Hydrometallurgical Method for AgCu Alloy Powder Synthesis and Its Application in Pd(II) Recovery Through Cementation

This study investigates the synthesis, characterization, and potential applications of silver–copper (AgCu) alloy powders produced from co-precipitated carbonates. The Cu/Ag carbonate samples were analyzed using EDXRF, TGA-DSC, XRD, SEM, and electrical conductivity tests to examine their composition...

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Main Authors: Tomasz Michałek, Konrad Wojtaszek, Stanisław Małecki, Marek Wojnicki
Format: Article
Language:English
Published: MDPI AG 2024-12-01
Series:Metals
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Online Access:https://www.mdpi.com/2075-4701/14/12/1450
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author Tomasz Michałek
Konrad Wojtaszek
Stanisław Małecki
Marek Wojnicki
author_facet Tomasz Michałek
Konrad Wojtaszek
Stanisław Małecki
Marek Wojnicki
author_sort Tomasz Michałek
collection DOAJ
description This study investigates the synthesis, characterization, and potential applications of silver–copper (AgCu) alloy powders produced from co-precipitated carbonates. The Cu/Ag carbonate samples were analyzed using EDXRF, TGA-DSC, XRD, SEM, and electrical conductivity tests to examine their composition, thermal behavior, structure, and morphology. The results showed slight deviations from the theoretical Cu/Ag ratios in the carbonates, attributed to equilibrium effects during precipitation. Thermal analysis indicated that the reduction process of carbonates with hydrogen was completed at 300 °C, while alloy formation was confirmed by endothermic peaks around 780 °C. XRD and SEM analyses revealed that AgCu alloys formed a solid solution, with smaller crystallite sizes observed at higher Cu contents. Electrical conductivity tests demonstrated that while pure Ag and Cu powders exhibited conductivity increases with compaction, the AgCu alloy showed stable conductivity without a significant decrease. In Pd(II) cementation experiments, AgCu alloys demonstrated higher efficiency in Pd(II) recovery than pure Ag and Cu. These findings suggest that AgCu alloys, particularly with a balanced composition, may offer improved performance for metal recovery applications, providing a promising approach for industrial cementation processes.
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spelling doaj-art-3d8f1331e48c40a68a23f89ba1bc46d02025-08-20T02:56:50ZengMDPI AGMetals2075-47012024-12-011412145010.3390/met14121450Hydrometallurgical Method for AgCu Alloy Powder Synthesis and Its Application in Pd(II) Recovery Through CementationTomasz Michałek0Konrad Wojtaszek1Stanisław Małecki2Marek Wojnicki3Faculty of Non-Ferrous Metals, AGH University of Krakow, al. A. Mickiewicza 30, 30-059 Kraków, PolandFaculty of Non-Ferrous Metals, AGH University of Krakow, al. A. Mickiewicza 30, 30-059 Kraków, PolandFaculty of Non-Ferrous Metals, AGH University of Krakow, al. A. Mickiewicza 30, 30-059 Kraków, PolandFaculty of Non-Ferrous Metals, AGH University of Krakow, al. A. Mickiewicza 30, 30-059 Kraków, PolandThis study investigates the synthesis, characterization, and potential applications of silver–copper (AgCu) alloy powders produced from co-precipitated carbonates. The Cu/Ag carbonate samples were analyzed using EDXRF, TGA-DSC, XRD, SEM, and electrical conductivity tests to examine their composition, thermal behavior, structure, and morphology. The results showed slight deviations from the theoretical Cu/Ag ratios in the carbonates, attributed to equilibrium effects during precipitation. Thermal analysis indicated that the reduction process of carbonates with hydrogen was completed at 300 °C, while alloy formation was confirmed by endothermic peaks around 780 °C. XRD and SEM analyses revealed that AgCu alloys formed a solid solution, with smaller crystallite sizes observed at higher Cu contents. Electrical conductivity tests demonstrated that while pure Ag and Cu powders exhibited conductivity increases with compaction, the AgCu alloy showed stable conductivity without a significant decrease. In Pd(II) cementation experiments, AgCu alloys demonstrated higher efficiency in Pd(II) recovery than pure Ag and Cu. These findings suggest that AgCu alloys, particularly with a balanced composition, may offer improved performance for metal recovery applications, providing a promising approach for industrial cementation processes.https://www.mdpi.com/2075-4701/14/12/1450coppersilveralloypalladiumcementation
spellingShingle Tomasz Michałek
Konrad Wojtaszek
Stanisław Małecki
Marek Wojnicki
Hydrometallurgical Method for AgCu Alloy Powder Synthesis and Its Application in Pd(II) Recovery Through Cementation
Metals
copper
silver
alloy
palladium
cementation
title Hydrometallurgical Method for AgCu Alloy Powder Synthesis and Its Application in Pd(II) Recovery Through Cementation
title_full Hydrometallurgical Method for AgCu Alloy Powder Synthesis and Its Application in Pd(II) Recovery Through Cementation
title_fullStr Hydrometallurgical Method for AgCu Alloy Powder Synthesis and Its Application in Pd(II) Recovery Through Cementation
title_full_unstemmed Hydrometallurgical Method for AgCu Alloy Powder Synthesis and Its Application in Pd(II) Recovery Through Cementation
title_short Hydrometallurgical Method for AgCu Alloy Powder Synthesis and Its Application in Pd(II) Recovery Through Cementation
title_sort hydrometallurgical method for agcu alloy powder synthesis and its application in pd ii recovery through cementation
topic copper
silver
alloy
palladium
cementation
url https://www.mdpi.com/2075-4701/14/12/1450
work_keys_str_mv AT tomaszmichałek hydrometallurgicalmethodforagcualloypowdersynthesisanditsapplicationinpdiirecoverythroughcementation
AT konradwojtaszek hydrometallurgicalmethodforagcualloypowdersynthesisanditsapplicationinpdiirecoverythroughcementation
AT stanisławmałecki hydrometallurgicalmethodforagcualloypowdersynthesisanditsapplicationinpdiirecoverythroughcementation
AT marekwojnicki hydrometallurgicalmethodforagcualloypowdersynthesisanditsapplicationinpdiirecoverythroughcementation