Strain-enhanced two-photon absorption in twisted bilayer graphene

Abstract We theoretically investigate the strain-tuned moiré flat bands and two-photon absorption (TPA) in magic-angle (MA) twisted bilayer graphene (TBG). Using a low-energy continuum model for strained TBG and second-order perturbation theory, we demonstrate that uniaxial strain significantly modu...

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Main Authors: Lianmeng Yu, Zhaoming Fu, Peizhi Yang, Xiaobo Feng
Format: Article
Language:English
Published: Nature Portfolio 2025-05-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-025-00158-4
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author Lianmeng Yu
Zhaoming Fu
Peizhi Yang
Xiaobo Feng
author_facet Lianmeng Yu
Zhaoming Fu
Peizhi Yang
Xiaobo Feng
author_sort Lianmeng Yu
collection DOAJ
description Abstract We theoretically investigate the strain-tuned moiré flat bands and two-photon absorption (TPA) in magic-angle (MA) twisted bilayer graphene (TBG). Using a low-energy continuum model for strained TBG and second-order perturbation theory, we demonstrate that uniaxial strain significantly modulates both electronic and optical properties. Strain magnitude controls the flat band separation, while strain direction induces periodic variations in the band structure. The TPA spectra reveal strain-dependent features: intraband transitions dominate at higher strains, enhancing the absorption coefficient by an order of magnitude, while interband transitions exhibit characteristic spectral shifts. Notably, smaller strain direction angles yield larger TPA coefficients with red-shifted peaks. These results provide fundamental insights for developing strain-tunable optoelectronic devices based on moiré materials.
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issn 2045-2322
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publishDate 2025-05-01
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spelling doaj-art-ac28a211fa9c4fea893d4af86e34c61d2025-08-20T03:52:23ZengNature PortfolioScientific Reports2045-23222025-05-0115111010.1038/s41598-025-00158-4Strain-enhanced two-photon absorption in twisted bilayer grapheneLianmeng Yu0Zhaoming Fu1Peizhi Yang2Xiaobo Feng3School of Physics and Electronic Information, Yunnan Normal UniversitySchool of Physics and Electronic Information, Yunnan Normal UniversityKey Laboratory of Advanced Technique and Preparation for Renewable Energy Materials, Ministry of Education, Yunnan Normal UniversitySchool of Physics and Electronic Information, Yunnan Normal UniversityAbstract We theoretically investigate the strain-tuned moiré flat bands and two-photon absorption (TPA) in magic-angle (MA) twisted bilayer graphene (TBG). Using a low-energy continuum model for strained TBG and second-order perturbation theory, we demonstrate that uniaxial strain significantly modulates both electronic and optical properties. Strain magnitude controls the flat band separation, while strain direction induces periodic variations in the band structure. The TPA spectra reveal strain-dependent features: intraband transitions dominate at higher strains, enhancing the absorption coefficient by an order of magnitude, while interband transitions exhibit characteristic spectral shifts. Notably, smaller strain direction angles yield larger TPA coefficients with red-shifted peaks. These results provide fundamental insights for developing strain-tunable optoelectronic devices based on moiré materials.https://doi.org/10.1038/s41598-025-00158-4
spellingShingle Lianmeng Yu
Zhaoming Fu
Peizhi Yang
Xiaobo Feng
Strain-enhanced two-photon absorption in twisted bilayer graphene
Scientific Reports
title Strain-enhanced two-photon absorption in twisted bilayer graphene
title_full Strain-enhanced two-photon absorption in twisted bilayer graphene
title_fullStr Strain-enhanced two-photon absorption in twisted bilayer graphene
title_full_unstemmed Strain-enhanced two-photon absorption in twisted bilayer graphene
title_short Strain-enhanced two-photon absorption in twisted bilayer graphene
title_sort strain enhanced two photon absorption in twisted bilayer graphene
url https://doi.org/10.1038/s41598-025-00158-4
work_keys_str_mv AT lianmengyu strainenhancedtwophotonabsorptionintwistedbilayergraphene
AT zhaomingfu strainenhancedtwophotonabsorptionintwistedbilayergraphene
AT peizhiyang strainenhancedtwophotonabsorptionintwistedbilayergraphene
AT xiaobofeng strainenhancedtwophotonabsorptionintwistedbilayergraphene