Additive manufacturing of thermoset elastomers: A review of emerging technologies

Thermoset elastomers (TSEs) are widely used in industries such as automotive, household appliances, healthcare, and fashion due to their flexibility and stability. However, these same properties make TSEs challenging to process using additive manufacturing (AM) techniques. This review categorizes AM...

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Main Authors: Csenge Tóth, Ábris Dávid Virág, István Halász-Kutasi, Norbert Krisztián Kovács, Tamás Bárány
Format: Article
Language:English
Published: Elsevier 2025-09-01
Series:Engineering Science and Technology, an International Journal
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Online Access:http://www.sciencedirect.com/science/article/pii/S2215098625001983
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author Csenge Tóth
Ábris Dávid Virág
István Halász-Kutasi
Norbert Krisztián Kovács
Tamás Bárány
author_facet Csenge Tóth
Ábris Dávid Virág
István Halász-Kutasi
Norbert Krisztián Kovács
Tamás Bárány
author_sort Csenge Tóth
collection DOAJ
description Thermoset elastomers (TSEs) are widely used in industries such as automotive, household appliances, healthcare, and fashion due to their flexibility and stability. However, these same properties make TSEs challenging to process using additive manufacturing (AM) techniques. This review categorizes AM technologies for producing TSEs into three main groups: photopolymerization-based, two-phase, and material extrusion–based techniques. Photopolymerization offers high resolution and material versatility but is constrained by build size and environmental impacts. Two-phase systems enable tunable properties but suffer from rheological and bonding issues, while material extrusion is more cost-effective yet less precise. Overall, current research primarily concentrates on technology and formulation development. Mechanical characterization of 3D-printed TSEs is typically limited to tensile properties. Comprehensive mechanical testing, including application-specific properties, is still rare and remains an essential area for future qualification of technological advances. The sustainability aspects of 3D printing TSEs are also addressed, with a focus on environmentally friendly raw material selection and the general environmental considerations of 3D printing methods. Emerging trends in this field include the development of smart materials, sustainable solutions, and integrated hybrid methods that incorporate artificial intelligence and machine learning.
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spelling doaj-art-5b3e2cf46dce4dbda685f113b1eeba2e2025-08-20T03:08:33ZengElsevierEngineering Science and Technology, an International Journal2215-09862025-09-016910214310.1016/j.jestch.2025.102143Additive manufacturing of thermoset elastomers: A review of emerging technologiesCsenge Tóth0Ábris Dávid Virág1István Halász-Kutasi2Norbert Krisztián Kovács3Tamás Bárány4Department of Polymer Engineering, Faculty of Mechanical Engineering, Budapest University of Technology and Economics, Műegyetem rkp. 3., H-1111 Budapest, Hungary; MTA-BME Lendület Lightweight Polymer Composites Research Group, Műegyetem rkp. 3., H-1111 Budapest, HungaryDepartment of Polymer Engineering, Faculty of Mechanical Engineering, Budapest University of Technology and Economics, Műegyetem rkp. 3., H-1111 Budapest, Hungary; Corresponding author.Department of Polymer Engineering, Faculty of Mechanical Engineering, Budapest University of Technology and Economics, Műegyetem rkp. 3., H-1111 Budapest, HungaryDepartment of Polymer Engineering, Faculty of Mechanical Engineering, Budapest University of Technology and Economics, Műegyetem rkp. 3., H-1111 Budapest, Hungary; MTA-BME Lendület Lightweight Polymer Composites Research Group, Műegyetem rkp. 3., H-1111 Budapest, HungaryDepartment of Polymer Engineering, Faculty of Mechanical Engineering, Budapest University of Technology and Economics, Műegyetem rkp. 3., H-1111 Budapest, Hungary; MTA-BME Lendület Lightweight Polymer Composites Research Group, Műegyetem rkp. 3., H-1111 Budapest, HungaryThermoset elastomers (TSEs) are widely used in industries such as automotive, household appliances, healthcare, and fashion due to their flexibility and stability. However, these same properties make TSEs challenging to process using additive manufacturing (AM) techniques. This review categorizes AM technologies for producing TSEs into three main groups: photopolymerization-based, two-phase, and material extrusion–based techniques. Photopolymerization offers high resolution and material versatility but is constrained by build size and environmental impacts. Two-phase systems enable tunable properties but suffer from rheological and bonding issues, while material extrusion is more cost-effective yet less precise. Overall, current research primarily concentrates on technology and formulation development. Mechanical characterization of 3D-printed TSEs is typically limited to tensile properties. Comprehensive mechanical testing, including application-specific properties, is still rare and remains an essential area for future qualification of technological advances. The sustainability aspects of 3D printing TSEs are also addressed, with a focus on environmentally friendly raw material selection and the general environmental considerations of 3D printing methods. Emerging trends in this field include the development of smart materials, sustainable solutions, and integrated hybrid methods that incorporate artificial intelligence and machine learning.http://www.sciencedirect.com/science/article/pii/S22150986250019833D printingRubberRapid prototypingCrosslinkPhotopolymerizationSustainability
spellingShingle Csenge Tóth
Ábris Dávid Virág
István Halász-Kutasi
Norbert Krisztián Kovács
Tamás Bárány
Additive manufacturing of thermoset elastomers: A review of emerging technologies
Engineering Science and Technology, an International Journal
3D printing
Rubber
Rapid prototyping
Crosslink
Photopolymerization
Sustainability
title Additive manufacturing of thermoset elastomers: A review of emerging technologies
title_full Additive manufacturing of thermoset elastomers: A review of emerging technologies
title_fullStr Additive manufacturing of thermoset elastomers: A review of emerging technologies
title_full_unstemmed Additive manufacturing of thermoset elastomers: A review of emerging technologies
title_short Additive manufacturing of thermoset elastomers: A review of emerging technologies
title_sort additive manufacturing of thermoset elastomers a review of emerging technologies
topic 3D printing
Rubber
Rapid prototyping
Crosslink
Photopolymerization
Sustainability
url http://www.sciencedirect.com/science/article/pii/S2215098625001983
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