Evaluation of Fracture Toughness, Color Stability, and Sorption Solubility of a Fabricated Novel Glass Ionomer Nano Zirconia-Silica-Hydroxyapatite Hybrid Composite Material

The aim of this study was to investigate the effects of adding a nano zirconia-silica-hydroxyapatite (nanoZrO2-SiO2-HA) composite synthesized using a one-pot sol-gel technique to a conventional glass ionomer cement (GIC), which was then characterized using X-ray diffraction (XRD). Following the char...

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Main Authors: Sami D. Aldhuwayhi, Arbaz Sajjad, Wan Zaripah W. Bakar, Dasmawati Mohamad, Thirumulu P. Kannan, Imran A. Moheet
Format: Article
Language:English
Published: Wiley 2021-01-01
Series:International Journal of Polymer Science
Online Access:http://dx.doi.org/10.1155/2021/6626712
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author Sami D. Aldhuwayhi
Arbaz Sajjad
Wan Zaripah W. Bakar
Dasmawati Mohamad
Thirumulu P. Kannan
Imran A. Moheet
author_facet Sami D. Aldhuwayhi
Arbaz Sajjad
Wan Zaripah W. Bakar
Dasmawati Mohamad
Thirumulu P. Kannan
Imran A. Moheet
author_sort Sami D. Aldhuwayhi
collection DOAJ
description The aim of this study was to investigate the effects of adding a nano zirconia-silica-hydroxyapatite (nanoZrO2-SiO2-HA) composite synthesized using a one-pot sol-gel technique to a conventional glass ionomer cement (GIC), which was then characterized using X-ray diffraction (XRD). Following the characterization studies, further investigations were carried out after the addition of nanoZrO2-SiO2-HA to cGIC (GIC nanoZrO2-SiO2-HA) at various percentages (~5% to 9%) to compare their fracture toughness, color stability, and sorption- solubility in relation to cGIC (Fuji IX). The XRD diffractogram indicated the presence of peaks for ZrO2, SiO2, and HA. The fracture toughness of GIC 5%nanoZrO2-SiO2-HA was statistically higher than that of other percentages of GIC nanoZrO2-SiO2-HA and cGIC. The highest values recorded were fracture toughness (1.35±0.15 MPa.m1/2), leading to an increase of ∼57%, as compared to cGIC. Overall, the color change (ΔE) values for GIC 5% nano Zr-Si-HA group were lower than those of cGIC over a one-month period and were between slight and perceptible. In addition, GIC 5%nanoZrO2-SiO2-HA recorded lower sorption values (23.64±2.3 μgmm−3) as compared to cGIC (36.28±2.6 μgmm−3) and higher solubility (66.46±2.4 μgmm−3) as compared to cGIC (56.76±1.6 μgmm−3). The addition of nanoZrO2-SiO2-HA to cGIC significantly enhanced its physicomechanical properties. Based on the results of our study, GIC nanoZrO2-SiO2-HA has the potential to be suggested as a restorative dental material with diverse applications ranging from cavity restoration, core build-up, and as a luting material.
