Carrier-envelope-phase characterization of ultrafast mid-infrared laser pulses through harmonic generation and interference in argon

Abstract The propagation of an intense, femtosecond, mid-infrared laser pulse in a gaseous medium results in the efficient generation of spectrally overlapping low-order harmonics, whose optical carrier phases are linked to the carrier-envelope phase (CEP) of the mid-infrared driver pulse. Random pe...

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Main Authors: Claudia Gollner, Valentina Shumakova, Jacob Barker, Audrius Pugžlys, Andrius Baltuška, Pavel Polynkin
Format: Article
Language:English
Published: Nature Portfolio 2025-01-01
Series:Communications Physics
Online Access:https://doi.org/10.1038/s42005-025-01949-x
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author Claudia Gollner
Valentina Shumakova
Jacob Barker
Audrius Pugžlys
Andrius Baltuška
Pavel Polynkin
author_facet Claudia Gollner
Valentina Shumakova
Jacob Barker
Audrius Pugžlys
Andrius Baltuška
Pavel Polynkin
author_sort Claudia Gollner
collection DOAJ
description Abstract The propagation of an intense, femtosecond, mid-infrared laser pulse in a gaseous medium results in the efficient generation of spectrally overlapping low-order harmonics, whose optical carrier phases are linked to the carrier-envelope phase (CEP) of the mid-infrared driver pulse. Random peak-power fluctuations of the driver pulses, converted to the fluctuations of the nonlinear phases, acquired by the pulses on propagation, cause this phase correlation to smear out. We show that this seemingly irreversible loss of phase can be recovered, and that the complete information needed for the phase correction is contained in the harmonic spectra itself. The optical phases of the intense driver pulse and its harmonics, as fragile as they appear to be against even weak disturbances, evolve deterministically during highly nonlinear propagation through the extended ionization region.
format Article
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institution Kabale University
issn 2399-3650
language English
publishDate 2025-01-01
publisher Nature Portfolio
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series Communications Physics
spelling doaj-art-2a8853530bfa408d9a2f62cae62d89a72025-01-26T12:37:02ZengNature PortfolioCommunications Physics2399-36502025-01-01811710.1038/s42005-025-01949-xCarrier-envelope-phase characterization of ultrafast mid-infrared laser pulses through harmonic generation and interference in argonClaudia Gollner0Valentina Shumakova1Jacob Barker2Audrius Pugžlys3Andrius Baltuška4Pavel Polynkin5Photonics Institute, Vienna University of TechnologyPhotonics Institute, Vienna University of TechnologyCollege of Optical Sciences, The University of ArizonaPhotonics Institute, Vienna University of TechnologyPhotonics Institute, Vienna University of TechnologyCollege of Optical Sciences, The University of ArizonaAbstract The propagation of an intense, femtosecond, mid-infrared laser pulse in a gaseous medium results in the efficient generation of spectrally overlapping low-order harmonics, whose optical carrier phases are linked to the carrier-envelope phase (CEP) of the mid-infrared driver pulse. Random peak-power fluctuations of the driver pulses, converted to the fluctuations of the nonlinear phases, acquired by the pulses on propagation, cause this phase correlation to smear out. We show that this seemingly irreversible loss of phase can be recovered, and that the complete information needed for the phase correction is contained in the harmonic spectra itself. The optical phases of the intense driver pulse and its harmonics, as fragile as they appear to be against even weak disturbances, evolve deterministically during highly nonlinear propagation through the extended ionization region.https://doi.org/10.1038/s42005-025-01949-x
spellingShingle Claudia Gollner
Valentina Shumakova
Jacob Barker
Audrius Pugžlys
Andrius Baltuška
Pavel Polynkin
Carrier-envelope-phase characterization of ultrafast mid-infrared laser pulses through harmonic generation and interference in argon
Communications Physics
title Carrier-envelope-phase characterization of ultrafast mid-infrared laser pulses through harmonic generation and interference in argon
title_full Carrier-envelope-phase characterization of ultrafast mid-infrared laser pulses through harmonic generation and interference in argon
title_fullStr Carrier-envelope-phase characterization of ultrafast mid-infrared laser pulses through harmonic generation and interference in argon
title_full_unstemmed Carrier-envelope-phase characterization of ultrafast mid-infrared laser pulses through harmonic generation and interference in argon
title_short Carrier-envelope-phase characterization of ultrafast mid-infrared laser pulses through harmonic generation and interference in argon
title_sort carrier envelope phase characterization of ultrafast mid infrared laser pulses through harmonic generation and interference in argon
url https://doi.org/10.1038/s42005-025-01949-x
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