Measurement report: Aircraft observations of aerosol and microphysical quantities of stratocumulus in autumn over Guangxi Province, China – daylight variation, vertical distribution, and aerosol–cloud interactions
<p>Aerosols and clouds play essential roles in the global climate system, and aerosol–cloud interactions have a significant impact on the radiation balance, water cycle, and energy cycle of the Earth–atmosphere system. To understand the effect of aerosols on the vertical distribution of strato...
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Copernicus Publications
2025-04-01
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| Series: | Atmospheric Chemistry and Physics |
| Online Access: | https://acp.copernicus.org/articles/25/4151/2025/acp-25-4151-2025.pdf |
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| author | S. Liu H. Wang D. Zhao D. Zhao W. Zhou Y. Du Z. Zhang P. Cheng T. Zhao Y. Ke Z. Wu M. Huang |
| author_facet | S. Liu H. Wang D. Zhao D. Zhao W. Zhou Y. Du Z. Zhang P. Cheng T. Zhao Y. Ke Z. Wu M. Huang |
| author_sort | S. Liu |
| collection | DOAJ |
| description | <p>Aerosols and clouds play essential roles in the global climate system, and aerosol–cloud interactions have a significant impact on the radiation balance, water cycle, and energy cycle of the Earth–atmosphere system. To understand the effect of aerosols on the vertical distribution of stratocumulus microphysical quantities in southwest China, we analyzed data from nine aircraft observations over Guangxi from 10 October to 3 November 2020. This analysis focused on the daylight variation characteristics and formation mechanisms of stratocumulus microphysical profiles, considering the influence of aerosol number concentration in relation to the source of air mass and individual cases. Aerosol number concentration (<span class="inline-formula"><i>N</i><sub>a</sub></span>) and cloud droplet concentration (<span class="inline-formula"><i>N</i><sub>c</sub></span>) decreased gradually with an altitude increase below 1500 m and did not change with a height between 1500 and 3300 m. The temperature inversion layer at the top of the planetary boundary layer (PBL) hindered the increase in the cloud droplet particle size. The lower layer of the stratocumulus cloud in Guangxi mainly contained small-sized cloud droplets (effective diameter of a cloud droplet (<span class="inline-formula"><i>E</i><sub>d</sub></span>) <span class="inline-formula"><</span> 15 <span class="inline-formula">µm</span>), and the middle and upper layers of cloud droplets were large-particle-size cloud droplets (<span class="inline-formula"><i>E</i><sub>d</sub></span> <span class="inline-formula">></span> 20 <span class="inline-formula">µm</span>). The vertical distribution of cloud microphysical quantity had apparent daylight variation. When aerosols in the PBL were transported to the upper air (14:00 to 20:00 Beijing time, BJT), <span class="inline-formula"><i>N</i><sub>c</sub></span> in the lower layer decreased, and the small-particle-size cloud droplets (<span class="inline-formula"><i>E</i><sub>d</sub></span> <span class="inline-formula"><</span> 20 <span class="inline-formula">µm</span>) in the middle layer and upper layer increased. Aerosols from the free atmosphere were transported into the PBL (10:00 to 13:00 BJT), providing an abundance of cloud condensation nuclei, which increased the number of small-particle-size cloud droplets in the lower layer of the cloud (near the top of the PBL). The characteristics of cloud microphysical quantities (<span class="inline-formula"><i>N</i><sub>c</sub></span> and <span class="inline-formula"><i>E</i><sub>d</sub></span>) were also affected by the source of air mass and the height of the PBL. <span class="inline-formula"><i>N</i><sub>a</sub></span> and <span class="inline-formula"><i>N</i><sub>c</sub></span> were high under the influence of land air mass or aerosols within the PBL, and the cloud droplet number concentration spectrum was unimodal. <span class="inline-formula"><i>N</i><sub>a</sub></span> and <span class="inline-formula"><i>N</i><sub>c</sub></span> were low under the influence of marine air mass or above the boundary layer, and the cloud droplet number concentration spectrum was bimodal. The relationship between stratocumulus and aerosol in this region is consistent with the Twomey effect. <span class="inline-formula"><i>E</i><sub>d</sub></span> and <span class="inline-formula"><i>N</i><sub>a</sub></span> remain negatively correlated in different liquid water content ranges, and the FIE (aerosol first indirect effect) ranged from <span class="inline-formula">−</span>0.07 to <span class="inline-formula">−</span>0.58.</p> |
