Oily-wastewater treatment using eco-friendly ceramic membranes derived from sugarcane bagasse waste: Optimization using response surface methodology

Treating oily-wastewater through separation technologies with advanced properties such as environmental-friendly and low cost is a challenging work. Herein, we successfully fabricated superhydrophic-superoleophilic green ceramic hollow fibre membrane prepared from sugarcane bagasse waste and modifie...

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Main Authors: Nurhayati Jamalludin, Mohd Riduan Jamalludin, Siti Khadijah Hubadillah, Mohd Hafiz Dzarfan Othman, Mohd Azizi Hakim Jamalludin
Format: Article
Language:English
Published: Elsevier 2025-12-01
Series:Cleaner Chemical Engineering
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Online Access:http://www.sciencedirect.com/science/article/pii/S2772782325000063
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author Nurhayati Jamalludin
Mohd Riduan Jamalludin
Siti Khadijah Hubadillah
Mohd Hafiz Dzarfan Othman
Mohd Azizi Hakim Jamalludin
author_facet Nurhayati Jamalludin
Mohd Riduan Jamalludin
Siti Khadijah Hubadillah
Mohd Hafiz Dzarfan Othman
Mohd Azizi Hakim Jamalludin
author_sort Nurhayati Jamalludin
collection DOAJ
description Treating oily-wastewater through separation technologies with advanced properties such as environmental-friendly and low cost is a challenging work. Herein, we successfully fabricated superhydrophic-superoleophilic green ceramic hollow fibre membrane prepared from sugarcane bagasse waste and modified through sol-gel method. Later, this study aims to optimize wastewater behaviour (pH, concentration and temperature) for oily-wastewater separation through green ceramic membrane using central composite design (CCD) of response surface methods (RSM). The three effective parameters analyzed were oil pH (3–11), oil concentration (10–10000 ppm), oil temperature (30–100 °C) and its combined effect to obtain high oil flux and excellent oil separation efficiency. Through the investigation it was found that the optimum value of pH, oil concentration and temperature were 10, 10.01 ppm and 69.04 °C. The result of the study has suggested that there are oil temperature has significantly influence the efficiency of the synthesized membrane separation performance. The fitted model was found to agree with the predicted and actual oil flux as well as separation efficiency which indicated by the high values of R2 = 0.954 and R2adj = 0.986. According to the optimized condition, the finding reported 4.71 % and 0.746 % average error for oil flux and separation efficiency which agrees with the forecasted and actual values. The novelty of this study lies in the development of an eco-friendly ceramic membrane derived from sugarcane bagasse waste, offering an innovative and sustainable solution for oily-wastewater treatment.
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spelling doaj-art-9970dab0e3df4fdf9f756e935ef2dabd2025-02-02T05:29:35ZengElsevierCleaner Chemical Engineering2772-78232025-12-0111100151Oily-wastewater treatment using eco-friendly ceramic membranes derived from sugarcane bagasse waste: Optimization using response surface methodologyNurhayati Jamalludin0Mohd Riduan Jamalludin1Siti Khadijah Hubadillah2Mohd Hafiz Dzarfan Othman3Mohd Azizi Hakim Jamalludin4Advanced Membrane Technology Research Centre (AMTEC), Faculty of Chemical and Energy Engineering, Universiti Teknologi Malaysia, 81310 Skudai, Johor, MalaysiaFaculty of Mechanical Engineering & Technology, Universiti Malaysia Perlis, Kampus Tetap Pauh Putra, 026000 Arau, Perlis, Malaysia; Corresponding author.School of Technology Management and Logistics, College of Business, Universiti Utara Malaysia, 06010 UUM Sintok, Kedah, MalaysiaAdvanced Membrane Technology Research Centre (AMTEC), Faculty of Chemical and Energy Engineering, Universiti Teknologi Malaysia, 81310 Skudai, Johor, MalaysiaAdvanced Membrane Technology Research Centre (AMTEC), Faculty of Chemical and Energy Engineering, Universiti Teknologi Malaysia, 81310 Skudai, Johor, MalaysiaTreating oily-wastewater through separation technologies with advanced properties such as environmental-friendly and low cost is a challenging work. Herein, we successfully fabricated superhydrophic-superoleophilic green ceramic hollow fibre membrane prepared from sugarcane bagasse waste and modified through sol-gel method. Later, this study aims to optimize wastewater behaviour (pH, concentration and temperature) for oily-wastewater separation through green ceramic membrane using central composite design (CCD) of response surface methods (RSM). The three effective parameters analyzed were oil pH (3–11), oil concentration (10–10000 ppm), oil temperature (30–100 °C) and its combined effect to obtain high oil flux and excellent oil separation efficiency. Through the investigation it was found that the optimum value of pH, oil concentration and temperature were 10, 10.01 ppm and 69.04 °C. The result of the study has suggested that there are oil temperature has significantly influence the efficiency of the synthesized membrane separation performance. The fitted model was found to agree with the predicted and actual oil flux as well as separation efficiency which indicated by the high values of R2 = 0.954 and R2adj = 0.986. According to the optimized condition, the finding reported 4.71 % and 0.746 % average error for oil flux and separation efficiency which agrees with the forecasted and actual values. The novelty of this study lies in the development of an eco-friendly ceramic membrane derived from sugarcane bagasse waste, offering an innovative and sustainable solution for oily-wastewater treatment.http://www.sciencedirect.com/science/article/pii/S2772782325000063Response surface methodologyCeramic membraneSugarcane bagasse wasteSol-gelsuperhydrophobicSuperoleophilic
spellingShingle Nurhayati Jamalludin
Mohd Riduan Jamalludin
Siti Khadijah Hubadillah
Mohd Hafiz Dzarfan Othman
Mohd Azizi Hakim Jamalludin
Oily-wastewater treatment using eco-friendly ceramic membranes derived from sugarcane bagasse waste: Optimization using response surface methodology
Cleaner Chemical Engineering
Response surface methodology
Ceramic membrane
Sugarcane bagasse waste
Sol-gel
superhydrophobic
Superoleophilic
title Oily-wastewater treatment using eco-friendly ceramic membranes derived from sugarcane bagasse waste: Optimization using response surface methodology
title_full Oily-wastewater treatment using eco-friendly ceramic membranes derived from sugarcane bagasse waste: Optimization using response surface methodology
title_fullStr Oily-wastewater treatment using eco-friendly ceramic membranes derived from sugarcane bagasse waste: Optimization using response surface methodology
title_full_unstemmed Oily-wastewater treatment using eco-friendly ceramic membranes derived from sugarcane bagasse waste: Optimization using response surface methodology
title_short Oily-wastewater treatment using eco-friendly ceramic membranes derived from sugarcane bagasse waste: Optimization using response surface methodology
title_sort oily wastewater treatment using eco friendly ceramic membranes derived from sugarcane bagasse waste optimization using response surface methodology
topic Response surface methodology
Ceramic membrane
Sugarcane bagasse waste
Sol-gel
superhydrophobic
Superoleophilic
url http://www.sciencedirect.com/science/article/pii/S2772782325000063
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