Modeling extensive defects in metals through classical potential-guided sampling and automated configuration reconstruction

Abstract Extended defects such as dislocation networks and general grain boundaries are ubiquitous in metals, and accurate modeling these extensive defects is crucial to elucidate their deformation mechanisms. However, existing machine learning interatomic potentials (MLIPs) often fall short in adeq...

Full description

Saved in:
Bibliographic Details
Main Authors: Fei Shuang, Kai Liu, Yucheng Ji, Wei Gao, Luca Laurenti, Poulumi Dey
Format: Article
Language:English
Published: Nature Portfolio 2025-05-01
Series:npj Computational Materials
Online Access:https://doi.org/10.1038/s41524-025-01599-1
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849314836661403648
author Fei Shuang
Kai Liu
Yucheng Ji
Wei Gao
Luca Laurenti
Poulumi Dey
author_facet Fei Shuang
Kai Liu
Yucheng Ji
Wei Gao
Luca Laurenti
Poulumi Dey
author_sort Fei Shuang
collection DOAJ
description Abstract Extended defects such as dislocation networks and general grain boundaries are ubiquitous in metals, and accurate modeling these extensive defects is crucial to elucidate their deformation mechanisms. However, existing machine learning interatomic potentials (MLIPs) often fall short in adequately describing these defects, as their large characteristic scales exceed the computational limits of first-principles calculations. To address this challenge, we present a computational framework combining a defect genome constructed via empirical interatomic potential-guided sampling, with an automated reconstruction technique that enables accurate first-principles modeling of general defects by converting atomic clusters into periodic configurations. The effectiveness of this approach was validated through simulations of nanoindentation, tensile deformation, and fracture in BCC tungsten. This framework enhances the modeling accuracy of extended defects in crystalline materials and provides a robust foundation for advancing MLIP development by leveraging defect genomes strategically.
format Article
id doaj-art-db72afefa45c44a58b16f85070d4226a
institution Kabale University
issn 2057-3960
language English
publishDate 2025-05-01
publisher Nature Portfolio
record_format Article
series npj Computational Materials
spelling doaj-art-db72afefa45c44a58b16f85070d4226a2025-08-20T03:52:19ZengNature Portfolionpj Computational Materials2057-39602025-05-0111111210.1038/s41524-025-01599-1Modeling extensive defects in metals through classical potential-guided sampling and automated configuration reconstructionFei Shuang0Kai Liu1Yucheng Ji2Wei Gao3Luca Laurenti4Poulumi Dey5Department of Materials Science and Engineering, Faculty of Mechanical Engineering, Delft University of Technology, Mekelweg 2Department of Materials Science and Engineering, Faculty of Mechanical Engineering, Delft University of Technology, Mekelweg 2Department of Materials Science and Engineering, Faculty of Mechanical Engineering, Delft University of Technology, Mekelweg 2J. Mike Walker’66 Department of Mechanical Engineering, Texas A&M University, College StationDelft Centre of System and Control (DCSC), Faculty of Mechanical Engineering, Delft University of Technology, Mekelweg 2Department of Materials Science and Engineering, Faculty of Mechanical Engineering, Delft University of Technology, Mekelweg 2Abstract Extended defects such as dislocation networks and general grain boundaries are ubiquitous in metals, and accurate modeling these extensive defects is crucial to elucidate their deformation mechanisms. However, existing machine learning interatomic potentials (MLIPs) often fall short in adequately describing these defects, as their large characteristic scales exceed the computational limits of first-principles calculations. To address this challenge, we present a computational framework combining a defect genome constructed via empirical interatomic potential-guided sampling, with an automated reconstruction technique that enables accurate first-principles modeling of general defects by converting atomic clusters into periodic configurations. The effectiveness of this approach was validated through simulations of nanoindentation, tensile deformation, and fracture in BCC tungsten. This framework enhances the modeling accuracy of extended defects in crystalline materials and provides a robust foundation for advancing MLIP development by leveraging defect genomes strategically.https://doi.org/10.1038/s41524-025-01599-1
spellingShingle Fei Shuang
Kai Liu
Yucheng Ji
Wei Gao
Luca Laurenti
Poulumi Dey
Modeling extensive defects in metals through classical potential-guided sampling and automated configuration reconstruction
npj Computational Materials
title Modeling extensive defects in metals through classical potential-guided sampling and automated configuration reconstruction
title_full Modeling extensive defects in metals through classical potential-guided sampling and automated configuration reconstruction
title_fullStr Modeling extensive defects in metals through classical potential-guided sampling and automated configuration reconstruction
title_full_unstemmed Modeling extensive defects in metals through classical potential-guided sampling and automated configuration reconstruction
title_short Modeling extensive defects in metals through classical potential-guided sampling and automated configuration reconstruction
title_sort modeling extensive defects in metals through classical potential guided sampling and automated configuration reconstruction
url https://doi.org/10.1038/s41524-025-01599-1
work_keys_str_mv AT feishuang modelingextensivedefectsinmetalsthroughclassicalpotentialguidedsamplingandautomatedconfigurationreconstruction
AT kailiu modelingextensivedefectsinmetalsthroughclassicalpotentialguidedsamplingandautomatedconfigurationreconstruction
AT yuchengji modelingextensivedefectsinmetalsthroughclassicalpotentialguidedsamplingandautomatedconfigurationreconstruction
AT weigao modelingextensivedefectsinmetalsthroughclassicalpotentialguidedsamplingandautomatedconfigurationreconstruction
AT lucalaurenti modelingextensivedefectsinmetalsthroughclassicalpotentialguidedsamplingandautomatedconfigurationreconstruction
AT poulumidey modelingextensivedefectsinmetalsthroughclassicalpotentialguidedsamplingandautomatedconfigurationreconstruction