Correlation of Dry Deposition Velocity and Friction Velocity over Different Surfaces for PM2.5 and Particle Number Concentrations

Dry deposition of particles is an important way of aerosol removal from the atmosphere and a key process in surface-atmosphere exchanges. The deposition velocities, Vd, are often parameterised in air quality and climate modelling as function of the friction velocity, u*, atmospheric stability, and p...

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Main Authors: Antonio Donateo, Daniele Contini
Format: Article
Language:English
Published: Wiley 2014-01-01
Series:Advances in Meteorology
Online Access:http://dx.doi.org/10.1155/2014/760393
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author Antonio Donateo
Daniele Contini
author_facet Antonio Donateo
Daniele Contini
author_sort Antonio Donateo
collection DOAJ
description Dry deposition of particles is an important way of aerosol removal from the atmosphere and a key process in surface-atmosphere exchanges. The deposition velocities, Vd, are often parameterised in air quality and climate modelling as function of the friction velocity, u*, atmospheric stability, and particle size (if size-segregated information is available). In this work, a study of the correlation between Vd and u* over different surfaces is presented for both PM2.5 and particle number fluxes. Results indicate an almost linear increase of Vd with u* with slopes similar for PM2.5 fluxes and particle number fluxes over the different surfaces analysed. This means that the ratios Vd/u* tend to collapse over similar values even if Vd and u* are significantly different because u* take into account most of the surface effects. There is a limited difference between stable cases and unstable/neutral cases with slightly lower deposition velocities in stable cases for fixed values of u*. The average value of Vd/u* is 0.010 ± 0.0017 (median 0.0062 ± 0.0015) (considering all stabilities) and 0.0097 ± 0.002 (median 0.005 ± 0.001) for stable cases. This could be the base for an empirical parameterisation of deposition velocities in air quality models.
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spelling doaj-art-aa4a82af6e974c1d90340ad0169e79472025-02-03T01:28:37ZengWileyAdvances in Meteorology1687-93091687-93172014-01-01201410.1155/2014/760393760393Correlation of Dry Deposition Velocity and Friction Velocity over Different Surfaces for PM2.5 and Particle Number ConcentrationsAntonio Donateo0Daniele Contini1Istituto di Scienze dell’Atmosfera e del Clima, ISAC-CNR, U.O.S. di Lecce, Strada Provinciale Lecce-Monteroni km 1.2, 73100 Lecce, ItalyIstituto di Scienze dell’Atmosfera e del Clima, ISAC-CNR, U.O.S. di Lecce, Strada Provinciale Lecce-Monteroni km 1.2, 73100 Lecce, ItalyDry deposition of particles is an important way of aerosol removal from the atmosphere and a key process in surface-atmosphere exchanges. The deposition velocities, Vd, are often parameterised in air quality and climate modelling as function of the friction velocity, u*, atmospheric stability, and particle size (if size-segregated information is available). In this work, a study of the correlation between Vd and u* over different surfaces is presented for both PM2.5 and particle number fluxes. Results indicate an almost linear increase of Vd with u* with slopes similar for PM2.5 fluxes and particle number fluxes over the different surfaces analysed. This means that the ratios Vd/u* tend to collapse over similar values even if Vd and u* are significantly different because u* take into account most of the surface effects. There is a limited difference between stable cases and unstable/neutral cases with slightly lower deposition velocities in stable cases for fixed values of u*. The average value of Vd/u* is 0.010 ± 0.0017 (median 0.0062 ± 0.0015) (considering all stabilities) and 0.0097 ± 0.002 (median 0.005 ± 0.001) for stable cases. This could be the base for an empirical parameterisation of deposition velocities in air quality models.http://dx.doi.org/10.1155/2014/760393
spellingShingle Antonio Donateo
Daniele Contini
Correlation of Dry Deposition Velocity and Friction Velocity over Different Surfaces for PM2.5 and Particle Number Concentrations
Advances in Meteorology
title Correlation of Dry Deposition Velocity and Friction Velocity over Different Surfaces for PM2.5 and Particle Number Concentrations
title_full Correlation of Dry Deposition Velocity and Friction Velocity over Different Surfaces for PM2.5 and Particle Number Concentrations
title_fullStr Correlation of Dry Deposition Velocity and Friction Velocity over Different Surfaces for PM2.5 and Particle Number Concentrations
title_full_unstemmed Correlation of Dry Deposition Velocity and Friction Velocity over Different Surfaces for PM2.5 and Particle Number Concentrations
title_short Correlation of Dry Deposition Velocity and Friction Velocity over Different Surfaces for PM2.5 and Particle Number Concentrations
title_sort correlation of dry deposition velocity and friction velocity over different surfaces for pm2 5 and particle number concentrations
url http://dx.doi.org/10.1155/2014/760393
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