Visualization of Gas Diffusion-Sorption in Coal: A Study Based on Synchrotron Radiation Nano-CT

Gas diffusion-sorption is a critical step in coalbed methane (CBM) exploitation and carbon dioxide sequestration. Because of the particularity of gas physical properties, it is difficult to visualize the gas diffusion-sorption process in coal by experimental methods. Due to the limitation of experim...

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Main Authors: Yingfeng Sun, Yixin Zhao, Hongwei Zhang, Cun Zhang
Format: Article
Language:English
Published: Wiley 2020-01-01
Series:Geofluids
Online Access:http://dx.doi.org/10.1155/2020/8835848
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author Yingfeng Sun
Yixin Zhao
Hongwei Zhang
Cun Zhang
author_facet Yingfeng Sun
Yixin Zhao
Hongwei Zhang
Cun Zhang
author_sort Yingfeng Sun
collection DOAJ
description Gas diffusion-sorption is a critical step in coalbed methane (CBM) exploitation and carbon dioxide sequestration. Because of the particularity of gas physical properties, it is difficult to visualize the gas diffusion-sorption process in coal by experimental methods. Due to the limitation of experimental approaches to image the three-dimensional coal pore structure, it is impossible to obtain the three-dimensional pore structure images of coal. As a result, the visualization of gas diffusion-sorption in coal pore structure by numerical ways is impossible. In this study, gas diffusion coefficients were firstly estimated by experiments. Then, a gas diffusion-sorption coupled model was developed which can be applied to the nanoscale geometry imaged by synchrotron radiation nano-CT. The dynamic process of gas diffusion and ad-/desorption in the nanoscale microstructure of coal was visualized by the developed gas diffusion-adsorption coupled model and the numerical simulation based on MATLAB. The simulation results show a good agreement with the experimental results. The gas diffusion-sorption coupled model and numerical method can help to investigate the effect of microstructure on gas diffusion and ad-/desorption and provides a possibility to investigate the multiscale gas transportation and adsorption in coal pore-fracture system.
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institution Kabale University
issn 1468-8115
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language English
publishDate 2020-01-01
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series Geofluids
spelling doaj-art-c3f70e845bc54ee38603ffaa570e0ffb2025-02-03T01:05:13ZengWileyGeofluids1468-81151468-81232020-01-01202010.1155/2020/88358488835848Visualization of Gas Diffusion-Sorption in Coal: A Study Based on Synchrotron Radiation Nano-CTYingfeng Sun0Yixin Zhao1Hongwei Zhang2Cun Zhang3Beijing Key Laboratory for Precise Mining of Intergrown Energy and Resources, China University of Mining and Technology (Beijing), Beijing 100083, ChinaBeijing Key Laboratory for Precise Mining of Intergrown Energy and Resources, China University of Mining and Technology (Beijing), Beijing 100083, ChinaBeijing Key Laboratory for Precise Mining of Intergrown Energy and Resources, China University of Mining and Technology (Beijing), Beijing 100083, ChinaBeijing Key Laboratory for Precise Mining of Intergrown Energy and Resources, China University of Mining and Technology (Beijing), Beijing 100083, ChinaGas diffusion-sorption is a critical step in coalbed methane (CBM) exploitation and carbon dioxide sequestration. Because of the particularity of gas physical properties, it is difficult to visualize the gas diffusion-sorption process in coal by experimental methods. Due to the limitation of experimental approaches to image the three-dimensional coal pore structure, it is impossible to obtain the three-dimensional pore structure images of coal. As a result, the visualization of gas diffusion-sorption in coal pore structure by numerical ways is impossible. In this study, gas diffusion coefficients were firstly estimated by experiments. Then, a gas diffusion-sorption coupled model was developed which can be applied to the nanoscale geometry imaged by synchrotron radiation nano-CT. The dynamic process of gas diffusion and ad-/desorption in the nanoscale microstructure of coal was visualized by the developed gas diffusion-adsorption coupled model and the numerical simulation based on MATLAB. The simulation results show a good agreement with the experimental results. The gas diffusion-sorption coupled model and numerical method can help to investigate the effect of microstructure on gas diffusion and ad-/desorption and provides a possibility to investigate the multiscale gas transportation and adsorption in coal pore-fracture system.http://dx.doi.org/10.1155/2020/8835848
spellingShingle Yingfeng Sun
Yixin Zhao
Hongwei Zhang
Cun Zhang
Visualization of Gas Diffusion-Sorption in Coal: A Study Based on Synchrotron Radiation Nano-CT
Geofluids
title Visualization of Gas Diffusion-Sorption in Coal: A Study Based on Synchrotron Radiation Nano-CT
title_full Visualization of Gas Diffusion-Sorption in Coal: A Study Based on Synchrotron Radiation Nano-CT
title_fullStr Visualization of Gas Diffusion-Sorption in Coal: A Study Based on Synchrotron Radiation Nano-CT
title_full_unstemmed Visualization of Gas Diffusion-Sorption in Coal: A Study Based on Synchrotron Radiation Nano-CT
title_short Visualization of Gas Diffusion-Sorption in Coal: A Study Based on Synchrotron Radiation Nano-CT
title_sort visualization of gas diffusion sorption in coal a study based on synchrotron radiation nano ct
url http://dx.doi.org/10.1155/2020/8835848
work_keys_str_mv AT yingfengsun visualizationofgasdiffusionsorptionincoalastudybasedonsynchrotronradiationnanoct
AT yixinzhao visualizationofgasdiffusionsorptionincoalastudybasedonsynchrotronradiationnanoct
AT hongweizhang visualizationofgasdiffusionsorptionincoalastudybasedonsynchrotronradiationnanoct
AT cunzhang visualizationofgasdiffusionsorptionincoalastudybasedonsynchrotronradiationnanoct