Advancements in active filler-contained polymer solid-state electrolytes for lithium-metal batteries: A concise review
Lithium-metal batteries (LMBs) usually are regarded as the pinnacle of next-generation energy storage due to the high specific capacity and low redox potential of the Li-metal anode. However, their development is hindered by safety hazards related to flammable electrolytes and uncontrolled side reac...
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KeAi Communications Co., Ltd.
2025-12-01
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| Series: | Supramolecular Materials |
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| Online Access: | http://www.sciencedirect.com/science/article/pii/S2667240525000066 |
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| author | Hang Ding Mingli Wang Xinyuan Shan Guang Yang Ming Tian |
| author_facet | Hang Ding Mingli Wang Xinyuan Shan Guang Yang Ming Tian |
| author_sort | Hang Ding |
| collection | DOAJ |
| description | Lithium-metal batteries (LMBs) usually are regarded as the pinnacle of next-generation energy storage due to the high specific capacity and low redox potential of the Li-metal anode. However, their development is hindered by safety hazards related to flammable electrolytes and uncontrolled side reactions within the battery. Both polymer and solid-state inorganic electrolytes, despite their potential, exhibit shortcomings that limit their practical applications. Active filler-containing polymer electrolytes (AFPEs) offer a promising solution by combining the benefits of both types. Enhanced by supramolecular interactions between the polymer matrix and active fillers, AFPEs demonstrate superior electrochemical performance over traditional polymer electrolytes. This review discusses the progress in active fillers and various polymer matrices, examining the factors that enhance performance, particularly ionic conductivity. It also outlines the future research directions of AFPEs, aiming to broaden the application of solid electrolytes in high-performance LMBs. |
| format | Article |
| id | doaj-art-dc2e983eef7341f2b08952c4bc568e03 |
| institution | Kabale University |
| issn | 2667-2405 |
| language | English |
| publishDate | 2025-12-01 |
| publisher | KeAi Communications Co., Ltd. |
| record_format | Article |
| series | Supramolecular Materials |
| spelling | doaj-art-dc2e983eef7341f2b08952c4bc568e032025-01-24T04:45:54ZengKeAi Communications Co., Ltd.Supramolecular Materials2667-24052025-12-014100097Advancements in active filler-contained polymer solid-state electrolytes for lithium-metal batteries: A concise reviewHang Ding0Mingli Wang1Xinyuan Shan2Guang Yang3Ming Tian4State Key Laboratory of Organic-Inorganic Composites, School of Materials Science and Engineering, Beijing University of Chemical Technology, Beijing 100029, PR ChinaState Key Laboratory of Organic-Inorganic Composites, School of Materials Science and Engineering, Beijing University of Chemical Technology, Beijing 100029, PR ChinaState Key Laboratory of Organic-Inorganic Composites, School of Materials Science and Engineering, Beijing University of Chemical Technology, Beijing 100029, PR China; Corresponding authors.Chemical Sciences Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37831, USA; The Bredesen Center for Interdisciplinary Research and Graduate Education, University of Tennessee Knoxville, Knoxville, TN 37996, USA; Corresponding authors.State Key Laboratory of Organic-Inorganic Composites, School of Materials Science and Engineering, Beijing University of Chemical Technology, Beijing 100029, PR ChinaLithium-metal batteries (LMBs) usually are regarded as the pinnacle of next-generation energy storage due to the high specific capacity and low redox potential of the Li-metal anode. However, their development is hindered by safety hazards related to flammable electrolytes and uncontrolled side reactions within the battery. Both polymer and solid-state inorganic electrolytes, despite their potential, exhibit shortcomings that limit their practical applications. Active filler-containing polymer electrolytes (AFPEs) offer a promising solution by combining the benefits of both types. Enhanced by supramolecular interactions between the polymer matrix and active fillers, AFPEs demonstrate superior electrochemical performance over traditional polymer electrolytes. This review discusses the progress in active fillers and various polymer matrices, examining the factors that enhance performance, particularly ionic conductivity. It also outlines the future research directions of AFPEs, aiming to broaden the application of solid electrolytes in high-performance LMBs.http://www.sciencedirect.com/science/article/pii/S2667240525000066Polymer electrolyteComposite electrolyteAll solid-state batteriesSupramolecule |
| spellingShingle | Hang Ding Mingli Wang Xinyuan Shan Guang Yang Ming Tian Advancements in active filler-contained polymer solid-state electrolytes for lithium-metal batteries: A concise review Supramolecular Materials Polymer electrolyte Composite electrolyte All solid-state batteries Supramolecule |
| title | Advancements in active filler-contained polymer solid-state electrolytes for lithium-metal batteries: A concise review |
| title_full | Advancements in active filler-contained polymer solid-state electrolytes for lithium-metal batteries: A concise review |
| title_fullStr | Advancements in active filler-contained polymer solid-state electrolytes for lithium-metal batteries: A concise review |
| title_full_unstemmed | Advancements in active filler-contained polymer solid-state electrolytes for lithium-metal batteries: A concise review |
| title_short | Advancements in active filler-contained polymer solid-state electrolytes for lithium-metal batteries: A concise review |
| title_sort | advancements in active filler contained polymer solid state electrolytes for lithium metal batteries a concise review |
| topic | Polymer electrolyte Composite electrolyte All solid-state batteries Supramolecule |
| url | http://www.sciencedirect.com/science/article/pii/S2667240525000066 |
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