Field measurement of atmospheric CO₂ column abundance based on portable laser heterodyne radiometer

This study presents a portable near-infrared laser heterodyne radiometer specifically designed for measuring the column abundance of atmospheric carbon dioxide (CO₂) in the Taiyuan area. The instrument modulates the solar radiation using a fiber optic switch and amplifies the solar radiation through...

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Main Authors: Yong Wang, Maolei Zhang, Jiapeng Wang, Gang Wang, Ruyue Cui, Lei Dong, Hongpeng Wu
Format: Article
Language:English
Published: Frontiers Media S.A. 2025-02-01
Series:Frontiers in Physics
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Online Access:https://www.frontiersin.org/articles/10.3389/fphy.2025.1553252/full
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author Yong Wang
Yong Wang
Maolei Zhang
Maolei Zhang
Jiapeng Wang
Jiapeng Wang
Gang Wang
Gang Wang
Ruyue Cui
Ruyue Cui
Lei Dong
Lei Dong
Hongpeng Wu
Hongpeng Wu
author_facet Yong Wang
Yong Wang
Maolei Zhang
Maolei Zhang
Jiapeng Wang
Jiapeng Wang
Gang Wang
Gang Wang
Ruyue Cui
Ruyue Cui
Lei Dong
Lei Dong
Hongpeng Wu
Hongpeng Wu
author_sort Yong Wang
collection DOAJ
description This study presents a portable near-infrared laser heterodyne radiometer specifically designed for measuring the column abundance of atmospheric carbon dioxide (CO₂) in the Taiyuan area. The instrument modulates the solar radiation using a fiber optic switch and amplifies the solar radiation through a semiconductor optical amplifier. The local oscillator laser is progressively scanned at the strong absorption characteristic of 1572.02 nm. Two beams of light are mixed on the photodetector to produce a heterodyne signal. To enhance performance, the radio frequency (RF) circuit system of the radiometer was thoroughly optimized, including adjustments to the filter bandwidth and the integration time of the lock-in amplifier. These improvements significantly enhanced the spectral signal-to-noise ratio (SNR) to a high level of 130 and achieved a spectral resolution of 0.0083 cm⁻1. The laser heterodyne signals were demodulated using a lock-in amplifier. Furthermore, a forward model based on line-by-line integration and an iterative fitting algorithm were employed to achieve high-precision CO₂ column abundance calculations. Outdoor field measurements conducted at Shanxi University validated the feasibility and practicality of this approach, laying a solid foundation for its broader application.
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institution Kabale University
issn 2296-424X
language English
publishDate 2025-02-01
publisher Frontiers Media S.A.
record_format Article
series Frontiers in Physics
spelling doaj-art-9c10cb3da1e44a088ac3921829a056612025-02-04T05:28:02ZengFrontiers Media S.A.Frontiers in Physics2296-424X2025-02-011310.3389/fphy.2025.15532521553252Field measurement of atmospheric CO₂ column abundance based on portable laser heterodyne radiometerYong Wang0Yong Wang1Maolei Zhang2Maolei Zhang3Jiapeng Wang4Jiapeng Wang5Gang Wang6Gang Wang7Ruyue Cui8Ruyue Cui9Lei Dong10Lei Dong11Hongpeng Wu12Hongpeng Wu13State Key Laboratory of Quantum Optics Technologies and Devices, Institute of Laser Spectroscopy, Shanxi University, Taiyuan, ChinaCollaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, ChinaState Key Laboratory of Quantum Optics Technologies and Devices, Institute of Laser Spectroscopy, Shanxi University, Taiyuan, ChinaCollaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, ChinaState Key Laboratory of Quantum Optics Technologies and Devices, Institute of Laser Spectroscopy, Shanxi University, Taiyuan, ChinaCollaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, ChinaState Key Laboratory of Quantum Optics Technologies and Devices, Institute of Laser Spectroscopy, Shanxi University, Taiyuan, ChinaCollaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, ChinaState Key Laboratory of Quantum Optics Technologies and Devices, Institute of Laser Spectroscopy, Shanxi University, Taiyuan, ChinaCollaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, ChinaState Key Laboratory of Quantum Optics Technologies and Devices, Institute of Laser Spectroscopy, Shanxi University, Taiyuan, ChinaCollaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, ChinaState Key Laboratory of Quantum Optics Technologies and Devices, Institute of Laser Spectroscopy, Shanxi University, Taiyuan, ChinaCollaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, ChinaThis study presents a portable near-infrared laser heterodyne radiometer specifically designed for measuring the column abundance of atmospheric carbon dioxide (CO₂) in the Taiyuan area. The instrument modulates the solar radiation using a fiber optic switch and amplifies the solar radiation through a semiconductor optical amplifier. The local oscillator laser is progressively scanned at the strong absorption characteristic of 1572.02 nm. Two beams of light are mixed on the photodetector to produce a heterodyne signal. To enhance performance, the radio frequency (RF) circuit system of the radiometer was thoroughly optimized, including adjustments to the filter bandwidth and the integration time of the lock-in amplifier. These improvements significantly enhanced the spectral signal-to-noise ratio (SNR) to a high level of 130 and achieved a spectral resolution of 0.0083 cm⁻1. The laser heterodyne signals were demodulated using a lock-in amplifier. Furthermore, a forward model based on line-by-line integration and an iterative fitting algorithm were employed to achieve high-precision CO₂ column abundance calculations. Outdoor field measurements conducted at Shanxi University validated the feasibility and practicality of this approach, laying a solid foundation for its broader application.https://www.frontiersin.org/articles/10.3389/fphy.2025.1553252/fulllaser heterodynecarbon dioxidecolumn abundanceportablegreenhouse gas
spellingShingle Yong Wang
Yong Wang
Maolei Zhang
Maolei Zhang
Jiapeng Wang
Jiapeng Wang
Gang Wang
Gang Wang
Ruyue Cui
Ruyue Cui
Lei Dong
Lei Dong
Hongpeng Wu
Hongpeng Wu
Field measurement of atmospheric CO₂ column abundance based on portable laser heterodyne radiometer
Frontiers in Physics
laser heterodyne
carbon dioxide
column abundance
portable
greenhouse gas
title Field measurement of atmospheric CO₂ column abundance based on portable laser heterodyne radiometer
title_full Field measurement of atmospheric CO₂ column abundance based on portable laser heterodyne radiometer
title_fullStr Field measurement of atmospheric CO₂ column abundance based on portable laser heterodyne radiometer
title_full_unstemmed Field measurement of atmospheric CO₂ column abundance based on portable laser heterodyne radiometer
title_short Field measurement of atmospheric CO₂ column abundance based on portable laser heterodyne radiometer
title_sort field measurement of atmospheric co₂ column abundance based on portable laser heterodyne radiometer
topic laser heterodyne
carbon dioxide
column abundance
portable
greenhouse gas
url https://www.frontiersin.org/articles/10.3389/fphy.2025.1553252/full
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