolution at disposal cell scaleErika Neeft0Guido Deissmann1Diederik Jacques2Central Organisation for Radioactive Waste (COVRA), Nieuwdorp, NetherlandsForschungszentrum Jülich GmbH, Jülich, GermanyBelgian Nuclear Research Centre (SCK CEN), Mol, BelgiumWithin the framework of the European Joint Programme on Radioactive Waste Management, the work package ACED–Assessment of chemical evolution of intermediate level (ILW) and high level (HLW) waste at disposal cell scale–used combined experimental and modelling methods in a multi-scale approach with process integration to improve the long-term modelling and assessment of the chemical evolution at the disposal cell scale. Part I provides the relevance of the assessment of the chemical evolution for safety, performance, and optimization. It further describes the main characteristics of disposal cells for ILW and vitrified HLW waste in European disposal programmes. From that, a number of interfaces between different types of material are identified that are highly relevant for many national disposal programs: glass-steel, steel-concrete, steel-clay, steel-crystalline, concrete-clay, and concrete-crystalline. Based on literature review, the main processes and consequences occurring at these interfaces are described. The key element is the narrative of the evolution at the disposal cell scale based on process understanding. In part II, tools to obtain process understanding–experiments, analogues, modelling–are discussed in detail.https://www.frontiersin.org/articles/10.3389/fnuen.2024.1433247/fullradioactive waste disposalchemical evolutionvitrified wastecementitious materialssteelclay
spellingShingle Erika Neeft
Guido Deissmann
Diederik Jacques
EURAD State-of-the-Art Report: ACED assessment of the chemical evolution at the disposal cell scale—part I—processes at interfaces and evolution at disposal cell scale
Frontiers in Nuclear Engineering
radioactive waste disposal
chemical evolution
vitrified waste
cementitious materials
steel
clay
title EURAD State-of-the-Art Report: ACED assessment of the chemical evolution at the disposal cell scale—part I—processes at interfaces and evolution at disposal cell scale
title_full EURAD State-of-the-Art Report: ACED assessment of the chemical evolution at the disposal cell scale—part I—processes at interfaces and evolution at disposal cell scale
title_fullStr EURAD State-of-the-Art Report: ACED assessment of the chemical evolution at the disposal cell scale—part I—processes at interfaces and evolution at disposal cell scale
title_full_unstemmed EURAD State-of-the-Art Report: ACED assessment of the chemical evolution at the disposal cell scale—part I—processes at interfaces and evolution at disposal cell scale
title_short EURAD State-of-the-Art Report: ACED assessment of the chemical evolution at the disposal cell scale—part I—processes at interfaces and evolution at disposal cell scale
title_sort eurad state of the art report aced assessment of the chemical evolution at the disposal cell scale part i processes at interfaces and evolution at disposal cell scale
topic radioactive waste disposal
chemical evolution
vitrified waste
cementitious materials
steel
clay
url https://www.frontiersin.org/articles/10.3389/fnuen.2024.1433247/full
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