Bottom-up fabrication of 2D Rydberg exciton arrays in cuprous oxide

Abstract Solid-state platforms provide exceptional opportunities for advancing on-chip quantum technologies by enhancing interaction strengths through coupling, scalability, and robustness. Cuprous oxide (Cu2O) has recently emerged as a promising medium for scalable quantum technology due to its hig...

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Main Authors: Kinjol Barua, Samuel Peana, Arya Deepak Keni, Vahagn Mkhitaryan, Vladimir M. Shalaev, Yong P. Chen, Alexandra Boltasseva, Hadiseh Alaeian
Format: Article
Language:English
Published: Nature Portfolio 2025-01-01
Series:Communications Materials
Online Access:https://doi.org/10.1038/s43246-025-00742-1
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author Kinjol Barua
Samuel Peana
Arya Deepak Keni
Vahagn Mkhitaryan
Vladimir M. Shalaev
Yong P. Chen
Alexandra Boltasseva
Hadiseh Alaeian
author_facet Kinjol Barua
Samuel Peana
Arya Deepak Keni
Vahagn Mkhitaryan
Vladimir M. Shalaev
Yong P. Chen
Alexandra Boltasseva
Hadiseh Alaeian
author_sort Kinjol Barua
collection DOAJ
description Abstract Solid-state platforms provide exceptional opportunities for advancing on-chip quantum technologies by enhancing interaction strengths through coupling, scalability, and robustness. Cuprous oxide (Cu2O) has recently emerged as a promising medium for scalable quantum technology due to its high-lying Rydberg excitonic states, akin to those in hydrogen atoms. To harness these nonlinearities for quantum applications, the confinement dimensions must match the Rydberg blockade size, which can reach several microns in Cu2O. Using a CMOS-compatible growth technique, this study demonstrates the bottom-up fabrication of site-selective arrays of Cu2O microparticles. We observed Rydberg excitons up to the principal quantum number n = 5 within these Cu2O arrays on a quartz substrate and analyzed the spatial variation of their spectrum across the array, showing robustness and reproducibility on a large chip. These results lay the groundwork for the deterministic growth of Cu2O around photonic structures, enabling substantial light-matter interaction on integrated photonic platforms and paving the way for scalable, on-chip quantum devices.
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institution Kabale University
issn 2662-4443
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publishDate 2025-01-01
publisher Nature Portfolio
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series Communications Materials
spelling doaj-art-8c9da43a25d445ffac06c5610538a2e62025-02-02T12:34:22ZengNature PortfolioCommunications Materials2662-44432025-01-01611810.1038/s43246-025-00742-1Bottom-up fabrication of 2D Rydberg exciton arrays in cuprous oxideKinjol Barua0Samuel Peana1Arya Deepak Keni2Vahagn Mkhitaryan3Vladimir M. Shalaev4Yong P. Chen5Alexandra Boltasseva6Hadiseh Alaeian7Elmore Family School of Electrical and Computer Engineering, Purdue UniversityElmore Family School of Electrical and Computer Engineering, Purdue UniversityElmore Family School of Electrical and Computer Engineering, Purdue UniversityElmore Family School of Electrical and Computer Engineering, Purdue UniversityElmore Family School of Electrical and Computer Engineering, Purdue UniversityElmore Family School of Electrical and Computer Engineering, Purdue UniversityElmore Family School of Electrical and Computer Engineering, Purdue UniversityElmore Family School of Electrical and Computer Engineering, Purdue UniversityAbstract Solid-state platforms provide exceptional opportunities for advancing on-chip quantum technologies by enhancing interaction strengths through coupling, scalability, and robustness. Cuprous oxide (Cu2O) has recently emerged as a promising medium for scalable quantum technology due to its high-lying Rydberg excitonic states, akin to those in hydrogen atoms. To harness these nonlinearities for quantum applications, the confinement dimensions must match the Rydberg blockade size, which can reach several microns in Cu2O. Using a CMOS-compatible growth technique, this study demonstrates the bottom-up fabrication of site-selective arrays of Cu2O microparticles. We observed Rydberg excitons up to the principal quantum number n = 5 within these Cu2O arrays on a quartz substrate and analyzed the spatial variation of their spectrum across the array, showing robustness and reproducibility on a large chip. These results lay the groundwork for the deterministic growth of Cu2O around photonic structures, enabling substantial light-matter interaction on integrated photonic platforms and paving the way for scalable, on-chip quantum devices.https://doi.org/10.1038/s43246-025-00742-1
spellingShingle Kinjol Barua
Samuel Peana
Arya Deepak Keni
Vahagn Mkhitaryan
Vladimir M. Shalaev
Yong P. Chen
Alexandra Boltasseva
Hadiseh Alaeian
Bottom-up fabrication of 2D Rydberg exciton arrays in cuprous oxide
Communications Materials
title Bottom-up fabrication of 2D Rydberg exciton arrays in cuprous oxide
title_full Bottom-up fabrication of 2D Rydberg exciton arrays in cuprous oxide
title_fullStr Bottom-up fabrication of 2D Rydberg exciton arrays in cuprous oxide
title_full_unstemmed Bottom-up fabrication of 2D Rydberg exciton arrays in cuprous oxide
title_short Bottom-up fabrication of 2D Rydberg exciton arrays in cuprous oxide
title_sort bottom up fabrication of 2d rydberg exciton arrays in cuprous oxide
url https://doi.org/10.1038/s43246-025-00742-1
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