Photocatalytic Activity of Ti-SBA-15/C3N4 for Degradation of 2,4-Dichlorophenoxyacetic Acid in Water under Visible Light
In the present study, the photocatalytic activity of Ti-SBA-15/C3N4 catalysts was investigated to degrade 2,4-Dichlorophenoxyacetic acid (2,4-D) herbicides in water under visible light irradiation. The catalysts were synthesized via a simple hydrothermal method and characterized by various analytica...
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2022-01-01
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Series: | Journal of Analytical Methods in Chemistry |
Online Access: | http://dx.doi.org/10.1155/2022/5531219 |
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author | Hoa T. T. Duong Mai T. P. Duong Oanh K. Nguyen Son T. Le Long V. Dang Binh T. Nguyen Dang V. Do |
author_facet | Hoa T. T. Duong Mai T. P. Duong Oanh K. Nguyen Son T. Le Long V. Dang Binh T. Nguyen Dang V. Do |
author_sort | Hoa T. T. Duong |
collection | DOAJ |
description | In the present study, the photocatalytic activity of Ti-SBA-15/C3N4 catalysts was investigated to degrade 2,4-Dichlorophenoxyacetic acid (2,4-D) herbicides in water under visible light irradiation. The catalysts were synthesized via a simple hydrothermal method and characterized by various analytical techniques, including SAXS, N2 adsorption-desorption isotherms, Zeta potential, PL, FT-IR, XRF, TGA, and UV-DRS. Our study indicated that the 2.5Ti-SBA-15/C3N4 had higher efficiency in the degradation of 2,4-D than Ti-SBA-15 and C3N4. The decomposition of 2,4-D reached 60% under 180 minutes of visible light irradiation at room temperature on 2.5Ti-SBA-15/C3N4. Moreover, the degradation of 2,4-D on Ti-SBA-15/C3N4 was pseudo-first-order kinetics with the highest rate constant (0.00484 min−1), which was much higher than that obtained for other photocatalysts reported recently. Furthermore, the catalyst can be reused at least two times for photodegradation of 2,4-D solution under visible light irradiation within a slight decrease in catalytic activity. |
format | Article |
id | doaj-art-541e4f4e06cd4b558b6a1d706db865b3 |
institution | Kabale University |
issn | 2090-8873 |
language | English |
publishDate | 2022-01-01 |
publisher | Wiley |
record_format | Article |
series | Journal of Analytical Methods in Chemistry |
spelling | doaj-art-541e4f4e06cd4b558b6a1d706db865b32025-02-03T06:05:55ZengWileyJournal of Analytical Methods in Chemistry2090-88732022-01-01202210.1155/2022/5531219Photocatalytic Activity of Ti-SBA-15/C3N4 for Degradation of 2,4-Dichlorophenoxyacetic Acid in Water under Visible LightHoa T. T. Duong0Mai T. P. Duong1Oanh K. Nguyen2Son T. Le3Long V. Dang4Binh T. Nguyen5Dang V. Do6Faculty of ChemistryFaculty of ChemistryFaculty of ChemistryFaculty of ChemistryFaculty of ChemistryFaculty of ChemistryFaculty of ChemistryIn the present study, the photocatalytic activity of Ti-SBA-15/C3N4 catalysts was investigated to degrade 2,4-Dichlorophenoxyacetic acid (2,4-D) herbicides in water under visible light irradiation. The catalysts were synthesized via a simple hydrothermal method and characterized by various analytical techniques, including SAXS, N2 adsorption-desorption isotherms, Zeta potential, PL, FT-IR, XRF, TGA, and UV-DRS. Our study indicated that the 2.5Ti-SBA-15/C3N4 had higher efficiency in the degradation of 2,4-D than Ti-SBA-15 and C3N4. The decomposition of 2,4-D reached 60% under 180 minutes of visible light irradiation at room temperature on 2.5Ti-SBA-15/C3N4. Moreover, the degradation of 2,4-D on Ti-SBA-15/C3N4 was pseudo-first-order kinetics with the highest rate constant (0.00484 min−1), which was much higher than that obtained for other photocatalysts reported recently. Furthermore, the catalyst can be reused at least two times for photodegradation of 2,4-D solution under visible light irradiation within a slight decrease in catalytic activity.http://dx.doi.org/10.1155/2022/5531219 |
spellingShingle | Hoa T. T. Duong Mai T. P. Duong Oanh K. Nguyen Son T. Le Long V. Dang Binh T. Nguyen Dang V. Do Photocatalytic Activity of Ti-SBA-15/C3N4 for Degradation of 2,4-Dichlorophenoxyacetic Acid in Water under Visible Light Journal of Analytical Methods in Chemistry |
title | Photocatalytic Activity of Ti-SBA-15/C3N4 for Degradation of 2,4-Dichlorophenoxyacetic Acid in Water under Visible Light |
title_full | Photocatalytic Activity of Ti-SBA-15/C3N4 for Degradation of 2,4-Dichlorophenoxyacetic Acid in Water under Visible Light |
title_fullStr | Photocatalytic Activity of Ti-SBA-15/C3N4 for Degradation of 2,4-Dichlorophenoxyacetic Acid in Water under Visible Light |
title_full_unstemmed | Photocatalytic Activity of Ti-SBA-15/C3N4 for Degradation of 2,4-Dichlorophenoxyacetic Acid in Water under Visible Light |
title_short | Photocatalytic Activity of Ti-SBA-15/C3N4 for Degradation of 2,4-Dichlorophenoxyacetic Acid in Water under Visible Light |
title_sort | photocatalytic activity of ti sba 15 c3n4 for degradation of 2 4 dichlorophenoxyacetic acid in water under visible light |
url | http://dx.doi.org/10.1155/2022/5531219 |
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