Coherent harmonic generation of magnons in spin textures

Abstract Harmonic generation, a notable non-linear phenomenon, has promising applications in information processing. For spin-waves in ferromagnetic materials, great progress has been made in the generation higher harmonics, however probing the coherence of these higher harmonics is challenging. Her...

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Main Authors: Guibin Lan, Kang-Yuan Liu, Zhenyu Wang, Fan Xia, Hongjun Xu, Tengyu Guo, Yu Zhang, Bin He, Jiahui Li, Caihua Wan, Gerrit E. W. Bauer, Peng Yan, Gang-Qin Liu, Xin-Yu Pan, Xiufeng Han, Guoqiang Yu
Format: Article
Language:English
Published: Nature Portfolio 2025-01-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-56558-7
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author Guibin Lan
Kang-Yuan Liu
Zhenyu Wang
Fan Xia
Hongjun Xu
Tengyu Guo
Yu Zhang
Bin He
Jiahui Li
Caihua Wan
Gerrit E. W. Bauer
Peng Yan
Gang-Qin Liu
Xin-Yu Pan
Xiufeng Han
Guoqiang Yu
author_facet Guibin Lan
Kang-Yuan Liu
Zhenyu Wang
Fan Xia
Hongjun Xu
Tengyu Guo
Yu Zhang
Bin He
Jiahui Li
Caihua Wan
Gerrit E. W. Bauer
Peng Yan
Gang-Qin Liu
Xin-Yu Pan
Xiufeng Han
Guoqiang Yu
author_sort Guibin Lan
collection DOAJ
description Abstract Harmonic generation, a notable non-linear phenomenon, has promising applications in information processing. For spin-waves in ferromagnetic materials, great progress has been made in the generation higher harmonics, however probing the coherence of these higher harmonics is challenging. Here, using in-situ diamond sensors, we study the coherent harmonic generation of spin waves in a soft ferromagnet. High-order resonance lines are generated via a microwave input and detected by nitrogen-vacancy (NV) centers in nanodiamonds. The phase coherence of the harmonic spin waves is verified by the Rabi oscillations of the NV electron spins. Numerical simulations indicate that the harmonic generation by microwaves below the ferromagnetic resonance frequency is associated with the nonlinear mixing of spin waves by magnetization structures at the film edge. Our finding of geometry-induced magnon harmonic generation constitutes a new way to generate magnon combs with coherent high-order harmonics and may pave the way for magnon-based information processing and quantum sensing applications.
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publishDate 2025-01-01
publisher Nature Portfolio
record_format Article
series Nature Communications
spelling doaj-art-a81c3d0ccd374d3b98c582f7b381423c2025-02-02T12:31:13ZengNature PortfolioNature Communications2041-17232025-01-011611710.1038/s41467-025-56558-7Coherent harmonic generation of magnons in spin texturesGuibin Lan0Kang-Yuan Liu1Zhenyu Wang2Fan Xia3Hongjun Xu4Tengyu Guo5Yu Zhang6Bin He7Jiahui Li8Caihua Wan9Gerrit E. W. Bauer10Peng Yan11Gang-Qin Liu12Xin-Yu Pan13Xiufeng Han14Guoqiang Yu15Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesSchool of Physics and State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of ChinaBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesSongshan Lake Materials LaboratoryBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesKavli Institute for Theoretical Sciences, University of Chinese Academy of SciencesSchool of Physics and State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of ChinaBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesAbstract Harmonic generation, a notable non-linear phenomenon, has promising applications in information processing. For spin-waves in ferromagnetic materials, great progress has been made in the generation higher harmonics, however probing the coherence of these higher harmonics is challenging. Here, using in-situ diamond sensors, we study the coherent harmonic generation of spin waves in a soft ferromagnet. High-order resonance lines are generated via a microwave input and detected by nitrogen-vacancy (NV) centers in nanodiamonds. The phase coherence of the harmonic spin waves is verified by the Rabi oscillations of the NV electron spins. Numerical simulations indicate that the harmonic generation by microwaves below the ferromagnetic resonance frequency is associated with the nonlinear mixing of spin waves by magnetization structures at the film edge. Our finding of geometry-induced magnon harmonic generation constitutes a new way to generate magnon combs with coherent high-order harmonics and may pave the way for magnon-based information processing and quantum sensing applications.https://doi.org/10.1038/s41467-025-56558-7
spellingShingle Guibin Lan
Kang-Yuan Liu
Zhenyu Wang
Fan Xia
Hongjun Xu
Tengyu Guo
Yu Zhang
Bin He
Jiahui Li
Caihua Wan
Gerrit E. W. Bauer
Peng Yan
Gang-Qin Liu
Xin-Yu Pan
Xiufeng Han
Guoqiang Yu
Coherent harmonic generation of magnons in spin textures
Nature Communications
title Coherent harmonic generation of magnons in spin textures
title_full Coherent harmonic generation of magnons in spin textures
title_fullStr Coherent harmonic generation of magnons in spin textures
title_full_unstemmed Coherent harmonic generation of magnons in spin textures
title_short Coherent harmonic generation of magnons in spin textures
title_sort coherent harmonic generation of magnons in spin textures
url https://doi.org/10.1038/s41467-025-56558-7
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