Dehydration of γ-FeOOH: Direct Observation of the Mechanism

The dehydration of γ-FeOOH to γ-Fe2O3 has been investigated by thermoanalytical, electron microscopic and X-ray diffraction methods, using single crystals of suitably small size as a starting material, in order to maintain short diffusion paths. While kinetical data alone are not conclusive, the el...

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Bibliographic Details
Main Authors: Rudolf Giovanoli, Rudolf Brütsch
Format: Article
Language:deu
Published: Swiss Chemical Society 1974-04-01
Series:CHIMIA
Online Access:https://www.chimia.ch/chimia/article/view/9138
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Summary:The dehydration of γ-FeOOH to γ-Fe2O3 has been investigated by thermoanalytical, electron microscopic and X-ray diffraction methods, using single crystals of suitably small size as a starting material, in order to maintain short diffusion paths. While kinetical data alone are not conclusive, the electron micrographs show unambiguously how the reaction proceeds in the crystals: Strings of perfectly oriented γ-Fe2O3 crystallites of about 70 Å diameter and disordered lithium site vacancies extend into the undecomposed matrix crystal which can be distinguished from decomposed parts by direct imaging of the (120) lattice planes of 3 Å spacing. An atomistic interpretation of this result is given.
ISSN:0009-4293
2673-2424