Burst plasma preparation of metallic nanoparticles on carbon fabrics for antibacterial and electrocatalytic applications

Abstract Metal nanoparticles have extraordinary properties, but their integration into mesostructures has been challenging. Producing uniformly dispersed nanoparticles attached to substrates in industrial quantities is difficult. Herein, a “plasmashock” method was developed to synthesize metal nanop...

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Main Authors: Guiyin Xu, Zheyi Meng, Yunteng Cao, Zixu Tao, Qing-Jie Li, Myles Stapelberg, Bing Han, Rui Gao, Qipeng Yu, Meng Gu, Benedetto Marelli, Hailiang Wang, Meifang Zhu, Ju Li
Format: Article
Language:English
Published: Nature Portfolio 2024-10-01
Series:NPG Asia Materials
Online Access:https://doi.org/10.1038/s41427-024-00566-4
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author Guiyin Xu
Zheyi Meng
Yunteng Cao
Zixu Tao
Qing-Jie Li
Myles Stapelberg
Bing Han
Rui Gao
Qipeng Yu
Meng Gu
Benedetto Marelli
Hailiang Wang
Meifang Zhu
Ju Li
author_facet Guiyin Xu
Zheyi Meng
Yunteng Cao
Zixu Tao
Qing-Jie Li
Myles Stapelberg
Bing Han
Rui Gao
Qipeng Yu
Meng Gu
Benedetto Marelli
Hailiang Wang
Meifang Zhu
Ju Li
author_sort Guiyin Xu
collection DOAJ
description Abstract Metal nanoparticles have extraordinary properties, but their integration into mesostructures has been challenging. Producing uniformly dispersed nanoparticles attached to substrates in industrial quantities is difficult. Herein, a “plasmashock” method was developed to synthesize metal nanoparticles anchored on different types of carbonaceous substrates using liquid salt solution precursors. These self-supporting, nanoparticle-loaded carbon fabrics are mechanically robust and have been tested as antibacterial substrates and electrocatalysts for reducing carbon dioxide and nitrite. A piece of silver–carbon nanotube paper with a silver loading of ~0.13 mg cm−2 treated after a few-second plasmashock presents good antibacterial and electrocatalytic properties in wastewater, even after 20 bactericidal immersion cycles, due to the strong bonding of the nanoparticles to the substrate. The results prove the effectiveness of this plasmashock method in creating free-standing functional composite films or membranes.
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institution Kabale University
issn 1884-4057
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publishDate 2024-10-01
publisher Nature Portfolio
record_format Article
series NPG Asia Materials
spelling doaj-art-99b3bacdc9564efa9521be62786f3d5c2025-01-19T12:28:57ZengNature PortfolioNPG Asia Materials1884-40572024-10-0116111110.1038/s41427-024-00566-4Burst plasma preparation of metallic nanoparticles on carbon fabrics for antibacterial and electrocatalytic applicationsGuiyin Xu0Zheyi Meng1Yunteng Cao2Zixu Tao3Qing-Jie Li4Myles Stapelberg5Bing Han6Rui Gao7Qipeng Yu8Meng Gu9Benedetto Marelli10Hailiang Wang11Meifang Zhu12Ju Li13State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Donghua UniversityState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Donghua UniversityDepartment of Civil and Environmental Engineering, Massachusetts Institute of TechnologyDepartment of Chemistry and Energy Sciences Institute, Yale UniversityDepartment of Materials Science and Engineering, and Department of Nuclear Science and Engineering, Massachusetts Institute of TechnologyDepartment of Materials Science and Engineering, and Department of Nuclear Science and Engineering, Massachusetts Institute of TechnologyDepartment of Materials Science and Engineering, Southern University of Science and TechnologyDepartment of Materials Science and Engineering, and Department of Nuclear Science and Engineering, Massachusetts Institute of TechnologyDepartment of Materials Science and Engineering, and Department of Nuclear Science and Engineering, Massachusetts Institute of TechnologyDepartment of Materials Science and Engineering, Southern University of Science and TechnologyDepartment of Civil and Environmental Engineering, Massachusetts Institute of TechnologyDepartment of Chemistry and Energy Sciences Institute, Yale UniversityState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Donghua UniversityDepartment of Materials Science and Engineering, and Department of Nuclear Science and Engineering, Massachusetts Institute of TechnologyAbstract Metal nanoparticles have extraordinary properties, but their integration into mesostructures has been challenging. Producing uniformly dispersed nanoparticles attached to substrates in industrial quantities is difficult. Herein, a “plasmashock” method was developed to synthesize metal nanoparticles anchored on different types of carbonaceous substrates using liquid salt solution precursors. These self-supporting, nanoparticle-loaded carbon fabrics are mechanically robust and have been tested as antibacterial substrates and electrocatalysts for reducing carbon dioxide and nitrite. A piece of silver–carbon nanotube paper with a silver loading of ~0.13 mg cm−2 treated after a few-second plasmashock presents good antibacterial and electrocatalytic properties in wastewater, even after 20 bactericidal immersion cycles, due to the strong bonding of the nanoparticles to the substrate. The results prove the effectiveness of this plasmashock method in creating free-standing functional composite films or membranes.https://doi.org/10.1038/s41427-024-00566-4
spellingShingle Guiyin Xu
Zheyi Meng
Yunteng Cao
Zixu Tao
Qing-Jie Li
Myles Stapelberg
Bing Han
Rui Gao
Qipeng Yu
Meng Gu
Benedetto Marelli
Hailiang Wang
Meifang Zhu
Ju Li
Burst plasma preparation of metallic nanoparticles on carbon fabrics for antibacterial and electrocatalytic applications
NPG Asia Materials
title Burst plasma preparation of metallic nanoparticles on carbon fabrics for antibacterial and electrocatalytic applications
title_full Burst plasma preparation of metallic nanoparticles on carbon fabrics for antibacterial and electrocatalytic applications
title_fullStr Burst plasma preparation of metallic nanoparticles on carbon fabrics for antibacterial and electrocatalytic applications
title_full_unstemmed Burst plasma preparation of metallic nanoparticles on carbon fabrics for antibacterial and electrocatalytic applications
title_short Burst plasma preparation of metallic nanoparticles on carbon fabrics for antibacterial and electrocatalytic applications
title_sort burst plasma preparation of metallic nanoparticles on carbon fabrics for antibacterial and electrocatalytic applications
url https://doi.org/10.1038/s41427-024-00566-4
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