Investigation on Mercury Reemission from Limestone-Gypsum Wet Flue Gas Desulfurization Slurry

Secondary atmospheric pollutions may result from wet flue gas desulfurization (WFGD) systems caused by the reduction of Hg2+ to Hg0 and lead to a damping of the cobenefit mercury removal efficiency by WFGD systems. The experiment on Hg0 reemission from limestone-gypsum WFGD slurry was carried out by...

Full description

Saved in:
Bibliographic Details
Main Authors: Chuanmin Chen, Songtao Liu, Yang Gao, Yongchao Liu
Format: Article
Language:English
Published: Wiley 2014-01-01
Series:The Scientific World Journal
Online Access:http://dx.doi.org/10.1155/2014/581724
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1832551569888903168
author Chuanmin Chen
Songtao Liu
Yang Gao
Yongchao Liu
author_facet Chuanmin Chen
Songtao Liu
Yang Gao
Yongchao Liu
author_sort Chuanmin Chen
collection DOAJ
description Secondary atmospheric pollutions may result from wet flue gas desulfurization (WFGD) systems caused by the reduction of Hg2+ to Hg0 and lead to a damping of the cobenefit mercury removal efficiency by WFGD systems. The experiment on Hg0 reemission from limestone-gypsum WFGD slurry was carried out by changing the operating conditions such as the pH, temperature, Cl− concentrations, and oxygen concentrations. The partitioning behavior of mercury in the solid and liquid byproducts was also discussed. The experimental results indicated that the Hg0 reemission rate from WFGD slurry increased as the operational temperatures and pH values increased. The Hg0 reemission rates decreased as the O2 concentration of flue gas and Cl− concentration of WFGD slurry increased. The concentrations of O2 in flue gas have an evident effect on the mercury retention in the solid byproducts. The temperature and Cl− concentration have a slight effect on the mercury partitioning in the byproducts. No evident relation was found between mercury retention in the solid byproducts and the pH. The present findings could be valuable for industrial application of characterizing and optimizing mercury control in wet FGD systems.
format Article
id doaj-art-dd464252c1214f31945adde44d8739af
institution Kabale University
issn 2356-6140
1537-744X
language English
publishDate 2014-01-01
publisher Wiley
record_format Article
series The Scientific World Journal
spelling doaj-art-dd464252c1214f31945adde44d8739af2025-02-03T06:01:09ZengWileyThe Scientific World Journal2356-61401537-744X2014-01-01201410.1155/2014/581724581724Investigation on Mercury Reemission from Limestone-Gypsum Wet Flue Gas Desulfurization SlurryChuanmin Chen0Songtao Liu1Yang Gao2Yongchao Liu3School of Environmental Science & Engineering, North China Electric Power University, Baoding 071003, ChinaSchool of Environmental Science & Engineering, North China Electric Power University, Baoding 071003, ChinaSchool of Environmental Science & Engineering, North China Electric Power University, Baoding 071003, ChinaSchool of Environmental Science & Engineering, North China Electric Power University, Baoding 071003, ChinaSecondary atmospheric pollutions may result from wet flue gas desulfurization (WFGD) systems caused by the reduction of Hg2+ to Hg0 and lead to a damping of the cobenefit mercury removal efficiency by WFGD systems. The experiment on Hg0 reemission from limestone-gypsum WFGD slurry was carried out by changing the operating conditions such as the pH, temperature, Cl− concentrations, and oxygen concentrations. The partitioning behavior of mercury in the solid and liquid byproducts was also discussed. The experimental results indicated that the Hg0 reemission rate from WFGD slurry increased as the operational temperatures and pH values increased. The Hg0 reemission rates decreased as the O2 concentration of flue gas and Cl− concentration of WFGD slurry increased. The concentrations of O2 in flue gas have an evident effect on the mercury retention in the solid byproducts. The temperature and Cl− concentration have a slight effect on the mercury partitioning in the byproducts. No evident relation was found between mercury retention in the solid byproducts and the pH. The present findings could be valuable for industrial application of characterizing and optimizing mercury control in wet FGD systems.http://dx.doi.org/10.1155/2014/581724
spellingShingle Chuanmin Chen
Songtao Liu
Yang Gao
Yongchao Liu
Investigation on Mercury Reemission from Limestone-Gypsum Wet Flue Gas Desulfurization Slurry
The Scientific World Journal
title Investigation on Mercury Reemission from Limestone-Gypsum Wet Flue Gas Desulfurization Slurry
title_full Investigation on Mercury Reemission from Limestone-Gypsum Wet Flue Gas Desulfurization Slurry
title_fullStr Investigation on Mercury Reemission from Limestone-Gypsum Wet Flue Gas Desulfurization Slurry
title_full_unstemmed Investigation on Mercury Reemission from Limestone-Gypsum Wet Flue Gas Desulfurization Slurry
title_short Investigation on Mercury Reemission from Limestone-Gypsum Wet Flue Gas Desulfurization Slurry
title_sort investigation on mercury reemission from limestone gypsum wet flue gas desulfurization slurry
url http://dx.doi.org/10.1155/2014/581724
work_keys_str_mv AT chuanminchen investigationonmercuryreemissionfromlimestonegypsumwetfluegasdesulfurizationslurry
AT songtaoliu investigationonmercuryreemissionfromlimestonegypsumwetfluegasdesulfurizationslurry
AT yanggao investigationonmercuryreemissionfromlimestonegypsumwetfluegasdesulfurizationslurry
AT yongchaoliu investigationonmercuryreemissionfromlimestonegypsumwetfluegasdesulfurizationslurry