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spelling doaj-art-af38ecec615045c9990f23009162047e2025-02-03T01:29:18ZengWileyInternational Journal of Polymer Science1687-94221687-94302021-01-01202110.1155/2021/66267126626712Evaluation of Fracture Toughness, Color Stability, and Sorption Solubility of a Fabricated Novel Glass Ionomer Nano Zirconia-Silica-Hydroxyapatite Hybrid Composite MaterialSami D. Aldhuwayhi0Arbaz Sajjad1Wan Zaripah W. Bakar2Dasmawati Mohamad3Thirumulu P. Kannan4Imran A. Moheet5Department of Prosthodontics, College of Dentistry, Majmaah University, Al-Majmaah 11952, Saudi ArabiaDental Materials Department, School of Dental Sciences, Universiti Sains Malaysia, Health Campus, 16150 Kubang Kerian, Kota Bharu, Kelantan, MalaysiaConservative Dentistry Unit, School of Dental Sciences, Universiti Sains Malaysia, Health Campus, 16150 Kubang Kerian, Kota Bharu, Kelantan, MalaysiaBiomaterials Unit, School of Dental Sciences, Universiti Sains Malaysia, Health Campus, 16150 Kubang Kerian, Kota Bharu, Kelantan, MalaysiaHuman Genome Centre & School of Dental Sciences, Universiti Sains Malaysia, Health Campus, 16150 Kubang Kerian, Kota Bharu, Kelantan, MalaysiaDepartment of Dental Materials, Baqai Dental College, Baqai Medical University, PakistanThe aim of this study was to investigate the effects of adding a nano zirconia-silica-hydroxyapatite (nanoZrO2-SiO2-HA) composite synthesized using a one-pot sol-gel technique to a conventional glass ionomer cement (GIC), which was then characterized using X-ray diffraction (XRD). Following the characterization studies, further investigations were carried out after the addition of nanoZrO2-SiO2-HA to cGIC (GIC nanoZrO2-SiO2-HA) at various percentages (~5% to 9%) to compare their fracture toughness, color stability, and sorption- solubility in relation to cGIC (Fuji IX). The XRD diffractogram indicated the presence of peaks for ZrO2, SiO2, and HA. The fracture toughness of GIC 5%nanoZrO2-SiO2-HA was statistically higher than that of other percentages of GIC nanoZrO2-SiO2-HA and cGIC. The highest values recorded were fracture toughness (1.35±0.15 MPa.m1/2), leading to an increase of ∼57%, as compared to cGIC. Overall, the color change (ΔE) values for GIC 5% nano Zr-Si-HA group were lower than those of cGIC over a one-month period and were between slight and perceptible. In addition, GIC 5%nanoZrO2-SiO2-HA recorded lower sorption values (23.64±2.3 μgmm−3) as compared to cGIC (36.28±2.6 μgmm−3) and higher solubility (66.46±2.4 μgmm−3) as compared to cGIC (56.76±1.6 μgmm−3). The addition of nanoZrO2-SiO2-HA to cGIC significantly enhanced its physicomechanical properties. Based on the results of our study, GIC nanoZrO2-SiO2-HA has the potential to be suggested as a restorative dental material with diverse applications ranging from cavity restoration, core build-up, and as a luting material.http://dx.doi.org/10.1155/2021/6626712
spellingShingle Sami D. Aldhuwayhi
Arbaz Sajjad
Wan Zaripah W. Bakar
Dasmawati Mohamad
Thirumulu P. Kannan
Imran A. Moheet
Evaluation of Fracture Toughness, Color Stability, and Sorption Solubility of a Fabricated Novel Glass Ionomer Nano Zirconia-Silica-Hydroxyapatite Hybrid Composite Material
International Journal of Polymer Science
title Evaluation of Fracture Toughness, Color Stability, and Sorption Solubility of a Fabricated Novel Glass Ionomer Nano Zirconia-Silica-Hydroxyapatite Hybrid Composite Material
title_full Evaluation of Fracture Toughness, Color Stability, and Sorption Solubility of a Fabricated Novel Glass Ionomer Nano Zirconia-Silica-Hydroxyapatite Hybrid Composite Material
title_fullStr Evaluation of Fracture Toughness, Color Stability, and Sorption Solubility of a Fabricated Novel Glass Ionomer Nano Zirconia-Silica-Hydroxyapatite Hybrid Composite Material
title_full_unstemmed Evaluation of Fracture Toughness, Color Stability, and Sorption Solubility of a Fabricated Novel Glass Ionomer Nano Zirconia-Silica-Hydroxyapatite Hybrid Composite Material
title_short Evaluation of Fracture Toughness, Color Stability, and Sorption Solubility of a Fabricated Novel Glass Ionomer Nano Zirconia-Silica-Hydroxyapatite Hybrid Composite Material
title_sort evaluation of fracture toughness color stability and sorption solubility of a fabricated novel glass ionomer nano zirconia silica hydroxyapatite hybrid composite material
url http://dx.doi.org/10.1155/2021/6626712
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