Facile Low-Temperature Synthesis of Carbon Nanotube/ Nanohybrids with Enhanced Visible-Light-Driven Photocatalytic Activity

We demonstrate a facile and novel chemical precipitation strategy for the accurate coating of TiO2 nanoparticles on the surface of carbon nanotubes (CNTs) to form CNT/TiO2 nanohybrids, which only requires titanium sulfate and CNTs as starting materials and reacts in the alkaline solution at 60°C for...

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Main Authors: Yunlong Xie, Huanhuan Qian, Yijun Zhong, Hangming Guo, Yong Hu
Format: Article
Language:English
Published: Wiley 2012-01-01
Series:International Journal of Photoenergy
Online Access:http://dx.doi.org/10.1155/2012/682138
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author Yunlong Xie
Huanhuan Qian
Yijun Zhong
Hangming Guo
Yong Hu
author_facet Yunlong Xie
Huanhuan Qian
Yijun Zhong
Hangming Guo
Yong Hu
author_sort Yunlong Xie
collection DOAJ
description We demonstrate a facile and novel chemical precipitation strategy for the accurate coating of TiO2 nanoparticles on the surface of carbon nanotubes (CNTs) to form CNT/TiO2 nanohybrids, which only requires titanium sulfate and CNTs as starting materials and reacts in the alkaline solution at 60°C for 6 h. Using this process, the as-prepared hybrid structures preserved the good dispersity and uniformity of initial CNTs. Furthermore, the CNT/TiO2 nanohybrids show a broad blue luminescence at 469 nm and exhibit significantly enhanced photocatalytic activity for the degradation of rhodamine B (RhB) under visible-light irradiation, which is about 1.5 times greater than that of commercial Degussa P25 TiO2 nanoparticles. It is believed that this facile chemical precipitation strategy is scalable and its application can be extended to synthesize other CNT/oxide nanohybrids for various applications.
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institution Kabale University
issn 1110-662X
1687-529X
language English
publishDate 2012-01-01
publisher Wiley
record_format Article
series International Journal of Photoenergy
spelling doaj-art-82eafa57d99d423eba15a087187fe4d32025-02-03T05:58:33ZengWileyInternational Journal of Photoenergy1110-662X1687-529X2012-01-01201210.1155/2012/682138682138Facile Low-Temperature Synthesis of Carbon Nanotube/ Nanohybrids with Enhanced Visible-Light-Driven Photocatalytic ActivityYunlong Xie0Huanhuan Qian1Yijun Zhong2Hangming Guo3Yong Hu4Institute of Physical Chemistry, Zhejiang Normal University, Jinhua 321004, ChinaInstitute of Physical Chemistry, Zhejiang Normal University, Jinhua 321004, ChinaInstitute of Physical Chemistry, Zhejiang Normal University, Jinhua 321004, ChinaDepartment of Chemistry, Jinhua College of Vocation and Technology, Jinhua 321007, ChinaInstitute of Physical Chemistry, Zhejiang Normal University, Jinhua 321004, ChinaWe demonstrate a facile and novel chemical precipitation strategy for the accurate coating of TiO2 nanoparticles on the surface of carbon nanotubes (CNTs) to form CNT/TiO2 nanohybrids, which only requires titanium sulfate and CNTs as starting materials and reacts in the alkaline solution at 60°C for 6 h. Using this process, the as-prepared hybrid structures preserved the good dispersity and uniformity of initial CNTs. Furthermore, the CNT/TiO2 nanohybrids show a broad blue luminescence at 469 nm and exhibit significantly enhanced photocatalytic activity for the degradation of rhodamine B (RhB) under visible-light irradiation, which is about 1.5 times greater than that of commercial Degussa P25 TiO2 nanoparticles. It is believed that this facile chemical precipitation strategy is scalable and its application can be extended to synthesize other CNT/oxide nanohybrids for various applications.http://dx.doi.org/10.1155/2012/682138
spellingShingle Yunlong Xie
Huanhuan Qian
Yijun Zhong
Hangming Guo
Yong Hu
Facile Low-Temperature Synthesis of Carbon Nanotube/ Nanohybrids with Enhanced Visible-Light-Driven Photocatalytic Activity
International Journal of Photoenergy
title Facile Low-Temperature Synthesis of Carbon Nanotube/ Nanohybrids with Enhanced Visible-Light-Driven Photocatalytic Activity
title_full Facile Low-Temperature Synthesis of Carbon Nanotube/ Nanohybrids with Enhanced Visible-Light-Driven Photocatalytic Activity
title_fullStr Facile Low-Temperature Synthesis of Carbon Nanotube/ Nanohybrids with Enhanced Visible-Light-Driven Photocatalytic Activity
title_full_unstemmed Facile Low-Temperature Synthesis of Carbon Nanotube/ Nanohybrids with Enhanced Visible-Light-Driven Photocatalytic Activity
title_short Facile Low-Temperature Synthesis of Carbon Nanotube/ Nanohybrids with Enhanced Visible-Light-Driven Photocatalytic Activity
title_sort facile low temperature synthesis of carbon nanotube nanohybrids with enhanced visible light driven photocatalytic activity
url http://dx.doi.org/10.1155/2012/682138
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AT yijunzhong facilelowtemperaturesynthesisofcarbonnanotubenanohybridswithenhancedvisiblelightdrivenphotocatalyticactivity
AT hangmingguo facilelowtemperaturesynthesisofcarbonnanotubenanohybridswithenhancedvisiblelightdrivenphotocatalyticactivity
AT yonghu facilelowtemperaturesynthesisofcarbonnanotubenanohybridswithenhancedvisiblelightdrivenphotocatalyticactivity