Study of phase evolution and phase stability in a novel FCC based Al30Ti35Mg5V10Fe8Cr12 lightweight high-entropy alloy processed by mechanical alloying

High-entropy alloys (HEAs) have gained significant attention from researchers due to their exceptional mechanical properties. While most the reported lightweight high-entropy alloys have Body Centered Cubic (BCC), Hexagonal Close Packed (HCP), and complex intermetallic phases, there is growing inter...

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Main Authors: Ayush Sourav, Ankit Singh Negi, Pranjal Chauhan, T. Sudeep Kumar, Shanmugasundaram Thangaraju
Format: Article
Language:English
Published: Elsevier 2025-03-01
Series:Journal of Alloys and Metallurgical Systems
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Online Access:http://www.sciencedirect.com/science/article/pii/S2949917824000919
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author Ayush Sourav
Ankit Singh Negi
Pranjal Chauhan
T. Sudeep Kumar
Shanmugasundaram Thangaraju
author_facet Ayush Sourav
Ankit Singh Negi
Pranjal Chauhan
T. Sudeep Kumar
Shanmugasundaram Thangaraju
author_sort Ayush Sourav
collection DOAJ
description High-entropy alloys (HEAs) have gained significant attention from researchers due to their exceptional mechanical properties. While most the reported lightweight high-entropy alloys have Body Centered Cubic (BCC), Hexagonal Close Packed (HCP), and complex intermetallic phases, there is growing interest in development of Face Centered Cubic (FCC) based Lightweight High-Entropy Alloys (LWHEA) for applications prioritizing energy efficiency. In this study, a design strategy for synthesizing a stable FCC-based LWHEA through multivariate optimization of elements and thermodynamic parameters was presented. A novel Al30Ti35Mg5V10Fe8Cr12 LWHEA was designed and processed through a mechanical alloying route with a theoretical density of 4.5 g/cc. The compaction of the alloy was performed by spark plasma sintering (SPS) at 890 ℃ and 60 MPa for 15 minutes. The hardness of sintered sample was found to be 550 ± 18 HV (5.3 GPa). Microstructural evolution of the alloy was studied using X-ray diffraction (XRD) and Scanning electron microscopy (SEM). The microstructural analysis of alloy revealed that a combination of FCC and BCC phases are present in milled sample as well as sintered sample. The phase stability was explained through Gibbs free energy calculations of competing phases.
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spelling doaj-art-94e28bde4e2840fba4f47c3da8baf4c42025-08-20T02:55:48ZengElsevierJournal of Alloys and Metallurgical Systems2949-91782025-03-01910014210.1016/j.jalmes.2024.100142Study of phase evolution and phase stability in a novel FCC based Al30Ti35Mg5V10Fe8Cr12 lightweight high-entropy alloy processed by mechanical alloyingAyush Sourav0Ankit Singh Negi1Pranjal Chauhan2T. Sudeep Kumar3Shanmugasundaram Thangaraju4Department of Metallurgical and Materials Engineering, Defence Institute of Advanced Technology, Pune, IndiaDepartment of Metallurgical and Materials Engineering, Defence Institute of Advanced Technology, Pune, IndiaDepartment of Metallurgical and Materials Engineering, Defence Institute of Advanced Technology, Pune, IndiaDepartment of Metallurgical and Materials Engineering, Defence Institute of Advanced Technology, Pune, India; Siddaganga Institute of Technology, Tumakuru, IndiaDepartment of Metallurgical and Materials Engineering, Defence Institute of Advanced Technology, Pune, India; Corresponding author.High-entropy alloys (HEAs) have gained significant attention from researchers due to their exceptional mechanical properties. While most the reported lightweight high-entropy alloys have Body Centered Cubic (BCC), Hexagonal Close Packed (HCP), and complex intermetallic phases, there is growing interest in development of Face Centered Cubic (FCC) based Lightweight High-Entropy Alloys (LWHEA) for applications prioritizing energy efficiency. In this study, a design strategy for synthesizing a stable FCC-based LWHEA through multivariate optimization of elements and thermodynamic parameters was presented. A novel Al30Ti35Mg5V10Fe8Cr12 LWHEA was designed and processed through a mechanical alloying route with a theoretical density of 4.5 g/cc. The compaction of the alloy was performed by spark plasma sintering (SPS) at 890 ℃ and 60 MPa for 15 minutes. The hardness of sintered sample was found to be 550 ± 18 HV (5.3 GPa). Microstructural evolution of the alloy was studied using X-ray diffraction (XRD) and Scanning electron microscopy (SEM). The microstructural analysis of alloy revealed that a combination of FCC and BCC phases are present in milled sample as well as sintered sample. The phase stability was explained through Gibbs free energy calculations of competing phases.http://www.sciencedirect.com/science/article/pii/S2949917824000919High entropy alloyLightweightMechanical alloyingMicrostructural evolutionGibbs free energy
spellingShingle Ayush Sourav
Ankit Singh Negi
Pranjal Chauhan
T. Sudeep Kumar
Shanmugasundaram Thangaraju
Study of phase evolution and phase stability in a novel FCC based Al30Ti35Mg5V10Fe8Cr12 lightweight high-entropy alloy processed by mechanical alloying
Journal of Alloys and Metallurgical Systems
High entropy alloy
Lightweight
Mechanical alloying
Microstructural evolution
Gibbs free energy
title Study of phase evolution and phase stability in a novel FCC based Al30Ti35Mg5V10Fe8Cr12 lightweight high-entropy alloy processed by mechanical alloying
title_full Study of phase evolution and phase stability in a novel FCC based Al30Ti35Mg5V10Fe8Cr12 lightweight high-entropy alloy processed by mechanical alloying
title_fullStr Study of phase evolution and phase stability in a novel FCC based Al30Ti35Mg5V10Fe8Cr12 lightweight high-entropy alloy processed by mechanical alloying
title_full_unstemmed Study of phase evolution and phase stability in a novel FCC based Al30Ti35Mg5V10Fe8Cr12 lightweight high-entropy alloy processed by mechanical alloying
title_short Study of phase evolution and phase stability in a novel FCC based Al30Ti35Mg5V10Fe8Cr12 lightweight high-entropy alloy processed by mechanical alloying
title_sort study of phase evolution and phase stability in a novel fcc based al30ti35mg5v10fe8cr12 lightweight high entropy alloy processed by mechanical alloying
topic High entropy alloy
Lightweight
Mechanical alloying
Microstructural evolution
Gibbs free energy
url http://www.sciencedirect.com/science/article/pii/S2949917824000919
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