TPU-assisted adhesive PDMS film for dry or underwater environments
Abstract Adhesive polymer films with anisotropic properties on either side have attracted tremendous interest for biomedical and engineering applications. However, developing an innovative solution that provides effective adhesion under both dry and wet conditions remains a considerable challenge. I...
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Nature Portfolio
2024-05-01
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Series: | NPG Asia Materials |
Online Access: | https://doi.org/10.1038/s41427-024-00546-8 |
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author | Sangyeun Park Minhyeok Kim Hongyun So |
author_facet | Sangyeun Park Minhyeok Kim Hongyun So |
author_sort | Sangyeun Park |
collection | DOAJ |
description | Abstract Adhesive polymer films with anisotropic properties on either side have attracted tremendous interest for biomedical and engineering applications. However, developing an innovative solution that provides effective adhesion under both dry and wet conditions remains a considerable challenge. In this study, we devised a novel process for creating adhesive films by casting polydimethylsiloxane (PDMS) onto a thermoplastic polyurethane (TPU) substrate. During the curing process, the PDMS layer in contact with the TPU was lightly cross-linked, which significantly increased adhesion. The catalytic reaction used for polymerization was regulated by the TPU, which is known to adsorb metal ions. This adhesive PDMS film (APF) demonstrated outstanding adhesion on various substrates under dry and underwater conditions and maintained adhesion even after repeated use. In practical applications, the APF proved to be an effective waterproof patch by adhering to the surfaces of objects submerged in water. |
format | Article |
id | doaj-art-1ee782a36d254cc3af7789d6f36135da |
institution | Kabale University |
issn | 1884-4057 |
language | English |
publishDate | 2024-05-01 |
publisher | Nature Portfolio |
record_format | Article |
series | NPG Asia Materials |
spelling | doaj-art-1ee782a36d254cc3af7789d6f36135da2025-01-19T12:28:59ZengNature PortfolioNPG Asia Materials1884-40572024-05-0116111010.1038/s41427-024-00546-8TPU-assisted adhesive PDMS film for dry or underwater environmentsSangyeun Park0Minhyeok Kim1Hongyun So2Department of Mechanical Engineering, Hanyang UniversityDepartment of Mechanical Engineering, Hanyang UniversityDepartment of Mechanical Engineering, Hanyang UniversityAbstract Adhesive polymer films with anisotropic properties on either side have attracted tremendous interest for biomedical and engineering applications. However, developing an innovative solution that provides effective adhesion under both dry and wet conditions remains a considerable challenge. In this study, we devised a novel process for creating adhesive films by casting polydimethylsiloxane (PDMS) onto a thermoplastic polyurethane (TPU) substrate. During the curing process, the PDMS layer in contact with the TPU was lightly cross-linked, which significantly increased adhesion. The catalytic reaction used for polymerization was regulated by the TPU, which is known to adsorb metal ions. This adhesive PDMS film (APF) demonstrated outstanding adhesion on various substrates under dry and underwater conditions and maintained adhesion even after repeated use. In practical applications, the APF proved to be an effective waterproof patch by adhering to the surfaces of objects submerged in water.https://doi.org/10.1038/s41427-024-00546-8 |
spellingShingle | Sangyeun Park Minhyeok Kim Hongyun So TPU-assisted adhesive PDMS film for dry or underwater environments NPG Asia Materials |
title | TPU-assisted adhesive PDMS film for dry or underwater environments |
title_full | TPU-assisted adhesive PDMS film for dry or underwater environments |
title_fullStr | TPU-assisted adhesive PDMS film for dry or underwater environments |
title_full_unstemmed | TPU-assisted adhesive PDMS film for dry or underwater environments |
title_short | TPU-assisted adhesive PDMS film for dry or underwater environments |
title_sort | tpu assisted adhesive pdms film for dry or underwater environments |
url | https://doi.org/10.1038/s41427-024-00546-8 |
work_keys_str_mv | AT sangyeunpark tpuassistedadhesivepdmsfilmfordryorunderwaterenvironments AT minhyeokkim tpuassistedadhesivepdmsfilmfordryorunderwaterenvironments AT hongyunso tpuassistedadhesivepdmsfilmfordryorunderwaterenvironments |