| format | Article |
| id | doaj-art-29f571e728b143769db656f6e2ff2a3f |
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| issn | 1680-7316 1680-7324 |
| language | English |
| publishDate | 2025-04-01 |
| publisher | Copernicus Publications |
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| series | Atmospheric Chemistry and Physics |
| spelling | doaj-art-29f571e728b143769db656f6e2ff2a3f2025-08-20T02:09:27ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242025-04-01254151416510.5194/acp-25-4151-2025Measurement report: Aircraft observations of aerosol and microphysical quantities of stratocumulus in autumn over Guangxi Province, China – daylight variation, vertical distribution, and aerosol–cloud interactionsS. Liu0H. Wang1D. Zhao2D. Zhao3W. Zhou4Y. Du5Z. Zhang6P. Cheng7T. Zhao8Y. Ke9Z. Wu10M. Huang11China Meteorological Administration Aerosol-Cloud and Precipitation Key Laboratory, Nanjing University of Information Science and Technology, Nanjing 210044, ChinaChina Meteorological Administration Aerosol-Cloud and Precipitation Key Laboratory, Nanjing University of Information Science and Technology, Nanjing 210044, ChinaWeather Modification Center, China Meteorological Administration (CMA), Beijing 100081, ChinaField Experiment Base of Cloud and Precipitation Research in North China, China Meteorological Administration, Beijing 101200, ChinaBeijing Weather Modification Center, Beijing 100089, ChinaBeijing Weather Modification Center, Beijing 100089, ChinaWeather Modification Office of Guangxi Zhuang Autonomous Region, Nanning 530022, ChinaWeather Modification Office of Guangxi Zhuang Autonomous Region, Nanning 530022, ChinaChina Meteorological Administration Aerosol-Cloud and Precipitation Key Laboratory, Nanjing University of Information Science and Technology, Nanjing 210044, ChinaChina Meteorological Administration Aerosol-Cloud and Precipitation Key Laboratory, Nanjing University of Information Science and Technology, Nanjing 210044, ChinaChina Meteorological Administration Aerosol-Cloud and Precipitation Key Laboratory, Nanjing University of Information Science and Technology, Nanjing 210044, ChinaBeijing Weather Modification Center, Beijing 100089, China<p>Aerosols and clouds play essential roles in the global climate system, and aerosol–cloud interactions have a significant impact on the radiation balance, water cycle, and energy cycle of the Earth–atmosphere system. To understand the effect of aerosols on the vertical distribution of stratocumulus microphysical quantities in southwest China, we analyzed data from nine aircraft observations over Guangxi from 10 October to 3 November 2020. This analysis focused on the daylight variation characteristics and formation mechanisms of stratocumulus microphysical profiles, considering the influence of aerosol number concentration in relation to the source of air mass and individual cases. Aerosol number concentration (<span class="inline-formula"><i>N</i><sub>a</sub></span>) and cloud droplet concentration (<span class="inline-formula"><i>N</i><sub>c</sub></span>) decreased gradually with an altitude increase below 1500 m and did not change with a height between 1500 and 3300 m. The temperature inversion layer at the top of the planetary boundary layer (PBL) hindered the increase in the cloud droplet particle size. The lower layer of the stratocumulus cloud in Guangxi mainly contained small-sized cloud droplets (effective diameter of a cloud droplet (<span class="inline-formula"><i>E</i><sub>d</sub></span>) <span class="inline-formula"><</span> 15 <span class="inline-formula">µm</span>), and