Generation of Massively Entangled Bright States of Light during Harmonic Generation in Resonant Media

At the fundamental level, full description of light-matter interaction requires quantum treatment of both matter and light. However, for standard light sources generating intense laser pulses carrying quadrillions of photons in a coherent state, the classical description of light during intense lase...

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Main Authors: Sili Yi, Nikolai D. Klimkin, Graham Gardiner Brown, Olga Smirnova, Serguei Patchkovskii, Ihar Babushkin, Misha Ivanov
Format: Article
Language:English
Published: American Physical Society 2025-02-01
Series:Physical Review X
Online Access:http://doi.org/10.1103/PhysRevX.15.011023
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author Sili Yi
Nikolai D. Klimkin
Graham Gardiner Brown
Olga Smirnova
Serguei Patchkovskii
Ihar Babushkin
Misha Ivanov
author_facet Sili Yi
Nikolai D. Klimkin
Graham Gardiner Brown
Olga Smirnova
Serguei Patchkovskii
Ihar Babushkin
Misha Ivanov
author_sort Sili Yi
collection DOAJ
description At the fundamental level, full description of light-matter interaction requires quantum treatment of both matter and light. However, for standard light sources generating intense laser pulses carrying quadrillions of photons in a coherent state, the classical description of light during intense laser-matter interaction has been expected to be adequate. Here, we show how nonlinear optical response of matter can be controlled to generate dramatic deviations from this standard picture, including generation of several squeezed and entangled harmonics of the incident laser light. In particular, such nontrivial quantum states of harmonics are generated as soon as one of the harmonics induces a transition between different laser-dressed states of the material system. Such transitions generate an entangled light-matter wave function, which can generate quantum states of harmonics even in the absence of a quantum driving field or material correlations. In turn, entanglement of the material system with a single harmonic generates and controls entanglement between different harmonics. Hence, nonlinear media that are near resonant with at least one of the harmonics appear to be quite attractive for controlled generation of massively entangled quantum states of light. Our analysis opens remarkable opportunities at the interface of attosecond physics and quantum optics, with implications for quantum information science.
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institution Kabale University
issn 2160-3308
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publisher American Physical Society
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series Physical Review X
spelling doaj-art-74e33e71020448419c671635bc4d0b502025-02-05T16:18:09ZengAmerican Physical SocietyPhysical Review X2160-33082025-02-0115101102310.1103/PhysRevX.15.011023Generation of Massively Entangled Bright States of Light during Harmonic Generation in Resonant MediaSili YiNikolai D. KlimkinGraham Gardiner BrownOlga SmirnovaSerguei PatchkovskiiIhar BabushkinMisha IvanovAt the fundamental level, full description of light-matter interaction requires quantum treatment of both matter and light. However, for standard light sources generating intense laser pulses carrying quadrillions of photons in a coherent state, the classical description of light during intense laser-matter interaction has been expected to be adequate. Here, we show how nonlinear optical response of matter can be controlled to generate dramatic deviations from this standard picture, including generation of several squeezed and entangled harmonics of the incident laser light. In particular, such nontrivial quantum states of harmonics are generated as soon as one of the harmonics induces a transition between different laser-dressed states of the material system. Such transitions generate an entangled light-matter wave function, which can generate quantum states of harmonics even in the absence of a quantum driving field or material correlations. In turn, entanglement of the material system with a single harmonic generates and controls entanglement between different harmonics. Hence, nonlinear media that are near resonant with at least one of the harmonics appear to be quite attractive for controlled generation of massively entangled quantum states of light. Our analysis opens remarkable opportunities at the interface of attosecond physics and quantum optics, with implications for quantum information science.http://doi.org/10.1103/PhysRevX.15.011023
spellingShingle Sili Yi
Nikolai D. Klimkin
Graham Gardiner Brown
Olga Smirnova
Serguei Patchkovskii
Ihar Babushkin
Misha Ivanov
Generation of Massively Entangled Bright States of Light during Harmonic Generation in Resonant Media
Physical Review X
title Generation of Massively Entangled Bright States of Light during Harmonic Generation in Resonant Media
title_full Generation of Massively Entangled Bright States of Light during Harmonic Generation in Resonant Media
title_fullStr Generation of Massively Entangled Bright States of Light during Harmonic Generation in Resonant Media
title_full_unstemmed Generation of Massively Entangled Bright States of Light during Harmonic Generation in Resonant Media
title_short Generation of Massively Entangled Bright States of Light during Harmonic Generation in Resonant Media
title_sort generation of massively entangled bright states of light during harmonic generation in resonant media
url http://doi.org/10.1103/PhysRevX.15.011023
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