High-Harmonic Generation in an Optical Fiber Functionalized with Zinc Oxide Thin Films

High-order harmonic generation (HHG) in semiconductor thin films from ultrashort mid-infrared laser drivers holds the potential for the realization of integrated sources of extreme ultraviolet light. Here, we demonstrate solid-state HHG in zinc oxide thin films synthesized by the radiofrequency reac...

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Main Authors: Idris Tiliouine, Yann Leventoux, Jean-Christophe Orlianges, Aurelian Crunteanu, Marie Froidevaux, Hamed Merdji, Sébastien Février
Format: Article
Language:English
Published: MDPI AG 2025-01-01
Series:Photonics
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Online Access:https://www.mdpi.com/2304-6732/12/1/82
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author Idris Tiliouine
Yann Leventoux
Jean-Christophe Orlianges
Aurelian Crunteanu
Marie Froidevaux
Hamed Merdji
Sébastien Février
author_facet Idris Tiliouine
Yann Leventoux
Jean-Christophe Orlianges
Aurelian Crunteanu
Marie Froidevaux
Hamed Merdji
Sébastien Février
author_sort Idris Tiliouine
collection DOAJ
description High-order harmonic generation (HHG) in semiconductor thin films from ultrashort mid-infrared laser drivers holds the potential for the realization of integrated sources of extreme ultraviolet light. Here, we demonstrate solid-state HHG in zinc oxide thin films synthesized by the radiofrequency reactive magnetron sputtering process directly on the cleaved facets of optical fibers. Harmonics 3 to 13 of the radiation from a fiber-based laser system delivering 500 kW, 96 fs pulses at 3130 nm are produced in the thin film and guided along the fiber. A proper choice of the laser wavelength and fiber material allows for filtering out the mid-IR pump laser and achieving the HHG mode selection. The possibility to nanostructure the fiber exit by, e.g., focused ion beam milling paves the way to an increased control over the HHG spatial mode.
format Article
id doaj-art-4ed7c9fba55540628f7fc87c10417785
institution Kabale University
issn 2304-6732
language English
publishDate 2025-01-01
publisher MDPI AG
record_format Article
series Photonics
spelling doaj-art-4ed7c9fba55540628f7fc87c104177852025-01-24T13:46:27ZengMDPI AGPhotonics2304-67322025-01-011218210.3390/photonics12010082High-Harmonic Generation in an Optical Fiber Functionalized with Zinc Oxide Thin FilmsIdris Tiliouine0Yann Leventoux1Jean-Christophe Orlianges2Aurelian Crunteanu3Marie Froidevaux4Hamed Merdji5Sébastien Février6XLIM UMR CNRS 7252, Université de Limoges, 87060 Limoges, FranceXLIM UMR CNRS 7252, Université de Limoges, 87060 Limoges, FranceXLIM UMR CNRS 7252, Université de Limoges, 87060 Limoges, FranceXLIM UMR CNRS 7252, Université de Limoges, 87060 Limoges, FranceLaboratoire d’Optique Appliquée, ENSTA ParisTech, CNRS, Ecole Polytechnique, 91120 Palaiseau, FranceLaboratoire d’Optique Appliquée, ENSTA ParisTech, CNRS, Ecole Polytechnique, 91120 Palaiseau, FranceXLIM UMR CNRS 7252, Université de Limoges, 87060 Limoges, FranceHigh-order harmonic generation (HHG) in semiconductor thin films from ultrashort mid-infrared laser drivers holds the potential for the realization of integrated sources of extreme ultraviolet light. Here, we demonstrate solid-state HHG in zinc oxide thin films synthesized by the radiofrequency reactive magnetron sputtering process directly on the cleaved facets of optical fibers. Harmonics 3 to 13 of the radiation from a fiber-based laser system delivering 500 kW, 96 fs pulses at 3130 nm are produced in the thin film and guided along the fiber. A proper choice of the laser wavelength and fiber material allows for filtering out the mid-IR pump laser and achieving the HHG mode selection. The possibility to nanostructure the fiber exit by, e.g., focused ion beam milling paves the way to an increased control over the HHG spatial mode.https://www.mdpi.com/2304-6732/12/1/82high-order harmonic generationfiber lasersmid-infrared
spellingShingle Idris Tiliouine
Yann Leventoux
Jean-Christophe Orlianges
Aurelian Crunteanu
Marie Froidevaux
Hamed Merdji
Sébastien Février
High-Harmonic Generation in an Optical Fiber Functionalized with Zinc Oxide Thin Films
Photonics
high-order harmonic generation
fiber lasers
mid-infrared
title High-Harmonic Generation in an Optical Fiber Functionalized with Zinc Oxide Thin Films
title_full High-Harmonic Generation in an Optical Fiber Functionalized with Zinc Oxide Thin Films
title_fullStr High-Harmonic Generation in an Optical Fiber Functionalized with Zinc Oxide Thin Films
title_full_unstemmed High-Harmonic Generation in an Optical Fiber Functionalized with Zinc Oxide Thin Films
title_short High-Harmonic Generation in an Optical Fiber Functionalized with Zinc Oxide Thin Films
title_sort high harmonic generation in an optical fiber functionalized with zinc oxide thin films
topic high-order harmonic generation
fiber lasers
mid-infrared
url https://www.mdpi.com/2304-6732/12/1/82
work_keys_str_mv AT idristiliouine highharmonicgenerationinanopticalfiberfunctionalizedwithzincoxidethinfilms
AT yannleventoux highharmonicgenerationinanopticalfiberfunctionalizedwithzincoxidethinfilms
AT jeanchristopheorlianges highharmonicgenerationinanopticalfiberfunctionalizedwithzincoxidethinfilms
AT aureliancrunteanu highharmonicgenerationinanopticalfiberfunctionalizedwithzincoxidethinfilms
AT mariefroidevaux highharmonicgenerationinanopticalfiberfunctionalizedwithzincoxidethinfilms
AT hamedmerdji highharmonicgenerationinanopticalfiberfunctionalizedwithzincoxidethinfilms
AT sebastienfevrier highharmonicgenerationinanopticalfiberfunctionalizedwithzincoxidethinfilms