the middle and upper layers of cloud droplets were large-particle-size cloud droplets (<span class="inline-formula"><i>E</i><sub>d</sub></span> <span class="inline-formula">></span> 20 <span class="inline-formula">µm</span>). The vertical distribution of cloud microphysical quantity had apparent daylight variation. When aerosols in the PBL were transported to the upper air (14:00 to 20:00 Beijing time, BJT), <span class="inline-formula"><i>N</i><sub>c</sub></span> in the lower layer decreased, and the small-particle-size cloud droplets (<span class="inline-formula"><i>E</i><sub>d</sub></span> <span class="inline-formula"><</span> 20 <span class="inline-formula">µm</span>) in the middle layer and upper layer increased. Aerosols from the free atmosphere were transported into the PBL (10:00 to 13:00 BJT), providing an abundance of cloud condensation nuclei, which increased the number of small-particle-size cloud droplets in the lower layer of the cloud (near the top of the PBL). The characteristics of cloud microphysical quantities (<span class="inline-formula"><i>N</i><sub>c</sub></span> and <span class="inline-formula"><i>E</i><sub>d</sub></span>) were also affected by the source of air mass and the height of the PBL. <span class="inline-formula"><i>N</i><sub>a</sub></span> and <span class="inline-formula"><i>N</i><sub>c</sub></span> were high under the influence of land air mass or aerosols within the PBL, and the cloud droplet number concentration spectrum was unimodal. <span class="inline-formula"><i>N</i><sub>a</sub></span> and <span class="inline-formula"><i>N</i><sub>c</sub></span> were low under the influence of marine air mass or above the boundary layer, and the cloud droplet number concentration spectrum was bimodal. The relationship between stratocumulus and aerosol in this region is consistent with the Twomey effect. <span class="inline-formula"><i>E</i><sub>d</sub></span> and <span class="inline-formula"><i>N</i><sub>a</sub></span> remain negatively correlated in different liquid water content ranges, and the FIE (aerosol first indirect effect) ranged from <span class="inline-formula">−</span>0.07 to <span class="inline-formula">−</span>0.58.</p>https://acp.copernicus.org/articles/25/4151/2025/acp-25-4151-2025.pdf |
| spellingShingle | S. Liu H. Wang D. Zhao D. Zhao W. Zhou Y. Du Z. Zhang P. Cheng T. Zhao Y. Ke Z. Wu M. Huang Measurement report: Aircraft observations of aerosol and microphysical quantities of stratocumulus in autumn over Guangxi Province, China – daylight variation, vertical distribution, and aerosol–cloud interactions Atmospheric Chemistry and Physics |
| title | Measurement report: Aircraft observations of aerosol and microphysical quantities of stratocumulus in autumn over Guangxi Province, China – daylight variation, vertical distribution, and aerosol–cloud interactions |
| title_full | Measurement report: Aircraft observations of aerosol and microphysical quantities of stratocumulus in autumn over Guangxi Province, China – daylight variation, vertical distribution, and aerosol–cloud interactions |
| title_fullStr | Measurement report: Aircraft observations of aerosol and microphysical quantities of stratocumulus in autumn over Guangxi Province, China – daylight variation, vertical distribution, and aerosol–cloud interactions |
| title_full_unstemmed | Measurement report: Aircraft observations of aerosol and microphysical quantities of stratocumulus in autumn over Guangxi Province, China – daylight variation, vertical distribution, and aerosol–cloud interactions |
| title_short | Measurement report: Aircraft observations of aerosol and microphysical quantities of stratocumulus in autumn over Guangxi Province, China – daylight variation, vertical distribution, and aerosol–cloud interactions |
| title_sort | measurement report aircraft observations of aerosol and microphysical quantities of stratocumulus in autumn over guangxi province china daylight variation vertical distribution and aerosol cloud interactions |
| url | https://acp.copernicus.org/articles/25/4151/2025/acp-25-4151-2025.pdf |
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