Magnetically tailored dielectric behaviour of (1-x)Ba0.98Sm0.02TiO3-xBa0.7Sr0.3Fe12O19 ceramic composites

With the growing need for materials for multifunctional devices, we are studying the behaviour of a composite consisting of titanate ferroelectric phase with strong dielectric properties and ferrites with magnetic properties. Solid-state reaction method was used to prepare Ba1-xSmxTiO3 powders, whil...

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Main Authors: Kaur Arshdeep, Nindrayog Amritpal Singh, Masih Sajan, Middha Shiffali, Kaur Shubhpreet, Kumar Sunil, Ghosh Rubina, Vishwakarma Prakash Nath, Arya Nisharika, Singh Satvir, Tandon Nitin, Sharma Indu, Arora ishal, Paul Surinder, Singh Mandeep, Chopra Vibha, Singh Anupinder
Format: Article
Language:English
Published: University of Novi Sad 2024-12-01
Series:Processing and Application of Ceramics
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Online Access:https://doiserbia.nb.rs/img/doi/1820-6131/2024/1820-61312404348K.pdf
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Summary:With the growing need for materials for multifunctional devices, we are studying the behaviour of a composite consisting of titanate ferroelectric phase with strong dielectric properties and ferrites with magnetic properties. Solid-state reaction method was used to prepare Ba1-xSmxTiO3 powders, while Ba1-xSrxFe12O19 powders were synthesized by sol-gel auto combustion method. The selected titanate and M-type hexaferrite powders were used for fabrication of (1-x)Ba0.98Sm0.02TiO3-xBa0.7Sr0.3Fe12O19 composites (x = 0.1, 0.2, 0.3, 0.4, and 0.5) by their mixing, compaction and sintering at 1240°C. Phase formation was investigated by XRD and multivalent state of Fe (Fe2+ and Fe3+) was identified from XPS. Matching the unique properties of these materials with each other will favour numerous application paths. The magnetic, magneto-dielectric and magnetoelectric properties of perovskite/hexaferrite composites were investigated. Magnetoelectric coupling was found in all of the composite samples by the magneto-dielectric investigation. The maximum magneto-dielectric response of ∼37.7% in terms of change in dielectric permittivity in presence of magnetic field was measured for the sample with x = 0.4 at magnetic field of 1.2 T and frequency of 100Hz.
ISSN:1820-6131
2406-1034