A Facile and Waste-Free Strategy to Fabricate Pt-C/TiO2 Microspheres: Enhanced Photocatalytic Performance for Hydrogen Evolution
A facile and waste-free flame thermal synthesis method was developed for preparing Pt modified C/TiO2 microspheres (Pt-C/TiO2). The photocatalysts were characterized with X-ray diffraction, field emission scanning electron microscopy, transmission electron microscope, ultraviolet-visible (UV-vis) di...
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Main Authors: | , , |
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Format: | Article |
Language: | English |
Published: |
Wiley
2014-01-01
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Series: | International Journal of Photoenergy |
Online Access: | http://dx.doi.org/10.1155/2014/414281 |
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Summary: | A facile and waste-free flame thermal synthesis method was developed for preparing Pt modified C/TiO2 microspheres (Pt-C/TiO2). The photocatalysts were characterized with X-ray diffraction, field emission scanning electron microscopy, transmission electron microscope, ultraviolet-visible (UV-vis) diffuse reflectance spectra, X-ray photoelectron spectroscopy, and thermogravimetry analysis. The photocatalytic activity was evaluated by hydrogen evolution from water splitting under UV-vis light illumination. Benefitting from the electron-hole separation behavior and reduced overpotential of H+/H2, remarkably enhanced hydrogen production was demonstrated and the photocatalytic hydrogen generation from 0.4 wt% Pt-C/TiO2 increased by 22 times. This study also demonstrates that the novel and facile method is highly attractive, due to its easy operation, requiring no post treatment and energy-saving features. |
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ISSN: | 1110-662X 1687-529X |