Nonthermal electron-photon steady states in open cavity quantum materials

Coupling a system to two different baths can lead to novel phenomena escaping the constraints of thermal equilibrium. In quantum materials inside optical cavities, this feature can be exploited as electrons and cavity photons are easily pulled away from their mutual equilibrium, even in the steady s...

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Main Authors: R. Flores-Calderón, Md Mursalin Islam, Michele Pini, Francesco Piazza
Format: Article
Language:English
Published: American Physical Society 2025-01-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.7.013073
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author R. Flores-Calderón
Md Mursalin Islam
Michele Pini
Francesco Piazza
author_facet R. Flores-Calderón
Md Mursalin Islam
Michele Pini
Francesco Piazza
author_sort R. Flores-Calderón
collection DOAJ
description Coupling a system to two different baths can lead to novel phenomena escaping the constraints of thermal equilibrium. In quantum materials inside optical cavities, this feature can be exploited as electrons and cavity photons are easily pulled away from their mutual equilibrium, even in the steady state. This offers new routes for a noninvasive control of material properties and functionalities. We show that the absence of thermal equilibrium between electrons and photons leads to reduced symmetries of the steady-state electronic distribution function. Moreover, by defining an effective temperature from the on-shell distribution function, we find a nonmonotonic behavior as a function of cavity frequency, consistent with recent experimental findings. Finally, we show that, the nonthermal behavior leads to qualitative modifications of the materials properties, as the standard Sommerfeld expansion for observables is modified by a leading-order correction linearly proportional to the temperature difference between the two baths and to the frequency derivative of the electron damping.
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institution Kabale University
issn 2643-1564
language English
publishDate 2025-01-01
publisher American Physical Society
record_format Article
series Physical Review Research
spelling doaj-art-d2431b427b044cd8addccb7325a2cd092025-01-21T15:11:52ZengAmerican Physical SocietyPhysical Review Research2643-15642025-01-017101307310.1103/PhysRevResearch.7.013073Nonthermal electron-photon steady states in open cavity quantum materialsR. Flores-CalderónMd Mursalin IslamMichele PiniFrancesco PiazzaCoupling a system to two different baths can lead to novel phenomena escaping the constraints of thermal equilibrium. In quantum materials inside optical cavities, this feature can be exploited as electrons and cavity photons are easily pulled away from their mutual equilibrium, even in the steady state. This offers new routes for a noninvasive control of material properties and functionalities. We show that the absence of thermal equilibrium between electrons and photons leads to reduced symmetries of the steady-state electronic distribution function. Moreover, by defining an effective temperature from the on-shell distribution function, we find a nonmonotonic behavior as a function of cavity frequency, consistent with recent experimental findings. Finally, we show that, the nonthermal behavior leads to qualitative modifications of the materials properties, as the standard Sommerfeld expansion for observables is modified by a leading-order correction linearly proportional to the temperature difference between the two baths and to the frequency derivative of the electron damping.http://doi.org/10.1103/PhysRevResearch.7.013073
spellingShingle R. Flores-Calderón
Md Mursalin Islam
Michele Pini
Francesco Piazza
Nonthermal electron-photon steady states in open cavity quantum materials
Physical Review Research
title Nonthermal electron-photon steady states in open cavity quantum materials
title_full Nonthermal electron-photon steady states in open cavity quantum materials
title_fullStr Nonthermal electron-photon steady states in open cavity quantum materials
title_full_unstemmed Nonthermal electron-photon steady states in open cavity quantum materials
title_short Nonthermal electron-photon steady states in open cavity quantum materials
title_sort nonthermal electron photon steady states in open cavity quantum materials
url http://doi.org/10.1103/PhysRevResearch.7.013073
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AT mdmursalinislam nonthermalelectronphotonsteadystatesinopencavityquantummaterials
AT michelepini nonthermalelectronphotonsteadystatesinopencavityquantummaterials
AT francescopiazza nonthermalelectronphotonsteadystatesinopencavityquantummaterials