Tropospheric ozone sensing with a differential absorption lidar based on a single CO<sub>2</sub> Raman cell

<p>This study presents the development and performance evaluation of an ozone differential absorption lidar system. The system could effectively obtain vertical profiles of lower-tropospheric ozone in an altitude range of 0.3 to 4 km with high spatiotemporal resolutions. The system emits three...

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Bibliographic Details
Main Authors: G. Fan, Y. Fu, J. Huo, Y. Xiang, T. Zhang, W. Liu, Z. Ning
Format: Article
Language:English
Published: Copernicus Publications 2025-01-01
Series:Atmospheric Measurement Techniques
Online Access:https://amt.copernicus.org/articles/18/443/2025/amt-18-443-2025.pdf
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Summary:<p>This study presents the development and performance evaluation of an ozone differential absorption lidar system. The system could effectively obtain vertical profiles of lower-tropospheric ozone in an altitude range of 0.3 to 4 km with high spatiotemporal resolutions. The system emits three laser beams at wavelengths of 276, 287 and 299 nm by using the stimulated Raman effect of carbon dioxide (CO<span class="inline-formula"><sub>2</sub>)</span>. A 250 mm telescope and a grating spectrometer are used to collect and separate the backscattering signals at the three wavelengths. Considering the influences of aerosol interference and statistical error, a wavelength pair of 276–287 nm is used for the altitude below 600 m and a wavelength pair of 287–299 nm is used for the altitude above 600 m to invert ozone concentration. We also evaluated the errors caused by the uncertainty of the wavelength index. The developed ozone lidar was deployed in a field campaign that was conducted to measure the vertical profiles of ozone using a tethered balloon platform. The lidar observations agree very well with those of the tethered balloon platform.</p>
ISSN:1867-1381
1867-8548