Bond Model of Second- and Third-Harmonic Generation in Body- and Face-Centered Crystal Structures
In this work, we describe the third- and fourth-rank tensors of body- and face-centered cubic systems and derive the s- and p-polarized SHG far field using the simplified bond-hyperpolarizability model. We also briefly discuss bulk nonlinear sources in such structures: quadrupole contribution, spati...
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| Main Authors: | , , , |
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| Format: | Article |
| Language: | English |
| Published: |
Wiley
2018-01-01
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| Series: | Advances in Materials Science and Engineering |
| Online Access: | http://dx.doi.org/10.1155/2018/7153247 |
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| Summary: | In this work, we describe the third- and fourth-rank tensors of body- and face-centered cubic systems and derive the s- and p-polarized SHG far field using the simplified bond-hyperpolarizability model. We also briefly discuss bulk nonlinear sources in such structures: quadrupole contribution, spatial dispersion, electric-field second-harmonic generation, and third-harmonic generation, deriving the corresponding fourth rank tensor. We show that all the third- and fourth-rank tensorial elements require only one independent fitting parameter. |
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| ISSN: | 1687-8434 1687-8442 |