Visible Discrimination of Broadband Infrared Light by Dye-Enhanced Upconversion in Lanthanide-Doped Nanocrystals

Optical upconversion of near infrared light to visible light is an attractive way to capture the optical energy or optical information contained in low-energy photons that is otherwise lost to the human eye or to certain photodetectors and solar cells. Until the recent application of broadband absor...

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Main Authors: Charles G. Dupuy, Thomas L. Allen, George M. Williams, David Schut
Format: Article
Language:English
Published: Wiley 2014-01-01
Series:Journal of Nanotechnology
Online Access:http://dx.doi.org/10.1155/2014/538163
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author Charles G. Dupuy
Thomas L. Allen
George M. Williams
David Schut
author_facet Charles G. Dupuy
Thomas L. Allen
George M. Williams
David Schut
author_sort Charles G. Dupuy
collection DOAJ
description Optical upconversion of near infrared light to visible light is an attractive way to capture the optical energy or optical information contained in low-energy photons that is otherwise lost to the human eye or to certain photodetectors and solar cells. Until the recent application of broadband absorbing optical antennas, upconversion efficiency in lanthanide-doped nanocrystals was limited by the weak, narrow atomic absorption of a handful of sensitizer elements. In this work, we extend the role of the optical antenna to provide false-color, visible discrimination between bands of infrared radiation. By pairing different optical antenna dyes to specific nanoparticle compositions, unique visible emission is associated with different bands of infrared excitation. In one material set, the peak emission was increased 10-fold, and the width of the spectral response was increased more than 10-fold.
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institution Kabale University
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series Journal of Nanotechnology
spelling doaj-art-12916ed3835c4cd291b52b56b8042e882025-02-03T01:32:40ZengWileyJournal of Nanotechnology1687-95031687-95112014-01-01201410.1155/2014/538163538163Visible Discrimination of Broadband Infrared Light by Dye-Enhanced Upconversion in Lanthanide-Doped NanocrystalsCharles G. Dupuy0Thomas L. Allen1George M. Williams2David Schut3Voxtel Inc., 15985 NW Schendel Avenue Ste. 200, Beaverton, OR 97006, USAVoxtel Inc., 15985 NW Schendel Avenue Ste. 200, Beaverton, OR 97006, USAVoxtel Inc., 15985 NW Schendel Avenue Ste. 200, Beaverton, OR 97006, USAVoxtel Inc., 15985 NW Schendel Avenue Ste. 200, Beaverton, OR 97006, USAOptical upconversion of near infrared light to visible light is an attractive way to capture the optical energy or optical information contained in low-energy photons that is otherwise lost to the human eye or to certain photodetectors and solar cells. Until the recent application of broadband absorbing optical antennas, upconversion efficiency in lanthanide-doped nanocrystals was limited by the weak, narrow atomic absorption of a handful of sensitizer elements. In this work, we extend the role of the optical antenna to provide false-color, visible discrimination between bands of infrared radiation. By pairing different optical antenna dyes to specific nanoparticle compositions, unique visible emission is associated with different bands of infrared excitation. In one material set, the peak emission was increased 10-fold, and the width of the spectral response was increased more than 10-fold.http://dx.doi.org/10.1155/2014/538163
spellingShingle Charles G. Dupuy
Thomas L. Allen
George M. Williams
David Schut
Visible Discrimination of Broadband Infrared Light by Dye-Enhanced Upconversion in Lanthanide-Doped Nanocrystals
Journal of Nanotechnology
title Visible Discrimination of Broadband Infrared Light by Dye-Enhanced Upconversion in Lanthanide-Doped Nanocrystals
title_full Visible Discrimination of Broadband Infrared Light by Dye-Enhanced Upconversion in Lanthanide-Doped Nanocrystals
title_fullStr Visible Discrimination of Broadband Infrared Light by Dye-Enhanced Upconversion in Lanthanide-Doped Nanocrystals
title_full_unstemmed Visible Discrimination of Broadband Infrared Light by Dye-Enhanced Upconversion in Lanthanide-Doped Nanocrystals
title_short Visible Discrimination of Broadband Infrared Light by Dye-Enhanced Upconversion in Lanthanide-Doped Nanocrystals
title_sort visible discrimination of broadband infrared light by dye enhanced upconversion in lanthanide doped nanocrystals
url http://dx.doi.org/10.1155/2014/538163
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