A metastable hexagonal-IrSe2 with activated basal-plane selenium atoms for efficient hydrogen electrocatalysis

Developing novel layered transition metal dichalcogenides (TMDs) has gained tremendous interest due to their attractive physicochemical properties and promising applications. Herein, for the first, quasi-monolayered hexagonal-IrSe2 (h-IrSe2) nanosheets with metastable two-dimensional structure to th...

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Main Authors: Luhong Fu, Fulin Yang, Yunbo Li, Yuanmeng Zhao, Pengyu Han, Hongnan Jia, Chaoyi Yang, Wei Luo
Format: Article
Language:English
Published: Elsevier 2025-01-01
Series:Next Materials
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Online Access:http://www.sciencedirect.com/science/article/pii/S2949822824003617
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author Luhong Fu
Fulin Yang
Yunbo Li
Yuanmeng Zhao
Pengyu Han
Hongnan Jia
Chaoyi Yang
Wei Luo
author_facet Luhong Fu
Fulin Yang
Yunbo Li
Yuanmeng Zhao
Pengyu Han
Hongnan Jia
Chaoyi Yang
Wei Luo
author_sort Luhong Fu
collection DOAJ
description Developing novel layered transition metal dichalcogenides (TMDs) has gained tremendous interest due to their attractive physicochemical properties and promising applications. Herein, for the first, quasi-monolayered hexagonal-IrSe2 (h-IrSe2) nanosheets with metastable two-dimensional structure to the thermodynamically stable orthorhombic counterpart (o-IrSe2) have been prepared via the colloidal synthesis. Atomic-resolution transmission electron microscopy and spectroscopic characterizations confirm the 1 T configuration of the as-synthesized h-IrSe2, constructed from Ir-Se octahedra units. The metastable h-IrSe2 exhibits significantly enhanced performance for hydrogen evolution/oxidation reactions in alkaline media compared to o-IrSe2, even surpassing the metallic Ir nanoparticles. In situ Raman spectra and theoretical calculations reveal that the Se sites on the basal-plane of h-IrSe2 are the actual active sites. The obtained quasi-monolayered lamellar morphology of h-IrSe2 provides abundant basal-planes, thereby leading to increased effective electrochemical active area and enhanced mass activity. The activation of the basal-plane Se atoms could be attributed to the reduced local interband energy separation between the lowest empty d-band on Ir and the occupied p-band on Se, which is responsible for the optimized binding strength of the key intermediates during hydrogen electrocatalysis.
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spelling doaj-art-aeb80158341e48cbbc8a092ee63efbd62025-08-20T03:02:07ZengElsevierNext Materials2949-82282025-01-01610046310.1016/j.nxmate.2024.100463A metastable hexagonal-IrSe2 with activated basal-plane selenium atoms for efficient hydrogen electrocatalysisLuhong Fu0Fulin Yang1Yunbo Li2Yuanmeng Zhao3Pengyu Han4Hongnan Jia5Chaoyi Yang6Wei Luo7Faculty of Materials Science and Engineering, Kunming University of Science and Technology, Kunming 650093, ChinaFaculty of Materials Science and Engineering, Kunming University of Science and Technology, Kunming 650093, China; Corresponding authors.College of Chemistry and Molecular Sciences, Wuhan University, Wuhan 430072, ChinaCollege of Chemistry and Molecular Sciences, Wuhan University, Wuhan 430072, ChinaCollege of Chemistry and Molecular Sciences, Wuhan University, Wuhan 430072, ChinaCollege of Chemistry and Molecular Sciences, Wuhan University, Wuhan 430072, ChinaCollege of Chemistry and Molecular Sciences, Wuhan University, Wuhan 430072, ChinaCollege of Chemistry and Molecular Sciences, Wuhan University, Wuhan 430072, China; Corresponding authors.Developing novel layered transition metal dichalcogenides (TMDs) has gained tremendous interest due to their attractive physicochemical properties and promising applications. Herein, for the first, quasi-monolayered hexagonal-IrSe2 (h-IrSe2) nanosheets with metastable two-dimensional structure to the thermodynamically stable orthorhombic counterpart (o-IrSe2) have been prepared via the colloidal synthesis. Atomic-resolution transmission electron microscopy and spectroscopic characterizations confirm the 1 T configuration of the as-synthesized h-IrSe2, constructed from Ir-Se octahedra units. The metastable h-IrSe2 exhibits significantly enhanced performance for hydrogen evolution/oxidation reactions in alkaline media compared to o-IrSe2, even surpassing the metallic Ir nanoparticles. In situ Raman spectra and theoretical calculations reveal that the Se sites on the basal-plane of h-IrSe2 are the actual active sites. The obtained quasi-monolayered lamellar morphology of h-IrSe2 provides abundant basal-planes, thereby leading to increased effective electrochemical active area and enhanced mass activity. The activation of the basal-plane Se atoms could be attributed to the reduced local interband energy separation between the lowest empty d-band on Ir and the occupied p-band on Se, which is responsible for the optimized binding strength of the key intermediates during hydrogen electrocatalysis.http://www.sciencedirect.com/science/article/pii/S2949822824003617hexagonal-IrSe2Transition metal dichalcogenideTwo-dimensionalMetastable phaseHydrogen electrocatalysis
spellingShingle Luhong Fu
Fulin Yang
Yunbo Li
Yuanmeng Zhao
Pengyu Han
Hongnan Jia
Chaoyi Yang
Wei Luo
A metastable hexagonal-IrSe2 with activated basal-plane selenium atoms for efficient hydrogen electrocatalysis
Next Materials
hexagonal-IrSe2
Transition metal dichalcogenide
Two-dimensional
Metastable phase
Hydrogen electrocatalysis
title A metastable hexagonal-IrSe2 with activated basal-plane selenium atoms for efficient hydrogen electrocatalysis
title_full A metastable hexagonal-IrSe2 with activated basal-plane selenium atoms for efficient hydrogen electrocatalysis
title_fullStr A metastable hexagonal-IrSe2 with activated basal-plane selenium atoms for efficient hydrogen electrocatalysis
title_full_unstemmed A metastable hexagonal-IrSe2 with activated basal-plane selenium atoms for efficient hydrogen electrocatalysis
title_short A metastable hexagonal-IrSe2 with activated basal-plane selenium atoms for efficient hydrogen electrocatalysis
title_sort metastable hexagonal irse2 with activated basal plane selenium atoms for efficient hydrogen electrocatalysis
topic hexagonal-IrSe2
Transition metal dichalcogenide
Two-dimensional
Metastable phase
Hydrogen electrocatalysis
url http://www.sciencedirect.com/science/article/pii/S2949822824003617
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