Extrusion of Heterogeneous Filament‐like Structures: A New Paradigm in Fabricating Soft Mechanical Gradient with Long Span

Soft‐to‐hard material interfaces found in multimaterial systems, such as microelectronics, prosthetics, body armor, and soft robotics, often suffer from mechanical mismatches that compromise their structural integrity overtime. These mismatches occur due to significant differences in mechanical prop...

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Main Authors: Akanksha Pragya, Tushar K. Ghosh
Format: Article
Language:English
Published: Wiley-VCH 2025-08-01
Series:Small Science
Subjects:
Online Access:https://doi.org/10.1002/smsc.202500234
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author Akanksha Pragya
Tushar K. Ghosh
author_facet Akanksha Pragya
Tushar K. Ghosh
author_sort Akanksha Pragya
collection DOAJ
description Soft‐to‐hard material interfaces found in multimaterial systems, such as microelectronics, prosthetics, body armor, and soft robotics, often suffer from mechanical mismatches that compromise their structural integrity overtime. These mismatches occur due to significant differences in mechanical properties, such as stiffness, between soft materials (e.g., polymers and biological tissues) and hard materials (e.g., metals and ceramics). In this study, an extrusion‐based approach is presented to fabricate continuous stiffness gradient materials using polydimethylsiloxane and thermoplastic expandable microspheres (EM). Morphological characterization shows the intended distribution of EM content along the length of the filament and the corresponding variation in tensile and bending stiffness. The gradient mechanical properties can be tuned by varying the EM expansion temperature. Compared to traditional fabrication techniques, this method allows for precise control over gradient magnitude and span, even post‐fabrication, offering greater flexibility for various applications. This work demonstrates a scalable and efficient solution for mitigating the mechanical mismatch at soft–hard material junctions, offering the potential for advanced material design in both industrial and biomedical applications.
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spelling doaj-art-d7d28bb2c8ba4191b51cd944ed44a7ac2025-08-20T04:02:31ZengWiley-VCHSmall Science2688-40462025-08-0158n/an/a10.1002/smsc.202500234Extrusion of Heterogeneous Filament‐like Structures: A New Paradigm in Fabricating Soft Mechanical Gradient with Long SpanAkanksha Pragya0Tushar K. Ghosh1Fiber and Polymer Science Program Department of Textile Engineering Chemistry and Science Wilson College of Textiles North Carolina State University Raleigh NC 27606 USAFiber and Polymer Science Program Department of Textile Engineering Chemistry and Science Wilson College of Textiles North Carolina State University Raleigh NC 27606 USASoft‐to‐hard material interfaces found in multimaterial systems, such as microelectronics, prosthetics, body armor, and soft robotics, often suffer from mechanical mismatches that compromise their structural integrity overtime. These mismatches occur due to significant differences in mechanical properties, such as stiffness, between soft materials (e.g., polymers and biological tissues) and hard materials (e.g., metals and ceramics). In this study, an extrusion‐based approach is presented to fabricate continuous stiffness gradient materials using polydimethylsiloxane and thermoplastic expandable microspheres (EM). Morphological characterization shows the intended distribution of EM content along the length of the filament and the corresponding variation in tensile and bending stiffness. The gradient mechanical properties can be tuned by varying the EM expansion temperature. Compared to traditional fabrication techniques, this method allows for precise control over gradient magnitude and span, even post‐fabrication, offering greater flexibility for various applications. This work demonstrates a scalable and efficient solution for mitigating the mechanical mismatch at soft–hard material junctions, offering the potential for advanced material design in both industrial and biomedical applications.https://doi.org/10.1002/smsc.202500234co‐extrusionexpandable microspheresmechanical gradientstrain distributionsoft‐hard interface
spellingShingle Akanksha Pragya
Tushar K. Ghosh
Extrusion of Heterogeneous Filament‐like Structures: A New Paradigm in Fabricating Soft Mechanical Gradient with Long Span
Small Science
co‐extrusion
expandable microspheres
mechanical gradient
strain distribution
soft‐hard interface
title Extrusion of Heterogeneous Filament‐like Structures: A New Paradigm in Fabricating Soft Mechanical Gradient with Long Span
title_full Extrusion of Heterogeneous Filament‐like Structures: A New Paradigm in Fabricating Soft Mechanical Gradient with Long Span
title_fullStr Extrusion of Heterogeneous Filament‐like Structures: A New Paradigm in Fabricating Soft Mechanical Gradient with Long Span
title_full_unstemmed Extrusion of Heterogeneous Filament‐like Structures: A New Paradigm in Fabricating Soft Mechanical Gradient with Long Span
title_short Extrusion of Heterogeneous Filament‐like Structures: A New Paradigm in Fabricating Soft Mechanical Gradient with Long Span
title_sort extrusion of heterogeneous filament like structures a new paradigm in fabricating soft mechanical gradient with long span
topic co‐extrusion
expandable microspheres
mechanical gradient
strain distribution
soft‐hard interface
url https://doi.org/10.1002/smsc.202500234
work_keys_str_mv AT akankshapragya extrusionofheterogeneousfilamentlikestructuresanewparadigminfabricatingsoftmechanicalgradientwithlongspan
AT tusharkghosh extrusionofheterogeneousfilamentlikestructuresanewparadigminfabricatingsoftmechanicalgradientwithlongspan