Precise surface patches on active particles of arbitrary shape through microstenciling

Abstract Active particles, which locally dissipate energy from their environment to function, are useful across disciplines given their dynamic and programmable behaviors. Altering particle shape or surface asymmetry has led to advancements in controlled locomotion or collective behavior for diverse...

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Main Authors: Kendra M. Kreienbrink, Zoe A. Cruse, Alisha Kumari, C. Wyatt Shields
Format: Article
Language:English
Published: Nature Portfolio 2025-07-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-61218-x
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author Kendra M. Kreienbrink
Zoe A. Cruse
Alisha Kumari
C. Wyatt Shields
author_facet Kendra M. Kreienbrink
Zoe A. Cruse
Alisha Kumari
C. Wyatt Shields
author_sort Kendra M. Kreienbrink
collection DOAJ
description Abstract Active particles, which locally dissipate energy from their environment to function, are useful across disciplines given their dynamic and programmable behaviors. Altering particle shape or surface asymmetry has led to advancements in controlled locomotion or collective behavior for diverse applications such as microrobotics or biomedicine. However, making arbitrary active particles of precise shape and surface composition remains a significant challenge due to limitations in conventional fabrication methods. This paper introduces a fabrication technique that combines two-photon lithography with sacrificial stencil masking to deposit arbitrary metallic patches onto particles of any shape with a limit of resolution as low as 0.2 µm. Using this method, we demonstrate three varieties of active particles displaying nonconventional dynamics: electrokinetic active spheres with tunable three-dimensional motions, catalytic microdiscs with chiral axial spinning, and steric magnetic particles forming self-limiting microrobots. Overall, this high-resolution microstenciling technique offers a versatile strategy to create well-defined active particles and microrobots for numerous practical uses.
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institution Kabale University
issn 2041-1723
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publishDate 2025-07-01
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spelling doaj-art-a2c9645c38cc4f2d84d62f81355b47d62025-08-20T03:37:38ZengNature PortfolioNature Communications2041-17232025-07-0116111210.1038/s41467-025-61218-xPrecise surface patches on active particles of arbitrary shape through microstencilingKendra M. Kreienbrink0Zoe A. Cruse1Alisha Kumari2C. Wyatt Shields3Materials Science and Engineering Program, University of Colorado BoulderDepartment of Chemical and Biological Engineering, University of Colorado BoulderBiomedical Engineering Program, University of Colorado BoulderMaterials Science and Engineering Program, University of Colorado BoulderAbstract Active particles, which locally dissipate energy from their environment to function, are useful across disciplines given their dynamic and programmable behaviors. Altering particle shape or surface asymmetry has led to advancements in controlled locomotion or collective behavior for diverse applications such as microrobotics or biomedicine. However, making arbitrary active particles of precise shape and surface composition remains a significant challenge due to limitations in conventional fabrication methods. This paper introduces a fabrication technique that combines two-photon lithography with sacrificial stencil masking to deposit arbitrary metallic patches onto particles of any shape with a limit of resolution as low as 0.2 µm. Using this method, we demonstrate three varieties of active particles displaying nonconventional dynamics: electrokinetic active spheres with tunable three-dimensional motions, catalytic microdiscs with chiral axial spinning, and steric magnetic particles forming self-limiting microrobots. Overall, this high-resolution microstenciling technique offers a versatile strategy to create well-defined active particles and microrobots for numerous practical uses.https://doi.org/10.1038/s41467-025-61218-x
spellingShingle Kendra M. Kreienbrink
Zoe A. Cruse
Alisha Kumari
C. Wyatt Shields
Precise surface patches on active particles of arbitrary shape through microstenciling
Nature Communications
title Precise surface patches on active particles of arbitrary shape through microstenciling
title_full Precise surface patches on active particles of arbitrary shape through microstenciling
title_fullStr Precise surface patches on active particles of arbitrary shape through microstenciling
title_full_unstemmed Precise surface patches on active particles of arbitrary shape through microstenciling
title_short Precise surface patches on active particles of arbitrary shape through microstenciling
title_sort precise surface patches on active particles of arbitrary shape through microstenciling
url https://doi.org/10.1038/s41467-025-61218-x
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AT alishakumari precisesurfacepatchesonactiveparticlesofarbitraryshapethroughmicrostenciling
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